The performance of UiO-66-NH2/graphene oxide (GO) composite membrane for removal of differently charged mixed dyes
The dye wastewater treatment by membrane separation technology has obtained extensive attention in recent years. Nevertheless, it was rare for research on the removal of differently charged mixed dyes. In this study, several UiO-66-NH2 composite membranes were prepared and optimization experiments w...
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| Published in | Chemosphere (Oxford) Vol. 237; p. 124517 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.12.2019
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| Subjects | |
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| Abstract | The dye wastewater treatment by membrane separation technology has obtained extensive attention in recent years. Nevertheless, it was rare for research on the removal of differently charged mixed dyes. In this study, several UiO-66-NH2 composite membranes were prepared and optimization experiments were conducted. The performance of composite membranes were evaluated by the removal of cationic (Methylene blue, MB), neutral (Rhodamine B, RB), and anionic (Congo red, CR) dyes. The optimization results demonstrated that the UiO-66-NH2/graphene oxide (UNG) composite membrane (PUF/PDA/UNG) which was loaded on polyurethane foam modified with polydopamine (PUF/PDA) had the best properties. In filtration experiments, the solution pH exhibited greater effect on the removal efficiency of MB and CR than RB. When NaCl, KCl, CaCl2 and Na2SO4 coexisted in the dye solution, the removal efficiency of MB by PUF/PDA/UNG membrane were 96.62%, 98.17%, 86.39% and 99.34% respectively. The presence of humic acid showed slight inhibitory effect on the removal of MB by PUF/PDA/UNG membrane (71.93%). The experimental results for mixed dyes filtration showed that PUF/PDA/UNG membrane could effectively remove MB, RB and CR in binary (i.e., MB/RB and RB/CR) and ternary (i.e., MB/RB/CR) systems through secondary filtration. And PUF/PDA/UNG membrane could remove MB and CR simultaneously through one-time filtration in MB/CR binary system. The removal mechanism was mainly attributed to the aggregation of mixed dyes, electrostatic interaction between dye molecules and the membrane surface, and hydrogen bonding. All results suggested that the as-prepared PUF/PDA/UNG membrane have great potential in practical treatment of dye wastewater.
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•Several UiO-66-NH2 composite membranes loaded on polyurethane foam were fabricated.•PUF/PDA/UNG membrane showed best properties in series of optimization experiments.•PUF/PDA/UNG composite membrane exhibited excellent removal efficiency towards MB.•PUF/PDA/UNG composite membrane could simultaneously remove RB, MB, and CR.•Electrostatic interaction and hydrogen bonding were contributed to the dyes removal. |
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| AbstractList | The dye wastewater treatment by membrane separation technology has obtained extensive attention in recent years. Nevertheless, it was rare for research on the removal of differently charged mixed dyes. In this study, several UiO-66-NH2 composite membranes were prepared and optimization experiments were conducted. The performance of composite membranes were evaluated by the removal of cationic (Methylene blue, MB), neutral (Rhodamine B, RB), and anionic (Congo red, CR) dyes. The optimization results demonstrated that the UiO-66-NH2/graphene oxide (UNG) composite membrane (PUF/PDA/UNG) which was loaded on polyurethane foam modified with polydopamine (PUF/PDA) had the best properties. In filtration experiments, the solution pH exhibited greater effect on the removal efficiency of MB and CR than RB. When NaCl, KCl, CaCl2 and Na2SO4 coexisted in the dye solution, the removal efficiency of MB by PUF/PDA/UNG membrane were 96.62%, 98.17%, 86.39% and 99.34% respectively. The presence of humic acid showed slight inhibitory effect on the removal of MB by PUF/PDA/UNG membrane (71.93%). The experimental results for mixed dyes filtration showed that