High thermoelectric performance realized through manipulating layered phonon-electron decoupling
Thermoelectric materials allow for direct conversion between heat and electricity, offering the potential for power generation. The average dimensionless figure of merit ZT ave determines device efficiency. N-type tin selenide crystals exhibit outstanding three-dimensional charge and two-dimensional...
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| Published in | Science (American Association for the Advancement of Science) Vol. 375; no. 6587; pp. 1385 - 1389 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
The American Association for the Advancement of Science
25.03.2022
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Thermoelectric materials allow for direct conversion between heat and electricity, offering the potential for power generation. The average dimensionless figure of merit
ZT
ave
determines device efficiency. N-type tin selenide crystals exhibit outstanding three-dimensional charge and two-dimensional phonon transport along the out-of-plane direction, contributing to a high maximum figure of merit
Z
max
of ~3.6 × 10
−3
per kelvin but a moderate
ZT
ave
of ~1.1. We found an attractive high
Z
max
of ~4.1 × 10
−3
per kelvin at 748 kelvin and a
ZT
ave
of ~1.7 at 300 to 773 kelvin in chlorine-doped and lead-alloyed tin selenide crystals by phonon-electron decoupling. The chlorine-induced low deformation potential improved the carrier mobility. The lead-induced mass and strain fluctuations reduced the lattice thermal conductivity. Phonon-electron decoupling plays a critical role to achieve high-performance thermoelectrics.
Thermoelectic materials convert heat to electricity and are attractive for energy generation or solid-state cooling. Su
et al
. found that doping tin selenide with chlorine and lead substantially improved the thermoelectric figure of merit over a wide temperature range. This effect was mostly due to an improvement in the material’s deformation potential related to mass and strain fluctuations introduced into the n-type material. Improving the figure of merit in this way is challenging because properties are often intertwined and trying to improve one will often degrade others. —BG
Doping tin selenide with lead and chlorine results in a material with high thermoelectric efficiency over a broad temperature range. |
|---|---|
| AbstractList | Thermoelectric materials allow for direct conversion between heat and electricity, offering the potential for power generation. The average dimensionless figure of merit ZTave determines device efficiency. N-type tin selenide crystals exhibit outstanding three-dimensional charge and two-dimensional phonon transport along the out-of-plane direction, contributing to a high maximum figure of merit Zmax of ~3.6 × 10-3 per kelvin but a moderate ZTave of ~1.1. We found an attractive high Zmax of ~4.1 × 10-3 per kelvin at 748 kelvin and a ZTave of ~1.7 at 300 to 773 kelvin in chlorine-doped and lead-alloyed tin selenide crystals by phonon-electron decoupling. The chlorine-induced low deformation potential improved the carrier mobility. The lead-induced mass and strain fluctuations reduced the lattice thermal conductivity. Phonon-electron decoupling plays a critical role to achieve high-performance thermoelectrics.Thermoelectric materials allow for direct conversion between heat and electricity, offering the potential for power generation. The average dimensionless figure of merit ZTave determines device efficiency. N-type tin selenide crystals exhibit outstanding three-dimensional charge and two-dimensional phonon transport along the out-of-plane direction, contributing to a high maximum figure of merit Zmax of ~3.6 × 10-3 per kelvin but a moderate ZTave of ~1.1. We found an attractive high Zmax of ~4.1 × 10-3 per kelvin at 748 kelvin and a ZTave of ~1.7 at 300 to 773 kelvin in chlorine-doped and lead-alloyed tin selenide crystals by phonon-electron decoupling. The chlorine-induced low deformation potential improved the carrier mobility. The lead-induced mass and strain fluctuations reduced the lattice thermal conductivity. Phonon-electron decoupling plays a critical role to achieve high-performance thermoelectrics. Thermoelectric materials allow for direct conversion between heat and electricity, offering the potential for power generation. The average dimensionless figure of merit determines device efficiency. N-type tin selenide crystals exhibit outstanding three-dimensional charge and two-dimensional phonon transport along the out-of-plane direction, contributing to a high maximum figure