Ferroelectricity‐Driven Self‐Powered Ultraviolet Photodetection with Strong Polarization Sensitivity in a Two‐Dimensional Halide Hybrid Perovskite
Polarization‐sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide‐band photodetectors. However, it still remains elusive to achieve the self‐powered devices, which can be operated in the absence of externa...
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| Published in | Angewandte Chemie International Edition Vol. 59; no. 43; pp. 18933 - 18937 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
19.10.2020
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Polarization‐sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide‐band photodetectors. However, it still remains elusive to achieve the self‐powered devices, which can be operated in the absence of external bias. Herein, for the first time, ferroelectricity‐driven self‐powered photodetection towards polarized UV light was successfully demonstrated in a 2D wide‐band gap hybrid ferroelectric (BPA)2PbBr4 (BPA=3‐bromopropylammonium) (1). We found that the prominent spontaneous polarization in 1 results in a bulk photovoltaic effect (BPVE) of 0.85 V, that independently drives photoexcited carriers separation and transport and thus supports self‐powered ability. This self‐powered detector shows strong polarization sensitivity to linearly polarized UV illumination with a polarization ratio up to 6.8, which is superior to that of previously reported UV‐polarized photodetectors (ZnO, GaN, and GeS2).
A ferroelectricity‐driven self‐powered ultraviolet photodetector employing a 2D hybrid perovskite ferroelectric (BPA)2PbBr4 (BPA=3‐bromopropylammonium) is presented. It shows strong polarization sensitivity, with a large polarization ratio of up to 6.8. |
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| AbstractList | Polarization-sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide-band photodetectors. However, it still remains elusive to achieve the self-powered devices, which can be operated in the absence of external bias. Herein, for the first time, ferroelectricity-driven self-powered photodetection towards polarized UV light was successfully demonstrated in a 2D wide-band gap hybrid ferroelectric (BPA)2 PbBr4 (BPA=3-bromopropylammonium) (1). We found that the prominent spontaneous polarization in 1 results in a bulk photovoltaic effect (BPVE) of 0.85 V, that independently drives photoexcited carriers separation and transport and thus supports self-powered ability. This self-powered detector shows strong polarization sensitivity to linearly polarized UV illumination with a polarization ratio up to 6.8, which is superior to that of previously reported UV-polarized photodetectors (ZnO, GaN, and GeS2 ).Polarization-sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide-band photodetectors. However, it still remains elusive to achieve the self-powered devices, which can be operated in the absence of external bias. Herein, for the first time, ferroelectricity-driven self-powered photodetection towards polarized UV light was successfully demonstrated in a 2D wide-band gap hybrid ferroelectric (BPA)2 PbBr4 (BPA=3-bromopropylammonium) (1). We found that the prominent spontaneous polarization in 1 results in a bulk photovoltaic effect (BPVE) of 0.85 V, that independently drives photoexcited carriers separation and transport and thus supports self-powered ability. This self-powered detector shows strong polarization sensitivity to linearly polarized UV illumination with a polarization ratio up to 6.8, which is superior to that of previously reported UV-polarized photodetectors (ZnO, GaN, and GeS2 ). Polarization‐sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide‐band photodetectors. However, it still remains elusive to achieve the self‐powered devices, which can be operated in the absence of external bias. Herein, for the first time, ferroelectricity‐driven self‐powered photodetection towards polarized UV light was successfully demonstrated in a 2D wide‐band gap hybrid ferroelectric (BPA) 2 PbBr 4 (BPA=3‐bromopropylammonium) ( 1 ). We found that the prominent spontaneous polarization in 1 results in a bulk photovoltaic effect (BPVE) of 0.85 V, that independently drives photoexcited carriers separation and transport and thus supports self‐powered ability. This self‐powered detector shows strong polarization sensitivity to linearly polarized UV illumination with a polarization ratio up to 6.8, which is superior to that of previously reported UV‐polarized photodetectors (ZnO, GaN, and GeS 2 ). Polarization‐sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide‐band photodetectors. However, it still remains elusive to achieve the self‐powered devices, which can be operated in the absence of external bias. Herein, for the first time, ferroelectricity‐driven self‐powered photodetection towards polarized UV light was successfully demonstrated in a 2D wide‐band gap hybrid ferroelectric (BPA)2PbBr4 (BPA=3‐bromopropylammonium) (1). We found that the prominent spontaneous polarization in 1 results in a bulk photovoltaic effect (BPVE) of 0.85 V, that independently drives photoexcited carriers separation and transport and thus supports self‐powered ability. This self‐powered detector shows strong polarization sensitivity to linearly polarized UV illumination with a polarization ratio up to 6.8, which is superior to that of previously reported UV‐polarized photodetectors (ZnO, GaN, and GeS2). A ferroelectricity‐driven self‐powered ultraviolet photodetector employing a 2D hybrid perovskite ferroelectric (BPA)2PbBr4 (BPA=3‐bromopropylammonium) is presented. It shows strong polarization sensitivity, with a large polarization ratio of up to 6.8. Polarization‐sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various wide‐band photodetectors. However, it still remains elusive to achieve the self‐powered devices, which can be operated in the absence of external bias. Herein, for the first time, ferroelectricity‐driven self‐powered photodetection towards polarized UV light was successfully demonstrated in a 2D wide‐band gap hybrid ferroelectric (BPA)2PbBr4 (BPA=3‐bromopropylammonium) (1). We found that the prominent spontaneous polarization in 1 results in a bulk photovoltaic effect (BPVE) of 0.85 V, that independently drives photoexcited carriers separation and transport and thus supports self‐powered ability. This self‐powered detector shows strong polarization sensitivity to linearly polarized UV illumination with a polarization ratio up to 6.8, which is superior to that of previously reported UV‐polarized photodetectors (ZnO, GaN, and GeS2). |
| Author | Li, Lina Dey, Dhananjay Liu, Xitao Luo, Junhua Peng, Yu Ji, Chengmin |
| Author_xml | – sequence: 1 givenname: Chengmin orcidid: 0000-0002-5355-9006 surname: Ji fullname: Ji, Chengmin organization: Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China – sequence: 2 givenname: Dhananjay surname: Dey fullname: Dey, Dhananjay organization: Chinese Academy of Sciences – sequence: 3 givenname: Yu surname: Peng fullname: Peng, Yu organization: Chinese Academy of Sciences – sequence: 4 givenname: Xitao surname: Liu fullname: Liu, Xitao organization: University of Chinese Academy of Sciences – sequence: 5 givenname: Lina surname: Li fullname: Li, Lina organization: University of Chinese Academy of Sciences – sequence: 6 givenname: Junhua orcidid: 0000-0002-3179-7652 surname: Luo fullname: Luo, Junhua email: jhluo@fjirsm.ac.cn organization: University of Chinese Academy of Sciences |
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| Snippet | Polarization‐sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various... Polarization-sensitive ultraviolet (UV) photodetection is highly indispensable in military and civilian applications and has been demonstrated with various... |
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| SubjectTerms | bulk photovoltaic effect Ferroelectricity ferroelectrics hybrid perovskites Linear polarization Military applications Perovskites Photometers Photovoltaic effect Photovoltaics Polarization polarization sensitivity self-powered photodetection Sensitivity Ultraviolet radiation Zinc oxide |
| Title | Ferroelectricity‐Driven Self‐Powered Ultraviolet Photodetection with Strong Polarization Sensitivity in a Two‐Dimensional Halide Hybrid Perovskite |
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