Formic Acid to Power towards Low‐Carbon Economy

The storage and utilization of low‐carbon electricity and decarbonization of transportation are essential components for the future energy transition into a low‐carbon economy. While hydrogen has been identified as a potential energy carrier, the lack of viable technologies for safe and efficient st...

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Bibliographic Details
Published inAdvanced energy materials Vol. 12; no. 15
Main Authors Dutta, Indranil, Chatterjee, Sudipta, Cheng, Hongfei, Parsapur, Rajesh Kumar, Liu, Zhaolin, Li, Zibiao, Ye, Enyi, Kawanami, Hajime, Low, Jonathan Sze Choong, Lai, Zhiping, Loh, Xian Jun, Huang, Kuo‐Wei
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 01.04.2022
Subjects
Carbon
Dehydrogenation
Economic analysis
Energy storage
Flammability
Formic acid
Fuel cells
high pressure gas production
hydrogen energy carrier
Hydrogen production
Hydrogen-based energy
Life cycle assessment
Liquefaction
Potential energy
Storage capacity
Toxicity
Transportation
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Abstract The storage and utilization of low‐carbon electricity and decarbonization of transportation are essential components for the future energy transition into a low‐carbon economy. While hydrogen has been identified as a potential energy carrier, the lack of viable technologies for safe and efficient storage and transportation of H2 greatly limits its applications and deployment at scale. Formic acid (FA) is considered one of the promising H2 energy carriers because of its high volumetric H2 storage capacity of 53 g H2/L, and relatively low toxicity and flammability for convenient and low‐cost storage and transportation. FA can be employed to generate electricity either in direct FA fuel cells (FCs) or indirectly as an H2 source for hydrogen FCs. FA can enable large‐scale chemical H2 storage to eliminate energy‐intensive and expensive processes for H2 liquefaction and compression and thus to achieve higher efficiency and broader utilization. This perspective summarizes recent advances in catalyst development for selective dehydrogenation of FA and high‐pressure H2 production. The advantages and limitations of FA‐to‐power options are highlighted. Existing life cycle assessment (LCA) and economic analysis studies are reviewed to discuss the feasibility and future potential of FA as a fuel. The utilization of low‐carbon electricity and decarbonization of transportation are essential to a low‐carbon economy. Hydrogen has been identified as an energy carrier, but the lack of viable storage and distribution technologies greatly limits its uses. A chemical hydrogen storage system powered by formic acid can replace energy‐intensive liquefaction and compression processes for hydrogen, enabling higher efficiency and broader applications.
AbstractList The storage and utilization of low‐carbon electricity and decarbonization of transportation are essential components for the future energy transition into a low‐carbon economy. While hydrogen has been identified as a potential energy carrier, the lack of viable technologies for safe and efficient storage and transportation of H2 greatly limits its applications and deployment at scale. Formic acid (FA) is considered one of the promising H2 energy carriers because of its high volumetric H2 storage capacity of 53 g H2/L, and relatively low toxicity and flammability for convenient and low‐cost storage and transportation. FA can be employed to generate electricity either in direct FA fuel cells (FCs) or indirectly as an H2 source for hydrogen FCs. FA can enable large‐scale chemical H2 storage to eliminate energy‐intensive and expensive processes for H2 liquefaction and compression and thus to achieve higher efficiency and broader utilization. This perspective summarizes recent advances in catalyst development for selective dehydrogenation of FA and high‐pressure H2 production. The advantages and limitations of FA‐to‐power options are highlighted. Existing life cycle assessment (LCA) and economic analysis studies are reviewed to discuss the feasibility and future potential of FA as a fuel.
The storage and utilization of low‐carbon electricity and decarbonization of transportation are essential components for the future energy transition into a low‐carbon economy. While hydrogen has been identified as a potential energy carrier, the lack of viable technologies for safe and efficient storage and transportation of H 2 greatly limits its applications and deployment at scale. Formic acid (FA) is considered one of the promising H 2 energy carriers because of its high volumetric H 2 storage capacity of 53 g H 2 /L, and relatively low toxicity and flammability for convenient and low‐cost storage and transportation. FA can be employed to generate electricity either in direct FA fuel cells (FCs) or indirectly as an H 2 source for hydrogen FCs. FA can enable large‐scale chemical H 2 storage to eliminate energy‐intensive and expensive processes for H 2 liquefaction and compression and thus to achieve higher efficiency and broader utilization. This perspective summarizes recent advances in catalyst development for selective dehydrogenation of FA and high‐pressure H 2 production. The advantages and limitations of FA‐to‐power options are highlighted. Existing life cycle assessment (LCA) and economic analysis studies are reviewed to discuss the feasibility and future potential of FA as a fuel.
