Over 17% efficiency ternary organic solar cells enabled by two non-fullerene acceptors working in an alloy-like model
Nowadays, organic solar cells (OSCs) with Y6 and its derivatives as electron acceptors provide the highest efficiencies among the studied binary OSCs. To further improve the performances of OSCs, the fabrication of ternary OSCs (TOSCs) is a convenient strategy. Essentially, morphology control and th...
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| Published in | Energy & environmental science Vol. 13; no. 2; pp. 635 - 645 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
01.01.2020
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | Nowadays, organic solar cells (OSCs) with Y6 and its derivatives as electron acceptors provide the highest efficiencies among the studied binary OSCs. To further improve the performances of OSCs, the fabrication of ternary OSCs (TOSCs) is a convenient strategy. Essentially, morphology control and the trade-off between voltage and photocurrent are the main critical issues in TOSCs. Herein, we address these problems by constructing TOSCs where an alloy-like composite is formed between Y6 and a newly designed derivative, BTP-M. Employing an electron-pushing methyl substituent as a replacement for the electron-withdrawing F atoms on Y6, BTP-M shows higher energy levels and lower crystallinity than Y6. As a result, the obtained Y6:BTP-M alloy can simultaneously optimize energy levels to reduce energy loss as well as the morphologies of the active layers to favor photocurrent generation, leading to an enhanced open-circuit voltage (
V
oc
) of 0.875 V together with a larger short-circuit current density (
J
sc
) of 26.56 mA cm
−2
for TOSCs based on the polymer donor PM6 and Y6:BTP-M acceptor alloy. Consequently, a best efficiency of 17.03% is achieved for the corresponding TOSCs, which is among the best values for single-junction OSCs. In addition, our TOSCs also exhibit good thickness tolerance, and can reach 14.23% efficiency even though the active layer is as thick as 300 nm.
An alloy-like model based on Y6 and its derivative BTP-M is constructed to fabricate ternary organic solar cells, leading to a best efficiency of 17.03%. |
|---|---|
| AbstractList | Nowadays, organic solar cells (OSCs) with Y6 and its derivatives as electron acceptors provide the highest efficiencies among the studied binary OSCs. To further improve the performances of OSCs, the fabrication of ternary OSCs (TOSCs) is a convenient strategy. Essentially, morphology control and the trade-off between voltage and photocurrent are the main critical issues in TOSCs. Herein, we address these problems by constructing TOSCs where an alloy-like composite is formed between Y6 and a newly designed derivative, BTP-M. Employing an electron-pushing methyl substituent as a replacement for the electron-withdrawing F atoms on Y6, BTP-M shows higher energy levels and lower crystallinity than Y6. As a result, the obtained Y6:BTP-M alloy can simultaneously optimize energy levels to reduce energy loss as well as the morphologies of the active layers to favor photocurrent generation, leading to an enhanced open-circuit voltage (Voc) of 0.875 V together with a larger short-circuit current density (Jsc) of 26.56 mA cm−2 for TOSCs based on the polymer donor PM6 and Y6:BTP-M acceptor alloy. Consequently, a best efficiency of 17.03% is achieved for the corresponding TOSCs, which is among the best values for single-junction OSCs. In addition, our TOSCs also exhibit good thickness tolerance, and can reach 14.23% efficiency even though the active layer is as thick as 300 nm. Nowadays, organic solar cells (OSCs) with Y6 and its derivatives as electron acceptors provide the highest efficiencies among the studied binary OSCs. To further improve the performances of OSCs, the fabrication of ternary OSCs (TOSCs) is a convenient strategy. Essentially, morphology control and the trade-off between voltage and photocurrent are the main critical issues in TOSCs. Herein, we address these problems by constructing TOSCs where an alloy-like composite is formed between