Polyoxometalates (POMs): from electroactive clusters to energy materials

Polyoxometalates (POMs) represent a class of nanomaterials, which hold enormous promise for a range of energy-related applications. Their promise is owing to their "special" structure that gives POMs a truly unique ability to control redox reactions in energy conversion and storage. One su...

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Published inEnergy & environmental science Vol. 14; no. 4; pp. 1652 - 17
Main Authors Horn, Michael R, Singh, Amandeep, Alomari, Suaad, Goberna-Ferrón, Sara, Benages-Vilau, Raúl, Chodankar, Nilesh, Motta, Nunzio, Ostrikov, Kostya (Ken), MacLeod, Jennifer, Sonar, Prashant, Gomez-Romero, Pedro, Dubal, Deepak
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 2021
Subjects
Catalysts
chemical compound
Coordination compounds
Determinant factors
electrochemical method
Energy
Energy applications
Energy conversion
Energy conversion and storages
Energy storage
Fundamental studies
Metal oxides
Metals
Molecular clusters
Nanomaterials
Nanotechnology
Oxygen atoms
Polyoxometalates
Polyoxometallates
Redox reactions
Redox-active sites
Stability
Structure property
Three-dimensional clusters
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Abstract Polyoxometalates (POMs) represent a class of nanomaterials, which hold enormous promise for a range of energy-related applications. Their promise is owing to their "special" structure that gives POMs a truly unique ability to control redox reactions in energy conversion and storage. One such amazing capability is their large number of redox active sites that arises from the complex three-dimensional cluster of metal-oxide ions linked together by oxygen atoms. Here, a critical review on how POMs emerged from being molecular clusters for fundamental studies, to next-generation materials for energy applications is provided. We highlight how exploiting the versatility and activity of these molecules can lead to improved performance in energy devices such as supercapacitors and batteries, and in energy catalyst applications. The potential of POMs across numerous fields is systematically outlined by investigating structure-property-performance relationships and the determinant factors for energy systems. Finally, the challenges and opportunities for this class of materials with respect to addressing our pressing energy-related concerns are identified. Polyoxometalates as anionic molecular metal oxides clusters with open frameworks and rich redox chemistry have outstanding versatility in energy conversion and storage research.
AbstractList Polyoxometalates (POMs) represent a class of nanomaterials, which hold enormous promise for a range of energy-related applications. Their promise is owing to their “special” structure that gives POMs a truly unique ability to control redox reactions in energy conversion and storage. One such amazing capability is their large number of redox active sites that arises from the complex three-dimensional cluster of metal-oxide ions linked together by oxygen atoms. Here, a critical review on how POMs emerged from being molecular clusters for fundamental studies, to next-generation materials for energy applications is provided. We highlight how exploiting the versatility and activity of these molecules can lead to improved performance in energy devices such as supercapacitors and batteries, and in energy catalyst applications. The potential of POMs across numerous fields is systematically outlined by investigating structure–property–performance relationships and the determinant factors for energy systems. Finally, the challenges and opportunities for this class of materials with respect to addressing our pressing energy-related concerns are identified.
Polyoxometalates (POMs) represent a class of nanomaterials, which hold enormous promise for a range of energy-related applications. Their promise is owing to their "special"structure that gives POMs a truly unique ability to control redox reactions in energy conversion and storage. One such amazing capability is their large number of redox active sites that arises from the complex three-dimensional cluster of metal-oxide ions linked together by oxygen atoms. Here, a critical review on how POMs emerged from being molecular clusters for fundamental studies, to next-generation materials for energy applications is provided. We highlight how exploiting the versatility and activity of these molecules can lead to improved performance in energy devices such as supercapacitors and batteries, and in energy catalyst applications. The potential of POMs across numerous fields is systematically outlined by investigating structure-property-performance relationships and the determinant factors for energy systems. Finally, the challenges and opportunities for this class of materials with respect to addressing our pressing energy-related concerns are identified. This journal is © The Royal Society of Chemistry.
Polyoxometalates (POMs) represent a class of nanomaterials, which hold enormous promise for a range of energy-related applications. Their promise is owing to their "special" structure that gives POMs a truly unique ability to control redox reactions in energy conversion and storage. One such amazing capability is their large number of redox active sites that arises from the complex three-dimensional cluster of metal-oxide ions linked together by oxygen atoms. Here, a critical review on how POMs emerged from being molecular clusters for fundamental studies, to next-generation materials for energy applications is provided. We highlight how exploiting the versatility and activity of these molecules can lead to improved performance in energy devices such as supercapacitors and batteries, and in energy catalyst applications. The potential of POMs across numerous fields is systematically outlined by investigating structure-property-performance relationships and the determinant factors for energy systems. Finally, the challenges and opportunities for this class of materials with respect to addressing our pressing energy-related concerns are identified. Polyoxometalates as anionic molecular metal oxides clusters with open frameworks and rich redox chemistry have outstanding versatility in energy conversion and storage research.
