A predictive theoretical model for stretch-induced instabilities in liquid crystal elastomers
Following the experimental lead, we construct a general mathematical model which, depending on whether the uniaxial scalar order parameter is constant or not, can predict either the classical shear striping instability or the molecular auxetic response and mechanical Fréedericksz transition observed...
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Published in | Liquid crystals Vol. 50; no. 7-10; pp. 1426 - 1438 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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Taylor & Francis
09.08.2023
Taylor & Francis Ltd |
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Abstract | Following the experimental lead, we construct a general mathematical model which, depending on whether the uniaxial scalar order parameter is constant or not, can predict either the classical shear striping instability or the molecular auxetic response and mechanical Fréedericksz transition observed in different liquid crystal elastomers. Our theoretical model can shed some light on the role of nematic order in these stretch-induced mechanical instabilities not observed in conventional rubber-like solids. |
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AbstractList | Following the experimental lead, we construct a general mathematical model which, depending on whether the uniaxial scalar order parameter is constant or not, can predict either the classical shear striping instability or the molecular auxetic response and mechanical Fréedericksz transition observed in different liquid crystal elastomers. Our theoretical model can shed some light on the role of nematic order in these stretch-induced mechanical instabilities not observed in conventional rubber-like solids. |
Author | Mihai, L. Angela Gleeson, Helen F. Goriely, Alain Mistry, Devesh Raistrick, Thomas |
Author_xml | – sequence: 1 givenname: L. Angela surname: Mihai fullname: Mihai, L. Angela organization: School of Mathematics, Cardiff University, Cardiff, UK – sequence: 2 givenname: Thomas surname: Raistrick fullname: Raistrick, Thomas organization: School of Physics and Astronomy, University of Leeds, Leeds, UK – sequence: 3 givenname: Helen F. surname: Gleeson fullname: Gleeson, Helen F. organization: School of Physics and Astronomy, University of Leeds, Leeds, UK – sequence: 4 givenname: Devesh surname: Mistry fullname: Mistry, Devesh organization: School of Physics and Astronomy, University of Leeds, Leeds, UK – sequence: 5 givenname: Alain surname: Goriely fullname: Goriely, Alain organization: Mathematical Institute, University of Oxford, Oxford, UK |
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Cites_doi | 10.1016/S1381-5148(99)00032-2 10.1063/1.1979479 10.1140/epje/i2009-10467-9 10.3390/molecules26237313 10.1021/ma071104y 10.1038/s41467-018-07587-y 10.1080/1358314X.2022.2048974 10.1007/978-3-031-06692-4 10.1002/(SICI)1521-3935(19980401)199:4<677::AID-MACP677>3.0.CO;2-E 10.1016/S0022-5096(01)00120-X 10.1103/PhysRevLett.71.2947 10.1557/s43577-021-00115-2 10.1002/marc.1995.030160908 10.1039/C7SM02107K 10.1021/acs.macromol.9b02456 10.1103/PhysRevE.82.011703 10.1063/1.2234824 10.1103/PhysRevResearch.3.023191 10.1103/PhysRevLett.103.077801 10.1093/oso/9780198520245.001.0001 10.1016/S0167-2789(99)00153-0 10.1088/1361-6544/ac09c1 10.1098/rsta.2021.0326 10.1002/polb.24879 10.1177/1081286520914958 10.1098/rspa.1972.0026 10.1080/026782999203869 10.1007/s101890170060 10.1021/ma400771z 10.1016/j.jmps.2003.12.005 |
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References | e_1_3_3_30_1 Ogden RW (e_1_3_3_28_1) 1997 e_1_3_3_18_1 e_1_3_3_17_1 e_1_3_3_19_1 Finkelmann H (e_1_3_3_8_1) 1997; 7 e_1_3_3_14_1 e_1_3_3_13_1 e_1_3_3_35_1 e_1_3_3_15_1 e_1_3_3_10_1 e_1_3_3_33_1 Verwey GC (e_1_3_3_34_1) 1996; 6 e_1_3_3_12_1 e_1_3_3_31_1 e_1_3_3_11_1 e_1_3_3_32_1 e_1_3_3_7_1 e_1_3_3_6_1 e_1_3_3_9_1 e_1_3_3_29_1 e_1_3_3_25_1 e_1_3_3_24_1 e_1_3_3_27_1 Warner M (e_1_3_3_16_1) 2007 e_1_3_3_26_1 e_1_3_3_3_1 e_1_3_3_21_1 e_1_3_3_2_1 e_1_3_3_20_1 e_1_3_3_5_1 e_1_3_3_23_1 e_1_3_3_4_1 e_1_3_3_22_1 |
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SubjectTerms | auxeticity Elastomers Freedericksz transitions large strain deformation Liquid crystal elastomer Liquid crystals mathematical modelling Mathematical models non-linear elasticity Order parameters shear striping |
Title | A predictive theoretical model for stretch-induced instabilities in liquid crystal elastomers |
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