The storage and utilization of low‐carbon electricity and decarbonization of transportation are essential components for the future energy transition into a low‐carbon economy. While hydrogen has been identified as a potential energy carrier, the lack of viable technologies for safe and efficient storage and transportation of H2 greatly limits its applications and deployment at scale. Formic acid (FA) is considered one of the promising H2 energy carriers because of its high volumetric H2 storage capacity of 53 g H2/L, and relatively low toxicity and flammability for convenient and low‐cost storage and transportation. FA can be employed to generate electricity either in direct FA fuel cells (FCs) or indirectly as an H2 source for hydrogen FCs. FA can enable large‐scale chemical H2 storage to eliminate energy‐intensive and expensive processes for H2 liquefaction and compression and thus to achieve higher efficiency and broader utilization. This perspective summarizes recent advances in catalyst development for selective dehydrogenation of FA and high‐pressure H2 production. The advantages and limitations of FA‐to‐power options are highlighted. Existing life cycle assessment (LCA) and economic analysis studies are reviewed to discuss the feasibility and future potential of FA as a fuel. The utilization of low‐carbon electricity and decarbonization of transportation are essential to a low‐carbon economy. Hydrogen has been identified as an energy carrier, but the lack of viable storage and distribution technologies greatly limits its uses. A chemical hydrogen storage system powered by formic acid can replace energy‐intensive liquefaction and compression processes for hydrogen, enabling higher efficiency and broader applications.
Author Chatterjee, Sudipta
Li, Zibiao
Low, Jonathan Sze Choong
Cheng, Hongfei
Kawanami, Hajime
Dutta, Indranil
Lai, Zhiping
Loh, Xian Jun
Huang, Kuo‐Wei
Parsapur, Rajesh Kumar
Liu, Zhaolin
Ye, Enyi
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  fullname: Dutta, Indranil
  organization: King Abdullah University of Science and Technology
– sequence: 2
  givenname: Sudipta
  surname: Chatterjee
  fullname: Chatterjee, Sudipta
  organization: King Abdullah University of Science and Technology
– sequence: 3
  givenname: Hongfei
  surname: Cheng
  fullname: Cheng, Hongfei
  organization: Institute of Materials Research and Engineering
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  givenname: Rajesh Kumar
  surname: Parsapur
  fullname: Parsapur, Rajesh Kumar
  organization: King Abdullah University of Science and Technology
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  givenname: Zhaolin
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  email: zl-liu@imre.a-star.edu.sg
  organization: Institute of Materials Research and Engineering
– sequence: 6
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  surname: Li
  fullname: Li, Zibiao
  organization: Institute of Materials Research and Engineering
– sequence: 7
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  surname: Ye
  fullname: Ye, Enyi
  organization: Institute of Materials Research and Engineering
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  givenname: Hajime
  surname: Kawanami
  fullname: Kawanami, Hajime
  email: h-kawanami@aist.go.jp
  organization: National Institute of Advanced Industrial Science and Technology
– sequence: 9
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  fullname: Low, Jonathan Sze Choong
  organization: Singapore Institute of Manufacturing Technology
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  surname: Lai
  fullname: Lai, Zhiping
  organization: King Abdullah University of Science and Technology
– sequence: 11
  givenname: Xian Jun
  surname: Loh
  fullname: Loh, Xian Jun
  email: lohxj@imre.a-star.edu.sg
  organization: Institute of Materials Research and Engineering
– sequence: 12
  givenname: Kuo‐Wei
  orcidid: 0000-0003-1900-2658
  surname: Huang
  fullname: Huang, Kuo‐Wei
  email: hkw@kaust.edu.sa
  organization: Institute of Materials Research and Engineering
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Snippet The storage and utilization of low‐carbon electricity and decarbonization of transportation are essential components for the future energy transition into a...
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SubjectTerms Carbon
Dehydrogenation
Economic analysis
Energy storage
Flammability
Formic acid
Fuel cells
high pressure gas production
hydrogen energy carrier
Hydrogen production
Hydrogen-based energy
Life cycle assessment
Liquefaction
Potential energy
Storage capacity
Toxicity
Transportation
Title Formic Acid to Power towards Low‐Carbon Economy
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Volume 12
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