Constructing heterojunctions by surface sulfidation for efficient inverted perovskite solar cells
A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)–rich perovskite films. The formed lead-sulfur (Pb-S) bonds upshifted the Fermi level at the perovskite interface and induced an extra back-surface field for electron extraction. The r...
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| Published in | Science (American Association for the Advancement of Science) Vol. 375; no. 6579; pp. 434 - 437 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
The American Association for the Advancement of Science
28.01.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)–rich perovskite films. The formed lead-sulfur (Pb-S) bonds upshifted the Fermi level at the perovskite interface and induced an extra back-surface field for electron extraction. The resulting inverted devices exhibited a power conversion efficiency (PCE) >24% with a high open-circuit voltage of 1.19 volts, corresponding to a low voltage loss of 0.36 volts. The strong Pb-S bonds could stabilize perovskite heterojunctions and strengthen underlying perovskite structures that have a similar crystal lattice. Devices with surface sulfidation retained more than 90% of the initial PCE after aging at 85°C for 2200 hours or operating at the maximum power point under continuous illumination for 1000 hours at 55° ± 5°C.
Perovskite solar cells (PSCs) with high power conversion efficiency (PCE) and stability have been reported in regular n-i-p devices, but inverted p-i-n PSCs that could be easier to use in tandem solar cells usually have lower PCEs (22 to 23%) Li
et al
. sulfurized a lead-rich layer with hexamethyldisilathiane, and the lead-sulfur bonds shifted the Fermi level of perovskite-transporter layer interface to create an electric field that enhanced electron extraction. The inverted PSCs had PCEs >24%, and the strong lead-sulfur bonds helped to maintain >90% of this efficiency during illuminated operation for 1000 hours at 55°C and after dark aging at 85°C for 2200 hours. —PDS
Surface sulfidation of perovskite film increases its stability and improves electron extraction through band bending. |
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| AbstractList | A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)–rich perovskite films. The formed lead-sulfur (Pb-S) bonds upshifted the Fermi level at the perovskite interface and induced an extra back-surface field for electron extraction. The resulting inverted devices exhibited a power conversion efficiency (PCE) >24% with a high open-circuit voltage of 1.19 volts, corresponding to a low voltage loss of 0.36 volts. The strong Pb-S bonds could stabilize perovskite heterojunctions and strengthen underlying perovskite structures that have a similar crystal lattice. Devices with surface sulfidation retained more than 90% of the initial PCE after aging at 85°C for 2200 hours or operating at the maximum power point under continuous illumination for 1000 hours at 55° ± 5°C.
Perovskite solar cells (PSCs) with high power conversion efficiency (PCE) and stability have been reported in regular n-i-p devices, but inverted p-i-n PSCs that could be easier to use in tandem solar cells usually have lower PCEs (22 to 23%) Li
et al
. sulfurized a lead-rich layer with hexamethyldisilathiane, and the lead-sulfur bonds shifted the Fermi level of perovskite-transporter layer interface to create an electric field that enhanced electron extraction. The inverted PSCs had PCEs >24%, and the strong lead-sulfur bonds helped to maintain >90% of this efficiency during illuminated operation for 1000 hours at 55°C and after dark aging at 85°C for 2200 hours. —PDS
Surface sulfidation of perovskite film increases its stability and improves electron extraction through band bending. Inverted solar cells’ surface sulfidationPerovskite solar cells (PSCs) with high power conversion efficiency (PCE) and stability have been reported in regular n-i-p devices, but inverted p-i-n PSCs that could be easier to use in tandem solar cells usually have lower PCEs (22 to 23%) Li et al. sulfurized a lead-rich layer with hexamethyldisilathiane, and the lead-sulfur bonds shifted the Fermi level of perovskite-transporter layer interface to create an electric field that enhanced electron extraction. The inverted PSCs had PCEs >24%, and the strong lead-sulfur bonds helped to maintain >90% of this efficiency during illuminated operation for 1000 hours at 55°C and after dark aging at 85°C for 2200 hours. —PDS A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)-rich perovskite films. The formed lead-sulfur (Pb-S) bonds upshifted the Fermi level at the perovskite interface and induced an extra back-surface field for electron extraction. The resulting inverted devices exhibited a power conversion efficiency (PCE) >24% with a high open-circuit voltage of 1.19 volts, corresponding to a low