of merit of ~3.6 × 10 per kelvin but a moderate of ~1.1. We found an attractive high of ~4.1 × 10 per kelvin at 748 kelvin and a of ~1.7 at 300 to 773 kelvin in chlorine-doped and lead-alloyed tin selenide crystals by phonon-electron decoupling. The chlorine-induced low deformation potential improved the carrier mobility. The lead-induced mass and strain fluctuations reduced the lattice thermal conductivity. Phonon-electron decoupling plays a critical role to achieve high-performance thermoelectrics. Thermoelectric materials allow for direct conversion between heat and electricity, offering the potential for power generation. The average dimensionless figure of merit ZT ave determines device efficiency. N-type tin selenide crystals exhibit outstanding three-dimensional charge and two-dimensional phonon transport along the out-of-plane direction, contributing to a high maximum figure of merit Z max of ~3.6 × 10 −3 per kelvin but a moderate ZT ave of ~1.1. We found an attractive high Z max of ~4.1 × 10 −3 per kelvin at 748 kelvin and a ZT ave of ~1.7 at 300 to 773 kelvin in chlorine-doped and lead-alloyed tin selenide crystals by phonon-electron decoupling. The chlorine-induced low deformation potential improved the carrier mobility. The lead-induced mass and strain fluctuations reduced the lattice thermal conductivity. Phonon-electron decoupling plays a critical role to achieve high-performance thermoelectrics. Thermoelectic materials convert heat to electricity and are attractive for energy generation or solid-state cooling. Su et al . found that doping tin selenide with chlorine and lead substantially improved the thermoelectric figure of merit over a wide temperature range. This effect was mostly due to an improvement in the material’s deformation potential related to mass and strain fluctuations introduced into the n-type material. Improving the figure of merit in this way is challenging because properties are often intertwined and trying to improve one will often degrade others. —BG Doping tin selenide with lead and chlorine results in a material with high thermoelectric efficiency over a broad temperature range. A material with high potentialThermoelectic materials convert heat to electricity and are attractive for energy generation or solid-state cooling. Su et al. found that doping tin selenide with chlorine and lead substantially improved the thermoelectric figure of merit over a wide temperature range. This effect was mostly due to an improvement in the material’s deformation potential related to mass and strain fluctuations introduced into the n-type material. Improving the figure of merit in this way is challenging because properties are often intertwined and trying to improve one will often degrade others. —BG |
| Author | Zhao, Li-Dong Qin, Bingchao Wang, Sining Jin, Yang Wang, Yuping Qin, Yongxin Chang, Cheng Su, Lizhong Wang, Dongyang |
| Author_xml | – sequence: 1 givenname: Lizhong orcidid: 0000-0002-3313-0886 surname: Su fullname: Su, Lizhong organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 2 givenname: Dongyang orcidid: 0000-0001-8149-7394 surname: Wang fullname: Wang, Dongyang organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 3 givenname: Sining orcidid: 0000-0001-7630-4041 surname: Wang fullname: Wang, Sining organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 4 givenname: Bingchao orcidid: 0000-0003-2720-5922 surname: Qin fullname: Qin, Bingchao organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 5 givenname: Yuping orcidid: 0000-0001-8080-7338 surname: Wang fullname: Wang, Yuping organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 6 givenname: Yongxin orcidid: 0000-0002-1699-1369 surname: Qin fullname: Qin, Yongxin organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 7 givenname: Yang orcidid: 0000-0002-8084-761X surname: Jin fullname: Jin, Yang organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China – sequence: 8 givenname: Cheng orcidid: 0000-0002-9515-4277 surname: Chang fullname: Chang, Cheng organization: Institute of Science and Technology Austria, 3400 Klosterneuburg, Austria – sequence: 9 givenname: Li-Dong orcidid: 0000-0003-1247-4345 surname: Zhao fullname: Zhao, Li-Dong organization: School of Materials Science and Engineering, Beihang University, Beijing 100191, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35324303$$D View this record in MEDLINE/PubMed |
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| Title | High thermoelectric performance realized through manipulating layered phonon-electron decoupling |
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