Hidden first-order phase transitions and large magnetocaloric effects in GdNi1−xCox

We report a large magnetocaloric effect tunable between 70 and 115 K in a series of rare earth intermetallic compounds GdNi1−xCox with x varying from 0 to 0.15 that manifest rather unconventional second-order phase transitions with concurrent changes in both magnetic and crystallographic sublattices...

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Published inJournal of alloys and compounds Vol. 897; p. 163186
Main Authors Biswas, Anis, Del Rose, Tyler, Mudryk, Yaroslav, Ribeiro, P.O., Alho, B.P., de Sousa, V.S.R., Nóbrega, E.P., von Ranke, P.J., Pecharsky, Vitalij K.
Format Journal Article
LanguageEnglish
Published Lausanne Elsevier B.V 15.03.2022
Elsevier BV
Subjects
Coupling (molecular)
Crystallography
Curie temperature
Entropy
Gadolinium
Intermetallic alloys
Intermetallic compounds
Magnetic entropy change
Magnetic fields
Magnetic materials
Magnetic properties
Magnetic refrigeration
Magnetism
Magnetocaloric
Mean field theory
Phase transitions
Qualitative analysis
Magnetic refrigeration
Magnetic entropy change
Mean-field theory
Magnetocaloric
Intermetallic alloys
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Abstract We report a large magnetocaloric effect tunable between 70 and 115 K in a series of rare earth intermetallic compounds GdNi1−xCox with x varying from 0 to 0.15 that manifest rather unconventional second-order phase transitions with concurrent changes in both magnetic and crystallographic sublattices. While the Curie temperature, TC, linearly increases with x(Co), the maximum isothermal entropy change induced by magnetic field varying between 0 and 50 kOe slightly decreases from 14 J/kg K at 71 K when x(Co) = 0 to10 J/kg K at 115 K when x(Co) = 0.15. The temperature-averaged entropy change figures of merit calculated at temperature spans of 10 K for all examined compositions are comparable to those of the best known magnetocaloric materials that exhibit second-order phase transitions, including elemental Gd and La(Fe,Co,Si)13 alloys. Through a detailed analysis of the magnetic field-induced entropy changes along with assessment of critical exponents we explore the role magneto-elastic coupling plays in controlling magnetocaloric properties of GdNi1−xCox compounds. We also formulate a model based on the mean field theory approximation to describe both magnetic and magnetocaloric properties of the title materials in qualitative agreement with experimental results. •Large cryogenic MCE is obtained for GdNi1-xCox (x=0,0.05,0.10,0.15).•TEC s for GdNi1-xCox are comparable to other potential magnetocaloric material.•The role of magneto-elastic coupling on the MCE of GdNi1-xCox is explored.•A theoretical model is formulated to describe MCE of the compound.
AbstractList We report a large magnetocaloric effect tunable between 70 and 115 K in a series of rare earth intermetallic compounds GdNi1−xCox with x varying from 0 to 0.15 that manifest rather unconventional second-order phase transitions with concurrent changes in both magnetic and crystallographic sublattices. While the Curie temperature, TC, linearly increases with x(Co), the maximum isothermal entropy change induced by magnetic field varying between 0 and 50 kOe slightly decreases from 14 J/kg K at 71 K when x(Co) = 0 to10 J/kg K at 115 K when x(Co) = 0.15. The temperature-averaged entropy change figures of merit calculated at temperature spans of 10 K for all examined compositions are comparable to those of the best known magnetocaloric materials that exhibit second-order phase transitions, including elemental Gd and La(Fe,Co,Si)13 alloys. Through a detailed analysis of the magnetic field-induced entropy changes along with assessment of critical exponents we explore the role magneto-elastic coupling plays in controlling magnetocaloric properties of GdNi1−xCox compounds. We also formulate a model based on the mean field theory approximation to describe both magnetic and magnetocaloric properties of the title materials in qualitative agreement with experimental results.
We report a large magnetocaloric effect tunable between 70 and 115 K in a series of rare earth intermetallic compounds GdNi1−xCox with x varying from 0 to 0.15 that manifest rather unconventional second-order phase transitions with concurrent changes in both magnetic and crystallographic sublattices. While the Curie temperature, TC, linearly increases with x(Co), the maximum isothermal entropy change induced by magnetic field varying between 0 and 50 kOe slightly decreases from 14 J/kg K at 71 K when x(Co) = 0 to10 J/kg K at 115 K when x(Co) = 0.15. The temperature-averaged entropy change figures of merit calculated at temperature spans of 10 K for all examined compositions are comparable to those of the best known magnetocaloric materials that exhibit second-order phase transitions, including elemental Gd and La(Fe,Co,Si)13 alloys. Through a detailed analysis of the magnetic field-induced entropy changes along with assessment of critical exponents we explore the role magneto-elastic coupling plays in controlling magnetocaloric properties of GdNi1−xCox compounds. We also formulate a model based on the mean field theory approximation to describe both magnetic and magnetocaloric properties of the title materials in qualitative agreement with experimental results. •Large cryogenic MCE is obtained for GdNi1-xCox (x=0,0.05,0.10,0.15).•TEC s for GdNi1-xCox are comparable to other potential magnetocaloric material.•The role of magneto-elastic coupling on the MCE of GdNi1-xCox is explored.•A theoretical model is formulated to describe MCE of the compound.
ArticleNumber 163186
Author Mudryk, Yaroslav
Biswas, Anis
Pecharsky, Vitalij K.
von Ranke, P.J.
Alho, B.P.
de Sousa, V.S.R.
Del Rose, Tyler
Ribeiro, P.O.
Nóbrega, E.P.
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  givenname: Tyler
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  organization: The Ames Laboratory, US Department of Energy, Iowa State University, Ames, IA 50011, USA
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  organization: Instituto de Física, Universidade do Estado do Rio de Janeiro – UERJ, Rua São Francisco Xavier 524, RJ 20550-013, Brazil
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  surname: Nóbrega
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  givenname: P.J.
  surname: von Ranke
  fullname: von Ranke, P.J.
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  givenname: Vitalij K.
  surname: Pecharsky
  fullname: Pecharsky, Vitalij K.
  organization: The Ames Laboratory, US Department of Energy, Iowa State University, Ames, IA 50011, USA
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Magnetic entropy change
Mean-field theory
Magnetocaloric
Intermetallic alloys
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Snippet We report a large magnetocaloric effect tunable between 70 and 115 K in a series of rare earth intermetallic compounds GdNi1−xCox with x varying from 0 to 0.15...
We report a large magnetocaloric effect tunable between 70 and 115 K in a series of rare earth intermetallic compounds GdNi1−xCox with x varying from 0 to 0.15...
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StartPage 163186
SubjectTerms Coupling (molecular)
Crystallography
Curie temperature
Entropy
Gadolinium
Intermetallic alloys
Intermetallic compounds
Magnetic entropy change
Magnetic fields
Magnetic materials
Magnetic properties
Magnetic refrigeration
Magnetism
Magnetocaloric
Mean field theory
Phase transitions
Qualitative analysis
Title Hidden first-order phase transitions and large magnetocaloric effects in GdNi1−xCox
URI https://dx.doi.org/10.1016/j.jallcom.2021.163186
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Volume 897
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