Fabrication of ZnO quantum dots@SnO2 hollow nanospheres hybrid hierarchical structures for effectively detecting formaldehyde
•ZnO QDs@SnO2 HNSs hybrid hierarchical structures were fabricated by modifying ZnO quantum dots on the surface of SnO2 hollow nanospheres.•ZnO QDs@SnO2 HNSs hybrid hierarchical structures shows selective response to formaldehyde among four kinds of confusable indoor VOCs.•ZnO QDs@SnO2 HNSs hybrid hi...
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| Published in | Sensors and actuators. B, Chemical Vol. 318; p. 128222 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Lausanne
Elsevier B.V
01.09.2020
Elsevier Science Ltd |
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| Abstract | •ZnO QDs@SnO2 HNSs hybrid hierarchical structures were fabricated by modifying ZnO quantum dots on the surface of SnO2 hollow nanospheres.•ZnO QDs@SnO2 HNSs hybrid hierarchical structures shows selective response to formaldehyde among four kinds of confusable indoor VOCs.•ZnO QDs@SnO2 HNSs hybrid hierarchical structures exhibited superior sensing performance to formaldehyde which could be attributed to the special structure and the heterojunctions between ZnO and SnO2.
The ZnO quantum dots modified SnO2 hollow nanospheres (ZnO QDs@SnO2 HNSs) hybrid hierarchical structures were fabricated by modifying ZnO QDs on the surface of SnO2 HNSs using precipitation and hydrothermal method. The gas sensors based on ZnO QDs, SnO2 HNSs and ZnO QDs@SnO2 HNSs present superior sensing properties to formaldehyde compared with three other typical indoor volatile organic compounds (VOCs, including formaldehyde, toluene, benzene and ammonia). In particular, the ZnO QDs@SnO2 HNSs based sensor exhibits high response (36.5–50 ppm), good linearity (1−1000 ppm), rapid response/recovery time (9 s/ 10 s), ultra-low limit of detection (LOD, 5 ppb) and excellent long-term stability. The ZnO QDs@SnO2 HNSs hybrid hierarchical structures not only ensure the porosity but also create lots of heterojunctions, which is benefit for improving the gas sensing properties of a gas sensor. |
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| AbstractList | •ZnO QDs@SnO2 HNSs hybrid hierarchical structures were fabricated by modifying ZnO quantum dots on the surface of SnO2 hollow nanospheres.•ZnO QDs@SnO2 HNSs hybrid hierarchical structures shows selective response to formaldehyde among four kinds of confusable indoor VOCs.•ZnO QDs@SnO2 HNSs hybrid hierarchical structures exhibited superior sensing performance to formaldehyde which could be attributed to the special structure and the heterojunctions between ZnO and SnO2.
The ZnO quantum dots modified SnO2 hollow nanospheres (ZnO QDs@SnO2 HNSs) hybrid hierarchical structures were fabricated by modifying ZnO QDs on the surface of SnO2 HNSs using precipitation and hydrothermal method. The gas sensors based on ZnO QDs, SnO2 HNSs and ZnO QDs@SnO2 HNSs present superior sensing properties to formaldehyde compared with three other typical indoor volatile organic compounds (VOCs, including formaldehyde, toluene, benzene and ammonia). In particular, the ZnO QDs@SnO2 HNSs based sensor exhibits high response (36.5–50 ppm), good linearity (1−1000 ppm), rapid response/recovery time (9 s/ 10 s), ultra-low limit of detection (LOD, 5 ppb) and excellent long-term stability. The ZnO QDs@SnO2 HNSs hybrid hierarchical structures not only ensure the porosity but also create lots of heterojunctions, which is benefit for improving the gas sensing properties of a gas sensor. The ZnO quantum dots modified SnO2 hollow nanospheres (ZnO QDs@SnO2 HNSs) hybrid hierarchical structures were fabricated by modifying ZnO QDs on the surface of SnO2 HNSs using precipitation and hydrothermal method. The gas sensors based on ZnO QDs, SnO2 HNSs and ZnO QDs@SnO2 HNSs present superior sensing properties to formaldehyde compared with three other typical indoor volatile organic compounds (VOCs, including formaldehyde, toluene, benzene and ammonia). In particular, the ZnO QDs@SnO2 HNSs based sensor exhibits high response (36.5–50 ppm), good linearity (1−1000 ppm), rapid response/recovery time (9 s/ 10 s), ultra-low limit of detection (LOD, 5 ppb) and excellent long-term stability. The ZnO QDs@SnO2 HNSs hybrid hierarchical structures not only ensure the porosity but also create lots of heterojunctions, which is benefit for improving the gas sensing properties of a gas sensor. |