Author Horn, Michael R
Ostrikov, Kostya (Ken)
Motta, Nunzio
Alomari, Suaad
Gomez-Romero, Pedro
Sonar, Prashant
Dubal, Deepak
Chodankar, Nilesh
Singh, Amandeep
Benages-Vilau, Raúl
Goberna-Ferrón, Sara
MacLeod, Jennifer
AuthorAffiliation ICN2 (CSIC-BIST) Campus UAB
School of Chemistry and Physics
Queensland University of Technology (QUT)
Catalan Institute of Nanoscience and Nanotechnology
Department of Energy and Materials Engineering
Dongguk University-Seoul
Centre for Materials Science
Consejo Superior de Investigaciones Científicas (CSIC)
AuthorAffiliation_xml – name: School of Chemistry and Physics
– name: ICN2 (CSIC-BIST) Campus UAB
– name: Dongguk University-Seoul
– name: Consejo Superior de Investigaciones Científicas (CSIC)
– name: Department of Energy and Materials Engineering
– name: Catalan Institute of Nanoscience and Nanotechnology
– name: Queensland University of Technology (QUT)
– name: Centre for Materials Science
Author_xml – sequence: 1
  givenname: Michael R
  surname: Horn
  fullname: Horn, Michael R
– sequence: 2
  givenname: Amandeep
  surname: Singh
  fullname: Singh, Amandeep
– sequence: 3
  givenname: Suaad
  surname: Alomari
  fullname: Alomari, Suaad
– sequence: 4
  givenname: Sara
  surname: Goberna-Ferrón
  fullname: Goberna-Ferrón, Sara
– sequence: 5
  givenname: Raúl
  surname: Benages-Vilau
  fullname: Benages-Vilau, Raúl
– sequence: 6
  givenname: Nilesh
  surname: Chodankar
  fullname: Chodankar, Nilesh
– sequence: 7
  givenname: Nunzio
  surname: Motta
  fullname: Motta, Nunzio
– sequence: 8
  givenname: Kostya (Ken)
  surname: Ostrikov
  fullname: Ostrikov, Kostya (Ken)
– sequence: 9
  givenname: Jennifer
  surname: MacLeod
  fullname: MacLeod, Jennifer
– sequence: 10
  givenname: Prashant
  surname: Sonar
  fullname: Sonar, Prashant
– sequence: 11
  givenname: Pedro
  surname: Gomez-Romero
  fullname: Gomez-Romero, Pedro
– sequence: 12
  givenname: Deepak
  surname: Dubal
  fullname: Dubal, Deepak
BackLink https://urn.kb.se/resolve?urn=urn:nbn:se:miun:diva-43435$$DView record from Swedish Publication Index
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Notes Research team at Catalan Institute of Nanoscience and Nanotechnology (ICN2), Spain. From left to right: Dr Raúl Benages-Vilau (Post-Doctoral Fellow), Prof. Pedro Gomez-Romero (Professor), Dr Sara Goberna-Ferrón (Beatriu de Pinós Post-Doctoral Fellow). The team is expert in hybrid organic-inorganic materials, graphene, nanocomposites for energy storage and conversion (lithium batteries, supercapacitors, flow batteries, solar-thermal energy, nanofluids).
Research team at Queensland University of Technology (QUT), Australia. Front row from left to right: Mr Michael Horn (PhD student), Mr Amandeep Singh (PhD student) and Dr Deepak Dubal (Associate Professor). Back row from left to right: Dr Prashant Sonar (Associate Professor), Dr Jennifer MacLeod (Associate Professor) and Prof. Nunzio Motta (Professor). We miss Ms. Suaad Alomari, Dr Nilesh Chodankar and Prof. Kostya (Ken) Ostrikov in the photo. The research of QUT team is focused on graphene, oxides, polymers, polyoxometalates (POMs), surface science, energy conversion and storage devices, and organic semiconducting materials for electronic devices.
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Snippet Polyoxometalates (POMs) represent a class of nanomaterials, which hold enormous promise for a range of energy-related applications. Their promise is owing to...
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SubjectTerms Catalysts
chemical compound
Coordination compounds
Determinant factors
electrochemical method
Energy
Energy applications
Energy conversion
Energy conversion and storages
Energy storage
Fundamental studies
Metal oxides
Metals
Molecular clusters
Nanomaterials
Nanotechnology
Oxygen atoms
Polyoxometalates
Polyoxometallates
Redox reactions
Redox-active sites
Stability
Structure property
Three-dimensional clusters
Title Polyoxometalates (POMs): from electroactive clusters to energy materials
URI https://www.proquest.com/docview/2515763737
https://urn.kb.se/resolve?urn=urn:nbn:se:miun:diva-43435
Volume 14
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