Cellulose Regeneration and Chemical Recycling: Closing the “Cellulose Gap” Using Environmentally Benign Solvents

Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are employed for cellulose physical dissolution and shaping in different forms. This review focuses on the regeneration of dissolved cellulose as nanoparticle...

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Published inMacromolecular materials and engineering Vol. 305; no. 4
Main Authors El Seoud, Omar A., Kostag, Marc, Jedvert, Kerstin, Malek, Naved I.
Format Journal Article
LanguageEnglish
Published Weinheim John Wiley & Sons, Inc 01.04.2020
Subjects
Additives
Blending
Cellulose
cellulose blends
Cellulose fiber
Cellulose fibers
Cellulose films
cellulose nanoparticles
cellulose regeneration
chemical recycling
Depolymerization
Dissolution
Dissolving
Ethylene
Ionic liquids
Membranes
Mixing
Nanoparticles
Natural fibers
Non-wovens
nonwovens
Polyethylene terephthalate
Recycling
Regeneration
Solvents
Textile blends
Textile fibers
Wood
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Abstract Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are employed for cellulose physical dissolution and shaping in different forms. This review focuses on the regeneration of dissolved cellulose as nanoparticles, membranes, nonwoven materials, and fibers. The solvents employed in these applications include ILs and alkali solutions without and with additives. Cellulose fibers obtained via the carbonate and carbamate processes are included. Chemical recycling (CR) of polycotton (cellulose plus poly(ethylene terephthalate)) is addressed because depending on the recycling approach employed, this process is akin to regeneration. The strategies investigated in CR include preferential dissolution or depolymerization of one component of the blend, and separation of both components using ILs. It is hoped that this review focuses the attention on the potential applications of regenerated cellulose from its solutions and contributes to the important environmental issue of recycling of used materials. Ionic liquids and alkaline solutions dissolve cellulose physically. The resulting solutions are used to fabricate good‐quality fibers, nanoparticles, membranes, and nonwoven materials with interesting properties and relevant applications. Strategies for chemical recycling of polycotton (cellulose poly(ethylene terephthalate) blends) are discussed. Processes based on using these solvents have much less environmental impact than some of the existing ones.
AbstractList Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are employed for cellulose physical dissolution and shaping in different forms. This review focuses on the regeneration of dissolved cellulose as nanoparticles, membranes, nonwoven materials, and fibers. The solvents employed in these applications include ILs and alkali solutions without and with additives. Cellulose fibers obtained via the carbonate and carbamate processes are included. Chemical recycling (CR) of polycotton (cellulose plus poly(ethylene terephthalate)) is addressed because depending on the recycling approach employed, this process is akin to regeneration. The strategies investigated in CR include preferential dissolution or depolymerization of one component of the blend, and separation of both components using ILs. It is hoped that this review focuses the attention on the potential applications of regenerated cellulose from its solutions and contributes to the important environmental issue of recycling of used materials. Ionic liquids and alkaline solutions dissolve cellulose physically. The resulting solutions are used to fabricate good‐quality fibers, nanoparticles, membranes, and nonwoven materials with interesting properties and relevant applications. Strategies for chemical recycling of polycotton (cellulose poly(ethylene terephthalate) blends) are discussed. Processes based on using these solvents have much less environmental impact than some of the existing ones.
Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are employed for cellulose physical dissolution and shaping in different forms. This review focuses on the regeneration of dissolved cellulose as nanoparticles, membranes, nonwoven materials, and fibers. The solvents employed in these applications include ILs and alkali solutions without and with additives. Cellulose fibers obtained via the carbonate and carbamate processes are included. Chemical recycling (CR) of polycotton (cellulose plus poly(ethylene terephthalate)) is addressed because depending on the recycling approach employed, this process is akin to regeneration. The strategies investigated in CR include preferential dissolution or depolymerization of one component of the blend, and separation of both components using ILs. It is hoped that this review focuses the attention on the potential applications of regenerated cellulose from its solutions and contributes to the important environmental issue of recycling of used materials.
Abstract Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are employed for cellulose physical dissolution and shaping in different forms. This review focuses on the regeneration of dissolved cellulose as nanoparticles, membranes, nonwoven materials, and fibers. The solvents employed in these applications include ILs and alkali solutions without and with additives. Cellulose fibers obtained via the carbonate and carbamate processes are included. Chemical recycling (CR) of polycotton (cellulose plus poly(ethylene terephthalate)) is addressed because depending on the recycling approach employed, this process is akin to regeneration. The strategies investigated in CR include preferential dissolution or depolymerization of one component of the blend, and separation of both components using ILs. It is hoped that this review focuses the attention on the potential applications of regenerated cellulose from its solutions and contributes to the important environmental issue of recycling of used materials.
Author El Seoud, Omar A.
Kostag, Marc
Jedvert, Kerstin
Malek, Naved I.
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  organization: The University of São Paulo
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  givenname: Marc
  surname: Kostag
  fullname: Kostag, Marc
  organization: The University of São Paulo
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  surname: Jedvert
  fullname: Jedvert, Kerstin
  organization: Research Institutes of Sweden (RISE IVF)
– sequence: 4
  givenname: Naved I.
  surname: Malek
  fullname: Malek, Naved I.
  organization: Sardar Vallabhbhai National Institute of Technology
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Snippet Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are employed for...
Abstract Strategies to mitigate the expected “cellulose gap” include increased use of wood cellulose, fabric reuse, and recycling. Ionic liquids (ILs) are...
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SubjectTerms Additives
Blending
Cellulose
cellulose blends
Cellulose fiber
Cellulose fibers
Cellulose films
cellulose nanoparticles
cellulose regeneration
chemical recycling
Depolymerization
Dissolution
Dissolving
Ethylene
Ionic liquids
Membranes
Mixing
Nanoparticles
Natural fibers
Non-wovens
nonwovens
Polyethylene terephthalate
Recycling
Regeneration
Solvents
Textile blends
Textile fibers
Wood
Title Cellulose Regeneration and Chemical Recycling: Closing the “Cellulose Gap” Using Environmentally Benign Solvents
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fmame.201900832
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