| ArticleNumber | 128222 |
| Author | Sun, Yongjiao Suematsu, Koichi Yu, Zhichao Zhang, Wendong Hu, Jie Li, Pengwei Yang, Haoyue Zhao, Zhenting |
| Author_xml | – sequence: 1 givenname: Yongjiao orcidid: 0000-0003-0368-6987 surname: Sun fullname: Sun, Yongjiao email: sunyongjiao@tyut.edu.cn organization: Micro and Nano System Research Center, College of Information and Computer, Center of Nano Energy and Devices, Taiyuan University of Technology, Taiyuan, 030024, PR China – sequence: 2 givenname: Haoyue surname: Yang fullname: Yang, Haoyue organization: Micro and Nano System Research Center, College of Information and Computer, Center of Nano Energy and Devices, Taiyuan University of Technology, Taiyuan, 030024, PR China – sequence: 3 givenname: Zhenting surname: Zhao fullname: Zhao, Zhenting organization: Laboratory of Electronic Functional Materials, Huizhou University, Huizhou, 516001, PR China – sequence: 4 givenname: Koichi orcidid: 0000-0002-6170-447X surname: Suematsu fullname: Suematsu, Koichi organization: Department of Advanced Materials Science and Engineering, Faculty of Engineering Sciences, Kyushu University, Kasuga, Fukuoka, 816-8580, Japan – sequence: 5 givenname: Pengwei orcidid: 0000-0002-6199-4294 surname: Li fullname: Li, Pengwei organization: Micro and Nano System Research Center, College of Information and Computer, Center of Nano Energy and Devices, Taiyuan University of Technology, Taiyuan, 030024, PR China – sequence: 6 givenname: Zhichao surname: Yu fullname: Yu, Zhichao organization: Micro and Nano System Research Center, College of Information and Computer, Center of Nano Energy and Devices, Taiyuan University of Technology, Taiyuan, 030024, PR China – sequence: 7 givenname: Wendong surname: Zhang fullname: Zhang, Wendong organization: Micro and Nano System Research Center, College of Information and Computer, Center of Nano Energy and Devices, Taiyuan University of Technology, Taiyuan, 030024, PR China – sequence: 8 givenname: Jie orcidid: 0000-0003-0713-3458 surname: Hu fullname: Hu, Jie organization: Micro and Nano System Research Center, College of Information and Computer, Center of Nano Energy and Devices, Taiyuan University of Technology, Taiyuan, 030024, PR China |
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| Keywords | SnO2 hollow nanospheres Hybrid hierarchical structures Gas sensor ZnO quantum dots Formaldehyde |
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| Snippet | •ZnO QDs@SnO2 HNSs hybrid hierarchical structures were fabricated by modifying ZnO quantum dots on the surface of SnO2 hollow nanospheres.•ZnO QDs@SnO2 HNSs... The ZnO quantum dots modified SnO2 hollow nanospheres (ZnO QDs@SnO2 HNSs) hybrid hierarchical structures were fabricated by modifying ZnO QDs on the surface of... |
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| SubjectTerms | Ammonia Benzene Formaldehyde Gas sensor Gas sensors Heterojunctions Hybrid hierarchical structures Linearity Nanospheres Porosity Quantum dots Recovery time SnO2 hollow nanospheres Structural hierarchy Tin dioxide Toluene VOCs Volatile organic compounds Zinc oxide ZnO quantum dots |
| Title | Fabrication of ZnO quantum dots@SnO2 hollow nanospheres hybrid hierarchical structures for effectively detecting formaldehyde |
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