Cubic perturbed centrifugally stabilized excited state in orthorhombic manganites
A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper “Mexican hat” potential surface for a Mn3+ ion in an octahedral symmetry is formulated, and its eigenspectrum is explored. Theoretically calculated eigenvalues for cubic perturbed ground and exc...
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| Published in | The Journal of chemical physics Vol. 150; no. 6; pp. 064703 - 64716 |
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| Abstract | A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper “Mexican hat” potential surface for a Mn3+ ion in an octahedral symmetry is formulated, and its eigenspectrum is explored. Theoretically calculated eigenvalues for cubic perturbed ground and excited electronic states are employed to interpret the origin of higher energy narrow side bands (satellite transitions) appearing in the dielectric function spectra of the LaMnO3 complex, which exhibit anomalous temperature dependence in the vicinity of the Néel temperature, TN ≃ 140 K [N. N. Kovaleva et al., J. Exp. Theor. Phys. 122, 890 (2016)]. |
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| AbstractList | A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper "Mexican hat" potential surface for a Mn
ion in an octahedral symmetry is formulated, and its eigenspectrum is explored. Theoretically calculated eigenvalues for cubic perturbed ground and excited electronic states are employed to interpret the origin of higher energy narrow side bands (satellite transitions) appearing in the dielectric function spectra of the LaMnO
complex, which exhibit anomalous temperature dependence in the vicinity of the Néel temperature, T
≃ 140 K [N. N. Kovaleva et al., J. Exp. Theor. Phys. 122, 890 (2016)]. A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper “Mexican hat” potential surface for a Mn3+ ion in an octahedral symmetry is formulated, and its eigenspectrum is explored. Theoretically calculated eigenvalues for cubic perturbed ground and excited electronic states are employed to interpret the origin of higher energy narrow side bands (satellite transitions) appearing in the dielectric function spectra of the LaMnO3 complex, which exhibit anomalous temperature dependence in the vicinity of the Néel temperature, TN ≃ 140 K [N. N. Kovaleva et al., J. Exp. Theor. Phys. 122, 890 (2016)]. A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper "Mexican hat" potential surface for a Mn3+ ion in an octahedral symmetry is formulated, and its eigenspectrum is explored. Theoretically calculated eigenvalues for cubic perturbed ground and excited electronic states are employed to interpret the origin of higher energy narrow side bands (satellite transitions) appearing in the dielectric function spectra of the LaMnO3 complex, which exhibit anomalous temperature dependence in the vicinity of the Néel temperature, TN ≃ 140 K [N. N. Kovaleva et al., J. Exp. Theor. Phys. 122, 890 (2016)].A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper "Mexican hat" potential surface for a Mn3+ ion in an octahedral symmetry is formulated, and its eigenspectrum is explored. Theoretically calculated eigenvalues for cubic perturbed ground and excited electronic states are employed to interpret the origin of higher energy narrow side bands (satellite transitions) appearing in the dielectric function spectra of the LaMnO3 complex, which exhibit anomalous temperature dependence in the vicinity of the Néel temperature, TN ≃ 140 K [N. N. Kovaleva et al., J. Exp. Theor. Phys. 122, 890 (2016)]. |
| Author | Adhikari, Satrajit Dutta, Joy Kovaleva, N. N. |
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| Cites_doi | 10.1103/physrevb.72.214431 10.1103/physreva.62.032507 10.1103/physrevb.57.r3189 10.1070/pu1975v018n08abeh004913 10.1103/physrev.131.1596 10.1103/physrevlett.93.147204 10.1143/jpsj.65.3736 10.1098/rspa.1958.0038 10.1103/physreva.62.032506 10.1134/1.1448620 10.1088/0953-8984/25/15/155602 10.1002/qua.21870 10.1098/rspa.1957.0010 10.1098/rspa.1964.0185 10.1021/jp8029709 10.1103/physrevb.65.205113 10.1016/j.cplett.2010.01.032 10.1103/physrevb.97.125149 10.1134/s1063776116050174 10.1070/pu1982v025n04abeh004537 10.1098/rspa.1937.0142 10.1063/1.1750327 10.1039/c0cp02598d 10.1103/physrevb.81.235130 10.1063/1.2170089 |
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| Snippet | A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper “Mexican hat” potential surface for a Mn3+ ion in an... A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper "Mexican hat" potential surface for a Mn ion in an... A model Hamiltonian for centrifugally stabilized electronic-vibrational motion of a cubic perturbed upper "Mexican hat" potential surface for a Mn3+ ion in an... |
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| SubjectTerms | Eigenvalues Electron states Lanthanum compounds Manganese ions Physics Temperature dependence |
| Title | Cubic perturbed centrifugally stabilized excited state in orthorhombic manganites |
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