Reduced graphene oxide supported V2O5-WO3-TiO2 catalysts for selective catalytic reduction of NOx
We present a reduced-graphene-oxide (rGO)-supported V2O 5 -WO 3 -TiO 2 (VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support provides well-dispersed functional sites for the nucleation of nanoparticles, allowing the formation of VWTi catalysts with high specific su...
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| Published in | The Korean journal of chemical engineering Vol. 35; no. 10; pp. 1988 - 1993 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Springer US
01.10.2018
Springer Nature B.V 한국화학공학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0256-1115 1975-7220 |
| DOI | 10.1007/s11814-018-0109-6 |
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| Abstract | We present a reduced-graphene-oxide (rGO)-supported V2O
5
-WO
3
-TiO
2
(VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support provides well-dispersed functional sites for the nucleation of nanoparticles, allowing the formation of VWTi catalysts with high specific surface areas. The dispersion of the nanoparticles, as observed by transmission electron microscopy (TEM) and energy dispersive spectroscopy (EDS), confirmed the uniform dispersion of the particles on the rGO surface. Detailed Fourier-transform infrared (FT-IR) and NH
3
temperature-programmed desorption (NH
3
-TPD) analyses indicated that the high density of acidic sites provided by the rGO is key to the observed enhancement of NOx removal efficiency, and the rGO-supported catalysts exhibit improved NOx removal efficiencies with smaller amounts of V
2
O
5
and WO
3
compared with the commercially available V
2
O
5
-WO
3
-TiO
2
catalysts. |
|---|---|
| AbstractList | We present a reduced-graphene-oxide (rGO)-supported V2O5-WO3-TiO2 (VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support provides well-dispersed functional sites for the nucleation of nanoparticles, allowing the formation of VWTi catalysts with high specific surface areas. The dispersion of the nanoparticles, as observed by transmission electron microscopy (TEM) and energy dispersive spectroscopy (EDS), confirmed the uniform dispersion of the particles on the rGO surface. Detailed Fourier-transform infrared (FT-IR) and NH3 temperature-programmed desorption (NH3-TPD) analyses indicated that the high density of acidic sites provided by the rGO is key to the observed enhancement of NOx removal efficiency, and the rGO-supported catalysts exhibit improved NOx removal efficiencies with smaller amounts of V2O5 and WO3 compared with the commercially available V2O5-WO3-TiO2 catalysts. We present a reduced-graphene-oxide (rGO)-supported V2O5-WO3-TiO2 (VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support provides well-dispersed functional sites for the nucleation of nanoparticles, allowing the formation of VWTi catalysts with high specific surface areas. The dispersion of the nanoparticles, as observed by transmission electron microscopy (TEM) and energy dispersive spectroscopy (EDS), confirmed the uniform dispersion of the particles on the rGO surface. Detailed Fourier-transform infrared (FT-IR) and NH3 temperature-programmed desorption (NH3-TPD) analyses indicated that the high density of acidic sites provided by the rGO is key to the observed enhancement of NOx removal efficiency, and the rGO-supported catalysts exhibit improved NOx removal efficiencies with smaller amounts of V2O5 and WO3 compared with the commercially available V2O5-WO3-TiO2 catalysts. KCI Citation Count: 13 We present a reduced-graphene-oxide (rGO)-supported V2O 5 -WO 3 -TiO 2 (VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support provides well-dispersed functional sites for the nucleation of nanoparticles, allowing the formation of VWTi catalysts with high specific surface areas. The dispersion of the nanoparticles, as observed by transmission electron microscopy (TEM) and energy dispersive spectroscopy (EDS), confirmed the uniform dispersion of the particles on the rGO surface. Detailed Fourier-transform infrared (FT-IR) and NH 3 temperature-programmed desorption (NH 3 -TPD) analyses indicated that the high density of acidic sites provided by the rGO is key to the observed enhancement of NOx removal efficiency, and the rGO-supported catalysts exhibit improved NOx removal efficiencies with smaller amounts of V 2 O 5 and WO 3 compared with the commercially available V 2 O 5 -WO 3 -TiO 2 catalysts. |
| Author | Jeong, Bora Kim, Hong-Dae Ye, Bora Lee, Duck Hyun Park, Sam-sik Chun, Hye-yeon Lee, Heesoo Lee, Minwoo |
| Author_xml | – sequence: 1 givenname: Minwoo surname: Lee fullname: Lee, Minwoo organization: Green Materials & Processes Group, Ulsan Regional Division, Korea Institute of Industrial Technology, Department of Materials Science and Engineering, Pusan National University – sequence: 2 givenname: Bora surname: Ye fullname: Ye, Bora organization: Green Materials & Processes Group, Ulsan Regional Division, Korea Institute of Industrial Technology – sequence: 3 givenname: Bora surname: Jeong fullname: Jeong, Bora organization: Green Materials & Processes Group, Ulsan Regional Division, Korea Institute of Industrial Technology – sequence: 4 givenname: Hye-yeon surname: Chun fullname: Chun, Hye-yeon organization: Green Materials & Processes Group, Ulsan Regional Division, Korea Institute of Industrial Technology – sequence: 5 givenname: Duck Hyun surname: Lee fullname: Lee, Duck Hyun organization: Green Materials & Processes Group, Ulsan Regional Division, Korea Institute of Industrial Technology – sequence: 6 givenname: Sam-sik surname: Park fullname: Park, Sam-sik organization: R&D Center, NANO. Co., Ltd – sequence: 7 givenname: Heesoo surname: Lee fullname: Lee, Heesoo organization: Department of Materials Science and Engineering, Pusan National University – sequence: 8 givenname: Hong-Dae surname: Kim fullname: Kim, Hong-Dae email: hdkim@kitech.re.kr organization: Green Materials & Processes Group, Ulsan Regional Division, Korea Institute of Industrial Technology |
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| CitedBy_id | crossref_primary_10_1007_s10563_019_09277_1 crossref_primary_10_1177_1847980419886673 crossref_primary_10_1016_j_apsusc_2021_149934 crossref_primary_10_3390_nano11102677 crossref_primary_10_1039_D0RA01665A crossref_primary_10_1186_s40580_022_00341_7 crossref_primary_10_1007_s10563_020_09293_6 crossref_primary_10_1016_j_cattod_2018_12_007 crossref_primary_10_1002_er_6623 crossref_primary_10_1016_j_jpcs_2022_110782 crossref_primary_10_1007_s11814_018_0227_9 crossref_primary_10_1016_j_jcis_2020_05_066 crossref_primary_10_1021_acs_iecr_8b03973 |
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| Keywords | NOx Removal Efficiency Wet Impregnation Selective Catalytic Reduction High Dispersion Reduced Graphene Oxide |
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| Snippet | We present a reduced-graphene-oxide (rGO)-supported V2O
5
-WO
3
-TiO
2
(VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support... We present a reduced-graphene-oxide (rGO)-supported V2O5-WO3-TiO2 (VWTi) catalysts for the efficient selective catalytic reduction of NOx. The rGO support... |
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| StartPage | 1988 |
| SubjectTerms | Ammonia Biotechnology Catalysis Catalysts Chemistry Chemistry and Materials Science Energy transmission Fourier transforms Graphene Industrial Chemistry/Chemical Engineering Infrared analysis Materials Science Nanoparticles Nitrates Nitrogen oxides Reaction Engineering Selective catalytic reduction Titanium dioxide Transmission electron microscopy Tungsten oxides Vanadium pentoxide 화학공학 |
| Title | Reduced graphene oxide supported V2O5-WO3-TiO2 catalysts for selective catalytic reduction of NOx |
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