PUF/PDA/UNG membrane could effectively remove MB, RB and CR in binary (i.e., MB/RB and RB/CR) and ternary (i.e., MB/RB/CR) systems through secondary filtration. And PUF/PDA/UNG membrane could remove MB and CR simultaneously through one-time filtration in MB/CR binary system. The removal mechanism was mainly attributed to the aggregation of mixed dyes, electrostatic interaction between dye molecules and the membrane surface, and hydrogen bonding. All results suggested that the as-prepared PUF/PDA/UNG membrane have great potential in practical treatment of dye wastewater. The dye wastewater treatment by membrane separation technology has obtained extensive attention in recent years. Nevertheless, it was rare for research on the removal of differently charged mixed dyes. In this study, several UiO-66-NH2 composite membranes were prepared and optimization experiments were conducted. The performance of composite membranes were evaluated by the removal of cationic (Methylene blue, MB), neutral (Rhodamine B, RB), and anionic (Congo red, CR) dyes. The optimization results demonstrated that the UiO-66-NH2/graphene oxide (UNG) composite membrane (PUF/PDA/UNG) which was loaded on polyurethane foam modified with polydopamine (PUF/PDA) had the best properties. In filtration experiments, the solution pH exhibited greater effect on the removal efficiency of MB and CR than RB. When NaCl, KCl, CaCl2 and Na2SO4 coexisted in the dye solution, the removal efficiency of MB by PUF/PDA/UNG membrane were 96.62%, 98.17%, 86.39% and 99.34% respectively. The presence of humic acid showed slight inhibitory effect on the removal of MB by PUF/PDA/UNG membrane (71.93%). The experimental results for mixed dyes filtration showed that PUF/PDA/UNG membrane could effectively remove MB, RB and CR in binary (i.e., MB/RB and RB/CR) and ternary (i.e., MB/RB/CR) systems through secondary filtration. And PUF/PDA/UNG membrane could remove MB and CR simultaneously through one-time filtration in MB/CR binary system. The removal mechanism was mainly attributed to the aggregation of mixed dyes, electrostatic interaction between dye molecules and the membrane surface, and hydrogen bonding. All results suggested that the as-prepared PUF/PDA/UNG membrane have great potential in practical treatment of dye wastewater. [Display omitted] •Several UiO-66-NH2 composite membranes loaded on polyurethane foam were fabricated.•PUF/PDA/UNG membrane showed best properties in series of optimization experiments.•PUF/PDA/UNG composite membrane exhibited excellent removal efficiency towards MB.•PUF/PDA/UNG composite membrane could simultaneously remove RB, MB, and CR.•Electrostatic interaction and hydrogen bonding were contributed to the dyes removal. The dye wastewater treatment by membrane separation technology has obtained extensive attention in recent years. Nevertheless, it was rare for research on the removal of differently charged mixed dyes. In this study, several UiO-66-NH2 composite membranes were prepared and optimization experiments were conducted. The performance of composite membranes were evaluated by the removal of cationic (Methylene blue, MB), neutral (Rhodamine B, RB), and anionic (Congo red, CR) dyes. The optimization results demonstrated that the UiO-66-NH2/graphene oxide (UNG) composite membrane (PUF/PDA/UNG) which was loaded on polyurethane foam modified with polydopamine (PUF/PDA) had the best properties. In filtration experiments, the solution pH exhibited greater effect on the removal efficiency of MB and CR than RB. When NaCl, KCl, CaCl2 and Na2SO4 coexisted in the dye solution, the removal efficiency of MB by PUF/PDA/UNG membrane were 96.62%, 98.17%, 86.39% and 99.34% respectively. The presence of humic acid showed slight inhibitory effect on the removal of MB by PUF/PDA/UNG membrane (71.93%). The experimental results for mixed dyes filtration showed that PUF/PDA/UNG membrane could effectively remove MB, RB and CR in binary (i.e., MB/RB and RB/CR) and ternary (i.e., MB/RB/CR) systems through secondary filtration. And PUF/PDA/UNG membrane could remove MB and CR simultaneously through one-time filtration in MB/CR