voltage loss of 0.36 volts. The strong Pb-S bonds could stabilize perovskite heterojunctions and strengthen underlying perovskite structures that have a similar crystal lattice. Devices with surface sulfidation retained more than 90% of the initial PCE after aging at 85°C for 2200 hours or operating at the maximum power point under continuous illumination for 1000 hours at 55° ± 5°C. A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)-rich perovskite films. The formed lead-sulfur (Pb-S) bonds upshifted the Fermi level at the perovskite interface and induced an extra back-surface field for electron extraction. The resulting inverted devices exhibited a power conversion efficiency (PCE) >24% with a high open-circuit voltage of 1.19 volts, corresponding to a low voltage loss of 0.36 volts. The strong Pb-S bonds could stabilize perovskite heterojunctions and strengthen underlying perovskite structures that have a similar crystal lattice. Devices with surface sulfidation retained more than 90% of the initial PCE after aging at 85°C for 2200 hours or operating at the maximum power point under continuous illumination for 1000 hours at 55° ± 5°C.A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)-rich perovskite films. The formed lead-sulfur (Pb-S) bonds upshifted the Fermi level at the perovskite interface and induced an extra back-surface field for electron extraction. The resulting inverted devices exhibited a power conversion efficiency (PCE) >24% with a high open-circuit voltage of 1.19 volts, corresponding to a low voltage loss of 0.36 volts. The strong Pb-S bonds could stabilize perovskite heterojunctions and strengthen underlying perovskite structures that have a similar crystal lattice. Devices with surface sulfidation retained more than 90% of the initial PCE after aging at 85°C for 2200 hours or operating at the maximum power point under continuous illumination for 1000 hours at 55° ± 5°C. |
| Author | Li, Xiaodong Wei, Jiyao Zhang, Wenxiao Fang, Junfeng Lu, Chunyan Guo, Xuemin |
| Author_xml | – sequence: 1 givenname: Xiaodong orcidid: 0000-0003-0184-008X surname: Li fullname: Li, Xiaodong organization: School of Physics and Electronic Science, Engineering Research Center of Nanophotonics and Advanced Instrument, Ministry of Education, East China Normal University, Shanghai 200062, China – sequence: 2 givenname: Wenxiao surname: Zhang fullname: Zhang, Wenxiao organization: School of Physics and Electronic Science, Engineering Research Center of Nanophotonics and Advanced Instrument, Ministry of Education, East China Normal University, Shanghai 200062, China – sequence: 3 givenname: Xuemin surname: Guo fullname: Guo, Xuemin organization: School of Physics and Electronic Science, Engineering Research Center of Nanophotonics and Advanced Instrument, Ministry of Education, East China Normal University, Shanghai 200062, China – sequence: 4 givenname: Chunyan surname: Lu fullname: Lu, Chunyan organization: School of Physics and Electronic Science, Engineering Research Center of Nanophotonics and Advanced Instrument, Ministry of Education, East China Normal University, Shanghai 200062, China – sequence: 5 givenname: Jiyao surname: Wei fullname: Wei, Jiyao organization: School of Physics and Electronic Science, Engineering Research Center of Nanophotonics and Advanced Instrument, Ministry of Education, East China Normal University, Shanghai 200062, China – sequence: 6 givenname: Junfeng orcidid: 0000-0003-2094-8678 surname: Fang fullname: Fang, Junfeng organization: School of Physics and Electronic Science, Engineering Research Center of Nanophotonics and Advanced Instrument, Ministry of Education, East China Normal University, Shanghai 200062, China., Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35084976$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
| Copyright | Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works |
| Copyright_xml | – notice: Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works |
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| DOI | 10.1126/science.abl5676 |
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| Snippet | A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)–rich perovskite films. The formed... A stable perovskite heterojunction was constructed for inverted solar cells through surface sulfidation of lead (Pb)-rich perovskite films. The formed... Inverted solar cells’ surface sulfidationPerovskite solar cells (PSCs) with high power conversion efficiency (PCE) and stability have been reported in regular... |
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| SubjectTerms | Aging Bonding strength Electric fields Energy conversion efficiency Heterojunctions Perovskites Photovoltaic cells Solar cells Sulfidation Sulfur |
| Title | Constructing heterojunctions by surface sulfidation for efficient inverted perovskite solar cells |
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