Zein films with ZnO and ZnO:Mg quantum dots as functional nanofillers: New nanocomposites for food package with UV-blocker and antimicrobial properties
The preparation of a new nanocomposite by combining zein and quantum dots (QDs) was the main interest of the present work. By the sol-gel method, colloidal ethanolic dispersions of zinc oxide (ZnO) particles and ZnO particles doped with magnesium (II) (ZnO:Mg) were obtained, sized 4.26 and 3.65 nm,...
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Published in | Polymer testing Vol. 91; p. 106709 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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01.11.2020
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Abstract | The preparation of a new nanocomposite by combining zein and quantum dots (QDs) was the main interest of the present work. By the sol-gel method, colloidal ethanolic dispersions of zinc oxide (ZnO) particles and ZnO particles doped with magnesium (II) (ZnO:Mg) were obtained, sized 4.26 and 3.65 nm, respectively, as determined by UV–Vis spectroscopy. The prepared QDs were used as nanofillers in order to obtain zein-based nanocomposite films, which displayed good visual appearance, homogeneity, and transparency. The presence of QDs increased the hydrophobicity and reduced, up to three times, the amount of water uptake of the composite films when compared to pure zein. Those effects were more pronounced for ZnO:Mg QDs. TEM, FTIR, and fluorescence microscopy analysis indicated that zein interacts more effectively with ZnO:Mg than with ZnO. In addition, and most importantly, the presence of QDs in the films showed an important advantage when compared to those of pure zein: the extended UV-blocking in the absorbance spectra. The antimicrobial assays demonstrated that the ZnO NPs, loaded into zein films, are promising antibacterial materials since the inhibition of growth of S. aureus reached (96.5 ± 4.9)% at 44.8 wt% of ZnO NPs. Therefore, the nanocomposites show promising features for the development of food packaging, UV protective films, and for the development of new and sustainable materials.
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•Nanocomposites with zein and ZnO quantum dots as a substitute of synthetic plastics.•Zein@ZnO QDs and Zein@ZnO:Mg QDs in food packaging with UV-blocker properties.•Nanomaterial obtained with potential for food packaging with antimicrobial activity.•Nanocomposites obtained with higher hydrophobicity than pure zein.•Transparent bioplastic with zein and ZnO quantum dots. |
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AbstractList | The preparation of a new nanocomposite by combining zein and quantum dots (QDs) was the main interest of the present work. By the sol-gel method, colloidal ethanolic dispersions of zinc oxide (ZnO) particles and ZnO particles doped with magnesium (II) (ZnO:Mg) were obtained, sized 4.26 and 3.65 nm, respectively, as determined by UV–Vis spectroscopy. The prepared QDs were used as nanofillers in order to obtain zein-based nanocomposite films, which displayed good visual appearance, homogeneity, and transparency. The presence of QDs increased the hydrophobicity and reduced, up to three times, the amount of water uptake of the composite films when compared to pure zein. Those effects were more pronounced for ZnO:Mg QDs. TEM, FTIR, and fluorescence microscopy analysis indicated that zein interacts more effectively with ZnO:Mg than with ZnO. In addition, and most importantly, the presence of QDs in the films showed an important advantage when compared to those of pure zein: the extended UV-blocking in the absorbance spectra. The antimicrobial assays demonstrated that the ZnO NPs, loaded into zein films, are promising antibacterial materials since the inhibition of growth of S. aureus reached (96.5 ± 4.9)% at 44.8 wt% of ZnO NPs. Therefore, the nanocomposites show promising features for the development of food packaging, UV protective films, and for the development of new and sustainable materials.
[Display omitted]
•Nanocomposites with zein and ZnO quantum dots as a substitute of synthetic plastics.•Zein@ZnO QDs and Zein@ZnO:Mg QDs in food packaging with UV-blocker properties.•Nanomaterial obtained with potential for food packaging with antimicrobial activity.•Nanocomposites obtained with higher hydrophobicity than pure zein.•Transparent bioplastic with zein and ZnO quantum dots. |
ArticleNumber | 106709 |
Author | Riegel-Vidotti, Izabel Cristina Zimmermann, Lizandra Maria Alberton, Michele Debiasi Schmitz, Francielle Silva de Albuquerque, Maria Beatriz |
Author_xml | – sequence: 1 givenname: Francielle surname: Schmitz fullname: Schmitz, Francielle organization: Department of Chemistry, Regional University of Blumenau - FURB, 89030-903, Blumenau, SC, Brazil – sequence: 2 givenname: Maria Beatriz surname: Silva de Albuquerque fullname: Silva de Albuquerque, Maria Beatriz organization: Department of Pharmacy, Regional University of Blumenau - FURB, 89030-903, Blumenau, SC, Brazil – sequence: 3 givenname: Michele Debiasi surname: Alberton fullname: Alberton, Michele Debiasi organization: Department of Pharmacy, Regional University of Blumenau - FURB, 89030-903, Blumenau, SC, Brazil – sequence: 4 givenname: Izabel Cristina surname: Riegel-Vidotti fullname: Riegel-Vidotti, Izabel Cristina organization: Department of Chemistry, Grupo de Pesquisa em Macromoléculas e Interfaces, Universidade Federal do Paraná - UFPR, Zip Code 19081, CEP 81531-980, Curitiba, Brazil – sequence: 5 givenname: Lizandra Maria surname: Zimmermann fullname: Zimmermann, Lizandra Maria email: lmz@furb.br, lizazimer@gmail.com organization: Department of Chemistry, Regional University of Blumenau - FURB, 89030-903, Blumenau, SC, Brazil |
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Keywords | ZnO UV-blocker Nanocomposites Quantum dots Bioplastic Antibacterial materials |
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Snippet | The preparation of a new nanocomposite by combining zein and quantum dots (QDs) was the main interest of the present work. By the sol-gel method, colloidal... |
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SubjectTerms | Antibacterial materials Bioplastic Nanocomposites Quantum dots UV-blocker ZnO |
Title | Zein films with ZnO and ZnO:Mg quantum dots as functional nanofillers: New nanocomposites for food package with UV-blocker and antimicrobial properties |
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