Metastability in high entropy alloys

The high entropy effect is often insufficient to fully stabilize single-phase solid solutions (SPSS), yielding only few, mostly metastable SPSS. While the prospective space of favorable SPSS formation is smaller than commonly assumed, larger degrees of metastability can open up the vast High Entropy...

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Published inScripta materialia Vol. 186; no. C; pp. 392 - 400
Main Authors Kube, Sebastian A., Schroers, Jan
Format Journal Article
LanguageEnglish
Published United States Elsevier Ltd 01.09.2020
Elsevier
Subjects
Critical Cooling Rate
High Entropy Alloys
Materials Science
Metallic Glasses
Metallurgy & Metallurgical Engineering
Metastability
Science & Technology - Other Topics
Time-Temperature-Transformation Diagrams
Metallic Glasses
Time-Temperature-Transformation Diagrams
High Entropy Alloys
Critical Cooling Rate
Metastability
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Abstract The high entropy effect is often insufficient to fully stabilize single-phase solid solutions (SPSS), yielding only few, mostly metastable SPSS. While the prospective space of favorable SPSS formation is smaller than commonly assumed, larger degrees of metastability can open up the vast High Entropy Alloy space. We argue that HEAs form metastable SPSS through polymorphic solidification upon rapid cooling. To quantify a HEA's metastability, we propose the critical cooling rate of SPSS formation RCSPSS, analogous to RCGlass. Thereby, we can compare multicomponent alloys by their metastability and SPSS or glass forming ability, which is determined by their underlying atomic dispersity.
AbstractList Not provided.
The high entropy effect is often insufficient to fully stabilize single-phase solid solutions (SPSS), yielding only few, mostly metastable SPSS. While the prospective space of favorable SPSS formation is smaller than commonly assumed, larger degrees of metastability can open up the vast High Entropy Alloy space. We argue that HEAs form metastable SPSS through polymorphic solidification upon rapid cooling. To quantify a HEA's metastability, we propose the critical cooling rate of SPSS formation RCSPSS, analogous to RCGlass. Thereby, we can compare multicomponent alloys by their metastability and SPSS or glass forming ability, which is determined by their underlying atomic dispersity.
Author Kube, Sebastian A.
Schroers, Jan
Author_xml – sequence: 1
  givenname: Sebastian A.
  surname: Kube
  fullname: Kube, Sebastian A.
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  givenname: Jan
  surname: Schroers
  fullname: Schroers, Jan
  email: jan.schroers@yale.edu
BackLink https://www.osti.gov/biblio/1801611$$D View this record in Osti.gov
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Issue C
Keywords Metallic Glasses
Time-Temperature-Transformation Diagrams
High Entropy Alloys
Critical Cooling Rate
Metastability
Language English
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Snippet The high entropy effect is often insufficient to fully stabilize single-phase solid solutions (SPSS), yielding only few, mostly metastable SPSS. While the...
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SubjectTerms Critical Cooling Rate
High Entropy Alloys
Materials Science
Metallic Glasses
Metallurgy & Metallurgical Engineering
Metastability
Science & Technology - Other Topics
Time-Temperature-Transformation Diagrams
Title Metastability in high entropy alloys
URI https://dx.doi.org/10.1016/j.scriptamat.2020.05.049
https://www.osti.gov/biblio/1801611
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