binary system. The removal mechanism was mainly attributed to the aggregation of mixed dyes, electrostatic interaction between dye molecules and the membrane surface, and hydrogen bonding. All results suggested that the as-prepared PUF/PDA/UNG membrane have great potential in practical treatment of dye wastewater.The dye wastewater treatment by membrane separation technology has obtained extensive attention in recent years. Nevertheless, it was rare for research on the removal of differently charged mixed dyes. In this study, several UiO-66-NH2 composite membranes were prepared and optimization experiments were conducted. The performance of composite membranes were evaluated by the removal of cationic (Methylene blue, MB), neutral (Rhodamine B, RB), and anionic (Congo red, CR) dyes. The optimization results demonstrated that the UiO-66-NH2/graphene oxide (UNG) composite membrane (PUF/PDA/UNG) which was loaded on polyurethane foam modified with polydopamine (PUF/PDA) had the best properties. In filtration experiments, the solution pH exhibited greater effect on the removal efficiency of MB and CR than RB. When NaCl, KCl, CaCl2 and Na2SO4 coexisted in the dye solution, the removal efficiency of MB by PUF/PDA/UNG membrane were 96.62%, 98.17%, 86.39% and 99.34% respectively. The presence of humic acid showed slight inhibitory effect on the removal of MB by PUF/PDA/UNG membrane (71.93%). The experimental results for mixed dyes filtration showed that PUF/PDA/UNG membrane could effectively remove MB, RB and CR in binary (i.e., MB/RB and RB/CR) and ternary (i.e., MB/RB/CR) systems through secondary filtration. And PUF/PDA/UNG membrane could remove MB and CR simultaneously through one-time filtration in MB/CR binary system. The removal mechanism was mainly attributed to the aggregation of mixed dyes, electrostatic interaction between dye molecules and the membrane surface, and hydrogen bonding. All results suggested that the as-prepared PUF/PDA/UNG membrane have great potential in practical treatment of dye wastewater. |
| ArticleNumber | 124517 |
| Author | Zhang, Peng Cao, Wei-Cheng Song, Biao Li, Juan Huan, Shuang-Yan Fang, Si-Yuan Zeng, Guang-Ming Ye, Jun Gong, Ji-Lai |
| Author_xml | – sequence: 1 givenname: Juan surname: Li fullname: Li, Juan organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 2 givenname: Ji-Lai surname: Gong fullname: Gong, Ji-Lai email: jilaigong@gmail.com organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 3 givenname: Guang-Ming orcidid: 0000-0002-4230-7647 surname: Zeng fullname: Zeng, Guang-Ming organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 4 givenname: Peng surname: Zhang fullname: Zhang, Peng organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 5 givenname: Biao surname: Song fullname: Song, Biao organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 6 givenname: Wei-Cheng surname: Cao fullname: Cao, Wei-Cheng organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 7 givenname: Si-Yuan surname: Fang fullname: Fang, Si-Yuan organization: Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China – sequence: 8 givenname: Shuang-Yan surname: Huan fullname: Huan, Shuang-Yan organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, PR China – sequence: 9 givenname: Jun surname: Ye fullname: Ye, Jun organization: Hunan Qing Zhi Yuan Environmental Protection Technology Co., Ltd, Changsha, 410004, PR China |
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| Keywords | Polyurethane membrane Metal-organic framework Graphene oxide Wastewater treatment Organic dyes |
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| SubjectTerms | asymmetric membranes calcium chloride electrostatic interactions filtration foams Graphene oxide humic acids hydrogen bonding Metal-organic framework methylene blue Organic dyes Polyurethane membrane polyurethanes potassium chloride rhodamines sodium chloride sodium sulfate wastewater Wastewater treatment |
| Title | The performance of UiO-66-NH2/graphene oxide (GO) composite membrane for removal of differently charged mixed dyes |
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