Characterization of argon dielectric barrier discharges applied to ethyl lactate plasma polymerization

The influence of the input voltage frequency (35 and 150 kHz), interelectrode gap (1 and 2 mm) and precursor concentration (250, 350, and 450 ppm) on the electron temperature (Te), number density of metastable Ar atoms (n(Arm)), and discharge current density (proportional to the electron density ne)...

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Published inJournal of physics. D, Applied physics Vol. 50; no. 47; pp. 475205 - 475215
Main Authors Laurent, Morgane, Desjardins, Edouard, Meichelboeck, Maximilian, Naudé, Nicolas, Stafford, Luc, Gherardi, Nicolas, Laroche, Gaétan
Format Journal Article
LanguageEnglish
Published IOP Publishing 29.11.2017
Subjects
argon metastable
current density
dielectric barrier discharge
electron temperature
Engineering Sciences
ethyl lactate
optical emission spectroscopy
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Abstract The influence of the input voltage frequency (35 and 150 kHz), interelectrode gap (1 and 2 mm) and precursor concentration (250, 350, and 450 ppm) on the electron temperature (Te), number density of metastable Ar atoms (n(Arm)), and discharge current density (proportional to the electron density ne) is studied in an argon-ethyl lactate dielectric barrier discharge (DBD). An argon-ammonia Penning mixture is also considered as reference. These results are correlated to the chemistry (XPS, IR) and topography (AFM) of the ethyl-lactate-based plasma polymer coatings. Low Te values from 0.3 to 0.5 eV were obtained for all discharges. This observation, in addition to resemblances with the Ar-NH3 mixture, suggested that the ionization kinetics of ethyl lactate-based discharges is driven by Penning reactions. Among the investigated parameters, the dissipated power obtained through changes of the excitation frequency had the largest impact on both the coatings properties and the discharge behavior.
AbstractList The influence of the input voltage frequency (35 and 150 kHz), interelectrode gap (1 and 2 mm) and precursor concentration (250, 350, and 450 ppm) on the electron temperature (Te), number density of metastable Ar atoms (n(Arm)), and discharge current density (proportional to the electron density ne) is studied in an argon-ethyl lactate dielectric barrier discharge (DBD). An argon-ammonia Penning mixture is also considered as reference. These results are correlated to the chemistry (XPS, IR) and topography (AFM) of the ethyl-lactate-based plasma polymer coatings. Low Te values from 0.3 to 0.5 eV were obtained for all discharges. This observation, in addition to resemblances with the Ar-NH3 mixture, suggested that the ionization kinetics of ethyl lactate-based discharges is driven by Penning reactions. Among the investigated parameters, the dissipated power obtained through changes of the excitation frequency had the largest impact on both the coatings properties and the discharge behavior.
Author Desjardins, Edouard
Gherardi, Nicolas
Meichelboeck, Maximilian
Laurent, Morgane
Naudé, Nicolas
Stafford, Luc
Laroche, Gaétan
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Snippet The influence of the input voltage frequency (35 and 150 kHz), interelectrode gap (1 and 2 mm) and precursor concentration (250, 350, and 450 ppm) on the...
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SubjectTerms argon metastable
current density
dielectric barrier discharge
electron temperature
Engineering Sciences
ethyl lactate
optical emission spectroscopy
Title Characterization of argon dielectric barrier discharges applied to ethyl lactate plasma polymerization
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