Y6 and a newly designed derivative, BTP-M. Employing an electron-pushing methyl substituent as a replacement for the electron-withdrawing F atoms on Y6, BTP-M shows higher energy levels and lower crystallinity than Y6. As a result, the obtained Y6:BTP-M alloy can simultaneously optimize energy levels to reduce energy loss as well as the morphologies of the active layers to favor photocurrent generation, leading to an enhanced open-circuit voltage ( V oc ) of 0.875 V together with a larger short-circuit current density ( J sc ) of 26.56 mA cm −2 for TOSCs based on the polymer donor PM6 and Y6:BTP-M acceptor alloy. Consequently, a best efficiency of 17.03% is achieved for the corresponding TOSCs, which is among the best values for single-junction OSCs. In addition, our TOSCs also exhibit good thickness tolerance, and can reach 14.23% efficiency even though the active layer is as thick as 300 nm. An alloy-like model based on Y6 and its derivative BTP-M is constructed to fabricate ternary organic solar cells, leading to a best efficiency of 17.03%. Nowadays, organic solar cells (OSCs) with Y6 and its derivatives as electron acceptors provide the highest efficiencies among the studied binary OSCs. To further improve the performances of OSCs, the fabrication of ternary OSCs (TOSCs) is a convenient strategy. Essentially, morphology control and the trade-off between voltage and photocurrent are the main critical issues in TOSCs. Herein, we address these problems by constructing TOSCs where an alloy-like composite is formed between Y6 and a newly designed derivative, BTP-M. Employing an electron-pushing methyl substituent as a replacement for the electron-withdrawing F atoms on Y6, BTP-M shows higher energy levels and lower crystallinity than Y6. As a result, the obtained Y6:BTP-M alloy can simultaneously optimize energy levels to reduce energy loss as well as the morphologies of the active layers to favor photocurrent generation, leading to an enhanced open-circuit voltage ( V oc ) of 0.875 V together with a larger short-circuit current density ( J sc ) of 26.56 mA cm −2 for TOSCs based on the polymer donor PM6 and Y6:BTP-M acceptor alloy. Consequently, a best efficiency of 17.03% is achieved for the corresponding TOSCs, which is among the best values for single-junction OSCs. In addition, our TOSCs also exhibit good thickness tolerance, and can reach 14.23% efficiency even though the active layer is as thick as 300 nm. |
| Author | Shi, Minmin Hou, Jianhui Li, Chang-Zhi Li, Hanying Cui, Yong Lu, Xinhui Lau, Tsz-Ki Chen, Hongzheng Zhan, Lingling Li, Shuixing |
| AuthorAffiliation | Department of Polymer Science and Engineering Chinese Academy of Sciences Institute of Chemistry New Territories State Key Laboratory of Silicon Materials Chinese University of Hong Kong Zhejiang University MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Physics |
| AuthorAffiliation_xml | – sequence: 0 name: Department of Physics – sequence: 0 name: Chinese University of Hong Kong – sequence: 0 name: Chinese Academy of Sciences – sequence: 0 name: Department of Polymer Science and Engineering – sequence: 0 name: MOE Key Laboratory of Macromolecular Synthesis and Functionalization – sequence: 0 name: New Territories – sequence: 0 name: Zhejiang University – sequence: 0 name: Institute of Chemistry – sequence: 0 name: State Key Laboratory of Silicon Materials |
| Author_xml | – sequence: 1 givenname: Lingling surname: Zhan fullname: Zhan, Lingling – sequence: 2 givenname: Shuixing surname: Li fullname: Li, Shuixing – sequence: 3 givenname: Tsz-Ki surname: Lau fullname: Lau, Tsz-Ki – sequence: 4 givenname: Yong surname: Cui fullname: Cui, Yong – sequence: 5 givenname: Xinhui surname: Lu fullname: Lu, Xinhui – sequence: 6 givenname: Minmin surname: Shi fullname: Shi, Minmin – sequence: 7 givenname: Chang-Zhi surname: Li fullname: Li, Chang-Zhi – sequence: 8 givenname: Hanying surname: Li fullname: Li, Hanying – sequence: 9 givenname: Jianhui surname: Hou fullname: Hou, Jianhui – sequence: 10 givenname: Hongzheng surname: Chen fullname: Chen, Hongzheng |
