On the impact of global interactions on the structure of metallic glasses
The influence of global interactions between the static atomic structure and the valence electrons on structure formation in binary Al-(Ni,Cu,Zr), Zr-(Ni,Cu) and ternary Al-(Ni,Cu)-Zr metallic glasses is investigated over wide concentration ranges and discussed in terms of a Hume-Rothery-like theory...
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Published in | Journal of alloys and compounds Vol. 782; pp. 496 - 505 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
Published |
Lausanne
Elsevier B.V
25.04.2019
Elsevier BV |
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Abstract | The influence of global interactions between the static atomic structure and the valence electrons on structure formation in binary Al-(Ni,Cu,Zr), Zr-(Ni,Cu) and ternary Al-(Ni,Cu)-Zr metallic glasses is investigated over wide concentration ranges and discussed in terms of a Hume-Rothery-like theory by analysing and comparing data available in the literature. The results suggest that global interactions lead to an improvement of thermal stability and glass-forming ability. A complete understanding of structure formation in the considered alloys is assumed to be possible only by taking into account both local and global effects.
•The effect of global interactions on thermal stability and glass-forming ability in Al-(Ni,Cu)-Zr metallic glasses is analysed.•A Hume-Rothery-like effect according to a mean valence of 1.5 electrons per atom plays a major role.•Local and global effects mutually support each other to yield the energetically most favorable structure.•Correlations with other properties are pointed out. |
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AbstractList | The influence of global interactions between the static atomic structure and the valence electrons on structure formation in binary Al-(Ni,Cu,Zr), Zr-(Ni,Cu) and ternary Al-(Ni,Cu)-Zr metallic glasses is investigated over wide concentration ranges and discussed in terms of a Hume-Rothery-like theory by analysing and comparing data available in the literature. The results suggest that global interactions lead to an improvement of thermal stability and glass-forming ability. A complete understanding of structure formation in the considered alloys is assumed to be possible only by taking into account both local and global effects. The influence of global interactions between the static atomic structure and the valence electrons on structure formation in binary Al-(Ni,Cu,Zr), Zr-(Ni,Cu) and ternary Al-(Ni,Cu)-Zr metallic glasses is investigated over wide concentration ranges and discussed in terms of a Hume-Rothery-like theory by analysing and comparing data available in the literature. The results suggest that global interactions lead to an improvement of thermal stability and glass-forming ability. A complete understanding of structure formation in the considered alloys is assumed to be possible only by taking into account both local and global effects. •The effect of global interactions on thermal stability and glass-forming ability in Al-(Ni,Cu)-Zr metallic glasses is analysed.•A Hume-Rothery-like effect according to a mean valence of 1.5 electrons per atom plays a major role.•Local and global effects mutually support each other to yield the energetically most favorable structure.•Correlations with other properties are pointed out. |
Author | Stiehler, Martin E. Jolly, Mark R. Georgarakis, Konstantinos |
Author_xml | – sequence: 1 givenname: Martin E. orcidid: 0000-0002-6941-2025 surname: Stiehler fullname: Stiehler, Martin E. email: martin.stiehler@cranfield.ac.uk – sequence: 2 givenname: Mark R. orcidid: 0000-0001-6357-3584 surname: Jolly fullname: Jolly, Mark R. – sequence: 3 givenname: Konstantinos surname: Georgarakis fullname: Georgarakis, Konstantinos |
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CitedBy_id | crossref_primary_10_1007_s11837_021_05106_x crossref_primary_10_1016_j_mtcomm_2022_103531 crossref_primary_10_1016_j_matchar_2021_110967 crossref_primary_10_1016_j_jallcom_2019_153486 |
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Keywords | Metallic glasses Hume-Rothery Aluminum alloys Electronic structure Glass-forming ability Zirconium alloys |
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SubjectTerms | Aluminum Aluminum alloys Amorphous alloys Amorphous materials Atomic structure Copper Electronic structure Glass-forming ability Hume-Rothery Metallic glasses Nickel Thermal stability Zirconium Zirconium alloys |
Title | On the impact of global interactions on the structure of metallic glasses |
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