Phytosterol‐based oleogels self‐assembled with monoglyceride for controlled volatile release
BACKGROUND Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans‐fat and delivery of functional ingredients. Phytosterols, comprising plant‐derived natural steroid compounds, are preferred for oleogel production...
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| Published in | Journal of the science of food and agriculture Vol. 98; no. 2; pp. 582 - 589 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Chichester, UK
John Wiley & Sons, Ltd
01.01.2018
John Wiley and Sons, Limited |
| Subjects | |
| Online Access | Get full text |
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| Abstract | BACKGROUND
Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans‐fat and delivery of functional ingredients. Phytosterols, comprising plant‐derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol‐based oleogels self‐assembled with monoglyceride were studied with respect to tuning volatile release.
RESULTS
Microscopy images of the bicomponent oleogels of β‐sitosterol and monoglyceride showed the formation of a new three‐dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X‐ray scattering results suggests the self‐assembly of β‐sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v0), maximum headspace concentrations (Cmax) and partition coefficients (ka/o) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol‐based oleogels under both dynamic and static conditions. In addition, the solid‐like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding.
CONCLUSION
The self‐assembly of phytosterol‐based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry |
|---|---|
| AbstractList | BACKGROUND
Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans‐fat and delivery of functional ingredients. Phytosterols, comprising plant‐derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol‐based oleogels self‐assembled with monoglyceride were studied with respect to tuning volatile release.
RESULTS
Microscopy images of the bicomponent oleogels of β‐sitosterol and monoglyceride showed the formation of a new three‐dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X‐ray scattering results suggests the self‐assembly of β‐sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v0), maximum headspace concentrations (Cmax) and partition coefficients (ka/o) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol‐based oleogels under both dynamic and static conditions. In addition, the solid‐like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding.
CONCLUSION
The self‐assembly of phytosterol‐based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry BACKGROUND Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans-fat and delivery of functional ingredients. Phytosterols, comprising plant-derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol-based oleogels self-assembled with monoglyceride were studied with respect to tuning volatile release. RESULTS Microscopy images of the bicomponent oleogels of [beta]-sitosterol and monoglyceride showed the formation of a new three-dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X-ray scattering results suggests the self-assembly of [beta]-sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v0), maximum headspace concentrations (Cmax) and partition coefficients (ka/o) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol-based oleogels under both dynamic and static conditions. In addition, the solid-like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding. CONCLUSION The self-assembly of phytosterol-based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry BACKGROUND: Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans‐fat and delivery of functional ingredients. Phytosterols, comprising plant‐derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol‐based oleogels self‐assembled with monoglyceride were studied with respect to tuning volatile release. RESULTS: Microscopy images of the bicomponent oleogels of β‐sitosterol and monoglyceride showed the formation of a new three‐dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X‐ray scattering results suggests the self‐assembly of β‐sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v₀), maximum headspace concentrations (Cₘₐₓ) and partition coefficients (kₐ/ₒ) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol‐based oleogels under both dynamic and static conditions. In addition, the solid‐like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding. CONCLUSION: The self‐assembly of phytosterol‐based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans-fat and delivery of functional ingredients. Phytosterols, comprising plant-derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol-based oleogels self-assembled with monoglyceride were studied with respect to tuning volatile release. Microscopy images of the bicomponent oleogels of β-sitosterol and monoglyceride showed the formation of a new three-dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X-ray scattering results suggests the self-assembly of β-sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v ), maximum headspace concentrations (C ) and partition coefficients (k ) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol-based oleogels under both dynamic and static conditions. In addition, the solid-like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding. The self-assembly of phytosterol-based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry. Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans-fat and delivery of functional ingredients. Phytosterols, comprising plant-derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol-based oleogels self-assembled with monoglyceride were studied with respect to tuning volatile release.BACKGROUNDOleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans-fat and delivery of functional ingredients. Phytosterols, comprising plant-derived natural steroid compounds, are preferred for oleogel production because they are both natural and healthy. In the present study, phytosterol-based oleogels self-assembled with monoglyceride were studied with respect to tuning volatile release.Microscopy images of the bicomponent oleogels of β-sitosterol and monoglyceride showed the formation of a new three-dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X-ray scattering results suggests the self-assembly of β-sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v0 ), maximum headspace concentrations (Cmax ) and partition coefficients (ka/o ) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol-based oleogels under both dynamic and static conditions. In addition, the solid-like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding.RESULTSMicroscopy images of the bicomponent oleogels of β-sitosterol and monoglyceride showed the formation of a new three-dimensional network of entangled crystals and a controllable microstructure. Our analysis from differential scanning calorimetry and small angle X-ray scattering results suggests the self-assembly of β-sitosterol and monoglyceride via intermolecular hydrogen bonds into spherulitic microstructures. The results showed that the release rate (v0 ), maximum headspace concentrations (Cmax ) and partition coefficients (ka/o ) for oleogels showed a significantly controlled release and were tunable via the microstructure of phytosterol-based oleogels under both dynamic and static conditions. In addition, the solid-like oleogels had interesting thixotropic and thermoresponsive behaviors, probably as a result of intermolecular hydrogen bonding.The self-assembly of phytosterol-based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry.CONCLUSIONThe self-assembly of phytosterol-based oleogels with monoglyceride was attributed to intermolecular hydrogen and is demonstrated to be a promising tunable and functional strategy for delivering flavor compounds. © 2017 Society of Chemical Industry. |
| Author | Yang, Xiao‐Quan Chen, Xiao‐Wei Yang, Dan‐Xia |
| Author_xml | – sequence: 1 givenname: Dan‐Xia surname: Yang fullname: Yang, Dan‐Xia organization: Department of Food Science and Engineering, South China University of Technology – sequence: 2 givenname: Xiao‐Wei surname: Chen fullname: Chen, Xiao‐Wei organization: Department of Food Science and Engineering, South China University of Technology – sequence: 3 givenname: Xiao‐Quan orcidid: 0000-0002-0492-8987 surname: Yang fullname: Yang, Xiao‐Quan email: fexqyang@scut.edu.cn, fexqyang@163.com organization: South China University of Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28653331$$D View this record in MEDLINE/PubMed |
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Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans‐fat... Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans-fat and delivery... BACKGROUND Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans-fat... BACKGROUND: Oleogels have recently emerged as a subject of growing interest among industrial and academic researchers as an alternative to saturated/trans‐fat... |
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| SubjectTerms | Beta rays beta-sitosterol Calorimetry Calorimetry, Differential Scanning Chemical compounds Controlled release Crystals Differential scanning calorimetry Flavor compounds functional foods Glycerides - chemistry Headspace headspace analysis Hydrogen Hydrogen Bonding Hydrogen bonds microscopy Microstructure monoacylglycerols monoglyceride Monoglycerides - chemistry oleogels Organic Chemicals - chemistry partition coefficients Phytosterols Phytosterols - chemistry Plants researchers Self-assembly Small angle X ray scattering Stability volatile release Volatilization X-radiation X-ray scattering |
| Title | Phytosterol‐based oleogels self‐assembled with monoglyceride for controlled volatile release |
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