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| References | Mai (C9EE03710A-(cit63)/*[position()=1]) 2018; 30 Lee (C9EE03710A-(cit24)/*[position()=1]) 2019; 31 Liu (C9EE03710A-(cit46)/*[position()=1]) 2019; 12 Kyaw (C9EE03710A-(cit61)/*[position()=1]) 2013; 7 Xu (C9EE03710A-(cit19)/*[position()=1]) 2019; 31 Holliday (C9EE03710A-(cit9)/*[position()=1]) 2016; 7 Yan (C9EE03710A-(cit3)/*[position()=1]) 2018; 3 Cui (C9EE03710A-(cit18)/*[position()=1]) 2019; 10 Wang (C9EE03710A-(cit48)/*[position()=1]) 2019; 3 Sun (C9EE03710A-(cit20)/*[position()=1]) 2019; 12 Yuan (C9EE03710A-(cit15)/*[position()=1]) 2019; 31 Mai (C9EE03710A-(cit64)/*[position()=1]) 2016; 28 Zhan (C9EE03710A-(cit36)/*[position()=1]) 2018; 5 Zerio (C9EE03710A-(cit39)/*[position()=1]) 2018; 8 Yu (C9EE03710A-(cit32)/*[position()=1]) 2019; 31 Zhang (C9EE03710A-(cit31)/*[position()=1]) 2018; 11 Li (C9EE03710A-(cit52)/*[position()=1]) 2018; 6 Xiao (C9EE03710A-(cit58)/*[position()=1]) 2018; 2 Liu (C9EE03710A-(cit65)/*[position()=1]) 2018; 11 Yuan (C9EE03710A-(cit14)/*[position()=1]) 2019; 10 Lin (C9EE03710A-(cit6)/*[position()=1]) 2015; 27 Yu (C9EE03710A-(cit11)/*[position()=1]) 2019; 10 Qian (C9EE03710A-(cit49)/*[position()=1]) 2018; 17 Xiao (C9EE03710A-(cit8)/*[position()=1]) 2017; 62 Ye (C9EE03710A-(cit53)/*[position()=1]) 2018; 17 Li (C9EE03710A-(cit35)/*[position()=1]) 2017; 19 Li (C9EE03710A-(cit54)/*[position()=1]) 2016; 28 Yu (C9EE03710A-(cit22)/*[position()=1]) 2018; 8 Ma (C9EE03710A-(cit45)/*[position()=1]) 2019; 7 Li (C9EE03710A-(cit51)/*[position()=1]) 2019; 141 Pan (C9EE03710A-(cit34)/*[position()=1]) 2019; 7 Zhang (C9EE03710A-(cit12)/*[position()=1]) 2019; 35 Søndergaard (C9EE03710A-(cit56)/*[position()=1]) 2012; 15 Zhang (C9EE03710A-(cit40)/*[position()=1]) 2015; 137 Chen (C9EE03710A-(cit62)/*[position()=1]) 2019; 3 Zhang (C9EE03710A-(cit17)/*[position()=1]) 2015; 27 An (C9EE03710A-(cit26)/*[position()=1]) 2016; 9 Huang (C9EE03710A-(cit57)/*[position()=1]) 2020; 7 Li (C9EE03710A-(cit10)/*[position()=1]) 2018; 30 Zhan (C9EE03710A-(cit28)/*[position()=1]) 2019; 3 Zhao (C9EE03710A-(cit7)/*[position()=1]) 2017; 139 Lu (C9EE03710A-(cit21)/*[position()=1]) 2015; 9 Zhou (C9EE03710A-(cit42)/*[position()=1]) 2018; 3 Hou (C9EE03710A-(cit1)/*[position()=1]) 2018; 17 Kang (C9EE03710A-(cit5)/*[position()=1]) 2016; 28 Tang (C9EE03710A-(cit60)/*[position()=1]) 2019; 6 Nian (C9EE03710A-(cit30)/*[position()=1]) 2018; 11 Li (C9EE03710A-(cit2)/*[position()=1]) 2017; 13 Yuan (C9EE03710A-(cit13)/*[position()=1]) 2019; 3 Qian (C9EE03710A-(cit59)/*[position()=1]) 2012; 45 Li (C9EE03710A-(cit4)/*[position()=1]) 2019; 3 Zhan (C9EE03710A-(cit37)/*[position()=1]) 2018; 10 Su (C9EE03710A-(cit41)/*[position()=1]) 2017; 38 Zhao (C9EE03710A-(cit43)/*[position()=1]) 2019; 4 Yan (C9EE03710A-(cit33)/*[position()=1]) 2019; 31 Li (C9EE03710A-(cit25)/*[position()=1]) 2017; 7 Lai (C9EE03710A-(cit55)/*[position()=1]) 2019; 17 Cheng (C9EE03710A-(cit38)/*[position()=1]) 2016; 28 Chen (C9EE03710A-(cit16)/*[position()=1]) 2019; 62 Xie (C9EE03710A-(cit47)/*[position()=1]) 2019; 4 Chen (C9EE03710A-(cit44)/*[position()=1]) 2017; 29 Lu (C9EE03710A-(cit27)/*[position()=1]) 2015; 6 Ma (C9EE03710A-(cit29)/*[position()=1]) 2018; 11 Huang (C9EE03710A-(cit23)/*[position()=1]) 2018; 30 Liu (C9EE03710A-(cit50)/*[position()=1]) 2016; 1 |
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| Snippet | Nowadays, organic solar cells (OSCs) with Y6 and its derivatives as electron acceptors provide the highest efficiencies among the studied binary OSCs. To... |
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| SubjectTerms | Circuits Efficiency Electrons Energy Energy dissipation Energy levels Energy loss Fabrication Fullerenes Morphology NMR Nuclear magnetic resonance Open circuit voltage Organic chemistry Performance enhancement Photoelectric effect Photoelectric emission Photovoltaic cells Polymers Short circuit currents Short-circuit current Solar cells Voltage |
| Title | Over 17% efficiency ternary organic solar cells enabled by two non-fullerene acceptors working in an alloy-like model |
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