Separation and concentration of rare earth elements from wastewater using electrodialysis technology

•The ED technique shows promising potential for REEs recovery and removal.•The effect of ED operating parameters on REE removal and recovery was studied.•The presence of competing ions influences REE recovery and removal efficiency.•The energy consumption of ED processes using CC and CV modes was co...

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Published inSeparation and purification technology Vol. 254; p. 117442
Main Authors Li, Changbai, Ramasamy, Deepika L., Sillanpää, Mika, Repo, Eveliina
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.01.2021
Subjects
Electrodialysis
Energy consumption
Membrane
Rare earth elements
Scandium
Energy consumption
Membrane
Rare earth elements
Scandium
Electrodialysis
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Abstract •The ED technique shows promising potential for REEs recovery and removal.•The effect of ED operating parameters on REE removal and recovery was studied.•The presence of competing ions influences REE recovery and removal efficiency.•The energy consumption of ED processes using CC and CV modes was compared. Rare earth elements (REEs) including Scandium (Sc) are critical raw materials which are greatly needed in the advancement of many modern technologies. Due to the problems associated with the primary extraction of mining ores, the procurement of Sc and REEs from the secondary resources are currently explored adopting the principle of sustainability and circular economy. Herein, for the first time, the Electrodialysis (ED) technology based on electrochemical membrane separation process is successfully applied to separate and concentrate REEs from the diluted aqueous system. The overall performance of ED process in the recovery of Sc3+ ions from the wastewater was assessed by applied current, voltage, feed concentration, feed pH, co-ion competition and the overall energy consumption of the process. The REE recovery using the ED process was subjected to systematic investigations using both chronopotentiometric and chronoamperometric analyses. The results showed that ED process could be very promising in the recovery of Sc3+ ions (~99.52% removal) from the diluted wastewater, consuming the energy of only 0.26 kWh/m3 when operated at constant voltage mode (Sc3+ concentration of 20 ppm, pH 4, 1 h).
AbstractList Rare earth elements (REEs) including Scandium (Sc) are critical raw materials which are greatly needed in the advancement of many modern technologies. Due to the problems associated with the primary extraction of mining ores, the procurement of Sc and REEs from the secondary resources are currently explored adopting the principle of sustainability and circular economy. Herein, for the first time, the Electrodialysis (ED) technology based on electrochemical membrane separation process is successfully applied to separate and concentrate REEs from the diluted aqueous system. The overall performance of ED process in the recovery of Sc3+ ions from the wastewater was assessed by applied current, voltage, feed concentration, feed pH, co-ion competition and the overall energy consumption of the process. The REE recovery using the ED process was subjected to systematic investigations using both chronopotentiometric and chronoamperometric analyses. The results showed that ED process could be very promising in the recovery of Sc3+ ions (similar to 99.52% removal) from the diluted wastewater, consuming the energy of only 0.26 kWh/m(3) when operated at constant voltage mode (Sc3+ concentration of 20 ppm, pH 4, 1 h).
•The ED technique shows promising potential for REEs recovery and removal.•The effect of ED operating parameters on REE removal and recovery was studied.•The presence of competing ions influences REE recovery and removal efficiency.•The energy consumption of ED processes using CC and CV modes was compared. Rare earth elements (REEs) including Scandium (Sc) are critical raw materials which are greatly needed in the advancement of many modern technologies. Due to the problems associated with the primary extraction of mining ores, the procurement of Sc and REEs from the secondary resources are currently explored adopting the principle of sustainability and circular economy. Herein, for the first time, the Electrodialysis (ED) technology based on electrochemical membrane separation process is successfully applied to separate and concentrate REEs from the diluted aqueous system. The overall performance of ED process in the recovery of Sc3+ ions from the wastewater was assessed by applied current, voltage, feed concentration, feed pH, co-ion competition and the overall energy consumption of the process. The REE recovery using the ED process was subjected to systematic investigations using both chronopotentiometric and chronoamperometric analyses. The results showed that ED process could be very promising in the recovery of Sc3+ ions (~99.52% removal) from the diluted wastewater, consuming the energy of only 0.26 kWh/m3 when operated at constant voltage mode (Sc3+ concentration of 20 ppm, pH 4, 1 h).
ArticleNumber 117442
Author Repo, Eveliina
Sillanpää, Mika
Li, Changbai
Ramasamy, Deepika L.
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  givenname: Deepika L.
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Keywords Energy consumption
Membrane
Rare earth elements
Scandium
Electrodialysis
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Snippet •The ED technique shows promising potential for REEs recovery and removal.•The effect of ED operating parameters on REE removal and recovery was studied.•The...
Rare earth elements (REEs) including Scandium (Sc) are critical raw materials which are greatly needed in the advancement of many modern technologies. Due to...
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elsevier
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Publisher
StartPage 117442
SubjectTerms Electrodialysis
Energy consumption
Membrane
Rare earth elements
Scandium
Title Separation and concentration of rare earth elements from wastewater using electrodialysis technology
URI https://dx.doi.org/10.1016/j.seppur.2020.117442
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