Efficiency assessment of Cu and Al electrodes in the removal of anthraquinone based disperse dye aqueous solution in electrocoagulation-an analytical approach

Anthraquinone dyes are tough to degrade compared to azo dyes, due to the resonance in the anthracene structure that leads to more difficulty in the removal and challenges the possibility of an effective decolouration/degradation process. The purpose of this study was to examine the effect of copper...

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Published inInternational journal of environmental analytical chemistry Vol. 103; no. 17; pp. 5619 - 5638
Main Authors Kalivel, Parameswari, Choondal Jisson, Jithin, Kavitha, Subbiah, Padmanabhan, Dhanasekaran, Bhagavathsingh, Jebasingh, Palanichamy, Jegathambal, Stephen, Asath Murphy Maria, David, Jovitha Jane
Format Journal Article
LanguageEnglish
Published Abingdon Taylor & Francis 20.12.2023
Taylor & Francis LLC
Subjects
Aluminium
Aluminum
Analytical methods
Anthracene
Anthraquinone
Anthraquinone dyes
Aquatic crustaceans
Aqueous solutions
Artemia
Artemia salina
Azo dyes
Chromatography
Coagulation
Color removal
Copper
Current density
Decoloring
Decolorization
Dispersion
Dyes
EC method
ECE
ecotoxicity
Efficiency
Electrocoagulation
Electrodes
High performance liquid chromatography
HPLC
Hydroxides
Liquid chromatography
Photoelectron spectroscopy
Photoelectrons
Phytotoxicity
Red BFL dye
Removal
Sludge
Spectroscopy
Spectrum analysis
Toxicity
Vigna radiata
X ray photoelectron spectroscopy
X rays
XPS
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Abstract Anthraquinone dyes are tough to degrade compared to azo dyes, due to the resonance in the anthracene structure that leads to more difficulty in the removal and challenges the possibility of an effective decolouration/degradation process. The purpose of this study was to examine the effect of copper and aluminium electrodes in electrocoagulation process for the elimination of an anthraquinone based aqueous solution of Red BFL dye. The efficiency of the electrodes in the dye removal was studied using X-Ray Photoelectron Spectroscopy of the collected sludge, in terms of the respective M(OH) n formation which contributes in coagulation of the dispersed dye molecules and the results indicated that Al formed four types of hydroxides and Cu only one type. The maximum removal of the dye solution obtained with Al was 99.17% at the optimum conditions: pH 8, contact time 15 min, current density 40 A m −2 , and 91.88% with Cu: pH 9, contact time 25 min and current density 60 A m −2 . Phytotoxicity and ecotoxicity studies with Vigna radiata and Artemia salina was done to investigate the toxicity of intermediate products in the treated Red BFL dye solution, results showed that the Al used Red BFL dye solution was less toxic in comparison to copper. Abbreviation: EC: Electrocoagulation; AQ: Anthraquinone; CD: Current density; CT: Contact time; ECE%: Efficiency in Colour Elimination percentage; HPLC: High-performance liquid chromatography; XPS: X-ray photoelectron spectroscopy; V. radiata: Vigna radiata; A. salina: Artemia salina
AbstractList Anthraquinone dyes are tough to degrade compared to azo dyes, due to the resonance in the anthracene structure that leads to more difficulty in the removal and challenges the possibility of an effective decolouration/degradation process. The purpose of this study was to examine the effect of copper and aluminium electrodes in electrocoagulation process for the elimination of an anthraquinone based aqueous solution of Red BFL dye. The efficiency of the electrodes in the dye removal was studied using X-Ray Photoelectron Spectroscopy of the collected sludge, in terms of the respective M(OH) n formation which contributes in coagulation of the dispersed dye molecules and the results indicated that Al formed four types of hydroxides and Cu only one type. The maximum removal of the dye solution obtained with Al was 99.17% at the optimum conditions: pH 8, contact time 15 min, current density 40 A m −2 , and 91.88% with Cu: pH 9, contact time 25 min and current density 60 A m −2 . Phytotoxicity and ecotoxicity studies with Vigna radiata and Artemia salina was done to investigate the toxicity of intermediate products in the treated Red BFL dye solution, results showed that the Al used Red BFL dye solution was less toxic in comparison to copper. Abbreviation: EC: Electrocoagulation; AQ: Anthraquinone; CD: Current density; CT: Contact time; ECE%: Efficiency in Colour Elimination percentage; HPLC: High-performance liquid chromatography; XPS: X-ray photoelectron spectroscopy; V. radiata: Vigna radiata; A. salina: Artemia salina
Anthraquinone dyes are tough to degrade compared to azo dyes, due to the resonance in the anthracene structure that leads to more difficulty in the removal and challenges the possibility of an effective decolouration/degradation process. The purpose of this study was to examine the effect of copper and aluminium electrodes in electrocoagulation process for the elimination of an anthraquinone based aqueous solution of Red BFL dye. The efficiency of the electrodes in the dye removal was studied using X-Ray Photoelectron Spectroscopy of the collected sludge, in terms of the respective M(OH)n formation which contributes in coagulation of the dispersed dye molecules and the results indicated that Al formed four types of hydroxides and Cu only one type. The maximum removal of the dye solution obtained with Al was 99.17% at the optimum conditions: pH 8, contact time 15 min, current density 40 A m−2, and 91.88% with Cu: pH 9, contact time 25 min and current density 60 A m−2. Phytotoxicity and ecotoxicity studies with Vigna radiata and Artemia salina was done to investigate the toxicity of intermediate products in the treated Red BFL dye solution, results showed that the Al used Red BFL dye solution was less toxic in comparison to copper.Abbreviation: EC: Electrocoagulation; AQ: Anthraquinone; CD: Current density; CT: Contact time; ECE%: Efficiency in Colour Elimination percentage; HPLC: High-performance liquid chromatography; XPS: X-ray photoelectron spectroscopy; V. radiata: Vigna radiata; A. salina: Artemia salina
Author Bhagavathsingh, Jebasingh
Kalivel, Parameswari
Choondal Jisson, Jithin
David, Jovitha Jane
Palanichamy, Jegathambal
Padmanabhan, Dhanasekaran
Stephen, Asath Murphy Maria
Kavitha, Subbiah
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  organization: Karunya Institute of Technology and Sciences (Deemed to Be University)
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Snippet Anthraquinone dyes are tough to degrade compared to azo dyes, due to the resonance in the anthracene structure that leads to more difficulty in the removal and...
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SubjectTerms Aluminium
Aluminum
Analytical methods
Anthracene
Anthraquinone
Anthraquinone dyes
Aquatic crustaceans
Aqueous solutions
Artemia
Artemia salina
Azo dyes
Chromatography
Coagulation
Color removal
Copper
Current density
Decoloring
Decolorization
Dispersion
Dyes
EC method
ECE
ecotoxicity
Efficiency
Electrocoagulation
Electrodes
High performance liquid chromatography
HPLC
Hydroxides
Liquid chromatography
Photoelectron spectroscopy
Photoelectrons
Phytotoxicity
Red BFL dye
Removal
Sludge
Spectroscopy
Spectrum analysis
Toxicity
Vigna radiata
X ray photoelectron spectroscopy
X rays
XPS
Title Efficiency assessment of Cu and Al electrodes in the removal of anthraquinone based disperse dye aqueous solution in electrocoagulation-an analytical approach
URI https://www.tandfonline.com/doi/abs/10.1080/03067319.2021.1940988
https://www.proquest.com/docview/2879461389
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