A facile route to design pH-responsive viscoelastic wormlike micelles: Smart use of hydrotropes
A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route, pH-sensitive viscoelastic fluids can be easily obtained by introducing a pH-responsive hydrotrope into a surfactant solution. In this paper, the mix...
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| Published in | Journal of colloid and interface science Vol. 330; no. 2; pp. 449 - 455 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier Inc
15.02.2009
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route, pH-sensitive viscoelastic fluids can be easily obtained by introducing a pH-responsive hydrotrope into a surfactant solution. In this paper, the mixed system of cetyltrimethylammonium bromide (CTAB) and potassium phthalic acid (PPA) was studied in detail. This pH-sensitive fluid can be switched between a gellike state and a waterlike state within a narrow pH change. Rheology and DLS results revealed that the pH-sensitive flowing behavior was attributed to the microstructure transition between wormlike micelles and short cylindrical micelles. Combined with fluorescence anisotropy, NMR, and UV–vis, it was demonstrated that the pH response of viscoelastic fluid originated from the different binding abilities of hydrotrope to surfactant as pH varies. Furthermore, different kinds of hydrotropes can be utilized to prepare pH-responsive viscoelastic fluids in the desired pH areas.
The pH-responsive viscoelastic wormlike micelle solution is characterized by a macroscopic appearance and repeated viscosity switch. |
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| AbstractList | A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route, pH-sensitive viscoelastic fluids can be easily obtained by introducing a pH-responsive hydrotrope into a surfactant solution. In this paper, the mixed system of cetyltrimethylammonium bromide (CTAB) and potassium phthalic acid (PPA) was studied in detail. This pH-sensitive fluid can be switched between a gellike state and a waterlike state within a narrow pH change. Rheology and DLS results revealed that the pH-sensitive flowing behavior was attributed to the microstructure transition between wormlike micelles and short cylindrical micelles. Combined with fluorescence anisotropy, NMR, and UV-vis, it was demonstrated that the pH response of viscoelastic fluid originated from the different binding abilities of hydrotrope to surfactant as pH varies. Furthermore, different kinds of hydrotropes can be utilized to prepare pH-responsive viscoelastic fluids in the desired pH areas. A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route, pH-sensitive viscoelastic fluids can be easily obtained by introducing a pH-responsive hydrotrope into a surfactant solution. In this paper, the mixed system of cetyltrimethylammonium bromide (CTAB) and potassium phthalic acid (PPA) was studied in detail. This pH-sensitive fluid can be switched between a gellike state and a waterlike state within a narrow pH change. Rheology and DLS results revealed that the pH-sensitive flowing behavior was attributed to the microstructure transition between wormlike micelles and short cylindrical micelles. Combined with fluorescence anisotropy, NMR, and UV-vis, it was demonstrated that the pH response of viscoelastic fluid originated from the different binding abilities of hydrotrope to surfactant as pH varies. Furthermore, different kinds of hydrotropes can be utilized to prepare pH-responsive viscoelastic fluids in the desired pH areas.A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route, pH-sensitive viscoelastic fluids can be easily obtained by introducing a pH-responsive hydrotrope into a surfactant solution. In this paper, the mixed system of cetyltrimethylammonium bromide (CTAB) and potassium phthalic acid (PPA) was studied in detail. This pH-sensitive fluid can be switched between a gellike state and a waterlike state within a narrow pH change. Rheology and DLS results revealed that the pH-sensitive flowing behavior was attributed to the microstructure transition between wormlike micelles and short cylindrical micelles. Combined with fluorescence anisotropy, NMR, and UV-vis, it was demonstrated that the pH response of viscoelastic fluid originated from the different binding abilities of hydrotrope to surfactant as pH varies. Furthermore, different kinds of hydrotropes can be utilized to prepare pH-responsive viscoelastic fluids in the desired pH areas. A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route, pH-sensitive viscoelastic fluids can be easily obtained by introducing a pH-responsive hydrotrope into a surfactant solution. In this paper, the mixed system of cetyltrimethylammonium bromide (CTAB) and potassium phthalic acid (PPA) was studied in detail. This pH-sensitive fluid can be switched between a gellike state and a waterlike state within a narrow pH change. Rheology and DLS results revealed that the pH-sensitive flowing behavior was attributed to the microstructure transition between wormlike micelles and short cylindrical micelles. Combined with fluorescence anisotropy, NMR, and UV–vis, it was demonstrated that the pH response of viscoelastic fluid originated from the different binding abilities of hydrotrope to surfactant as pH varies. Furthermore, different kinds of hydrotropes can be utilized to prepare pH-responsive viscoelastic fluids in the desired pH areas. The pH-responsive viscoelastic wormlike micelle solution is characterized by a macroscopic appearance and repeated viscosity switch. |
| Author | Lin, Yiyang Yu, Cailan Huang, Jianbin Han, Xue Fu, Honglan |
| Author_xml | – sequence: 1 givenname: Yiyang surname: Lin fullname: Lin, Yiyang organization: Beijing National Laboratory for Molecular Sciences (BNLMS), State Key Laboratory for Structural Chemistry of Unstable and Stable Species, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, People's Republic of China – sequence: 2 givenname: Xue surname: Han fullname: Han, Xue organization: Beijing National Laboratory for Molecular Sciences (BNLMS), State Key Laboratory for Structural Chemistry of Unstable and Stable Species, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, People's Republic of China – sequence: 3 givenname: Jianbin surname: Huang fullname: Huang, Jianbin email: jbhuang@pku.edu.cn organization: Beijing National Laboratory for Molecular Sciences (BNLMS), State Key Laboratory for Structural Chemistry of Unstable and Stable Species, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, People's Republic of China – sequence: 4 givenname: Honglan surname: Fu fullname: Fu, Honglan organization: College of Life Science, Peking University, Beijing 100871, People's Republic of China – sequence: 5 givenname: Cailan surname: Yu fullname: Yu, Cailan organization: CAS Key Laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080, People's Republic of China |
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| Keywords | Viscoelastic fluid Hydrotrope Wormlike micelle pH responsive Binding Viscoelasticity Phthalic acid Rheology Fluid Cationic surfactant Fluorescence NMR spectrometry Surfactant Ionic surfactant Quaternary ammonium compound Design Anisotropy pH Microstructure Potassium Rheological properties |
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| Snippet | A simple and effective route to design pH-responsive viscoelastic wormlike micelles based on commercial compounds is reported. According to this route,... |
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| SubjectTerms | Cetrimonium Compounds - chemistry Chemistry Colloidal state and disperse state Exact sciences and technology General and physical chemistry Hydrogen-Ion Concentration Hydrotrope Micelles Micelles. Thin films Molecular Conformation pH responsive Phase Transition Phthalic Acids - chemistry Rheology Surface physical chemistry Viscoelastic fluid Wormlike micelle |
| Title | A facile route to design pH-responsive viscoelastic wormlike micelles: Smart use of hydrotropes |
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