A Spirobifluorene-Based Polymer of Intrinsic Microporosity with Improved Performance for Gas Separation

A highly gas‐permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer of intrinsic microporosity (PIM‐SBF) facilitates gas permeability data that lie above the 2008 Robeson upper bound, which is the universal pe...

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Published in	Advanced materials (Weinheim) Vol. 24; no. 44; pp. 5930 - 5933
Main Authors	Bezzu, C. Grazia, Carta, Mariolino, Tonkins, Alexander, Jansen, Johannes C., Bernardo, Paola, Bazzarelli, Fabio, McKeown, Neil B.
Format	Journal Article
Language	English
Published	Weinheim WILEY-VCH Verlag 20.11.2012 WILEY‐VCH Verlag
Subjects	Fluorenes - chemistry gas separation Gases - isolation & purification intrinsic microporosity Membranes, Artificial polymer membranes Polymers - chemistry Porosity Spiro Compounds - chemistry spirobifluorene Ultrafiltration - methods
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Abstract	A highly gas‐permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer of intrinsic microporosity (PIM‐SBF) facilitates gas permeability data that lie above the 2008 Robeson upper bound, which is the universal performance indicator for polymer gas separation membranes.
AbstractList	A highly gas-permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer of intrinsic microporosity (PIM-SBF) facilitates gas permeability data that lie above the 2008 Robeson upper bound, which is the universal performance indicator for polymer gas separation membranes.A highly gas-permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer of intrinsic microporosity (PIM-SBF) facilitates gas permeability data that lie above the 2008 Robeson upper bound, which is the universal performance indicator for polymer gas separation membranes. A highly gas-permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer of intrinsic microporosity (PIM-SBF) facilitates gas permeability data that lie above the 2008 Robeson upper bound, which is the universal performance indicator for polymer gas separation membranes.
Author	McKeown, Neil B. Bezzu, C. Grazia Carta, Mariolino Tonkins, Alexander Bernardo, Paola Bazzarelli, Fabio Jansen, Johannes C.
Author_xml	– sequence: 1 givenname: C. Grazia surname: Bezzu fullname: Bezzu, C. Grazia organization: School of Chemistry, Cardiff University, Cardiff, CF10 3AT, UK – sequence: 2 givenname: Mariolino surname: Carta fullname: Carta, Mariolino organization: School of Chemistry, Cardiff University, Cardiff, CF10 3AT, UK – sequence: 3 givenname: Alexander surname: Tonkins fullname: Tonkins, Alexander organization: School of Chemistry, Cardiff University, Cardiff, CF10 3AT, UK – sequence: 4 givenname: Johannes C. surname: Jansen fullname: Jansen, Johannes C. organization: Institute on Membrane Technology, ITM-CNR, c/o University of Calabria, Via P. Bucci 17/C, 87030 Rende (CS), Italy – sequence: 5 givenname: Paola surname: Bernardo fullname: Bernardo, Paola organization: Institute on Membrane Technology, ITM-CNR, c/o University of Calabria, Via P. Bucci 17/C, 87030 Rende (CS), Italy – sequence: 6 givenname: Fabio surname: Bazzarelli fullname: Bazzarelli, Fabio organization: Institute on Membrane Technology, ITM-CNR, c/o University of Calabria, Via P. Bucci 17/C, 87030 Rende (CS), Italy – sequence: 7 givenname: Neil B. surname: McKeown fullname: McKeown, Neil B. email: mckeownnb@cardiff.ac.uk organization: School of Chemistry, Cardiff University, Cardiff, CF10 3AT, UK
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/22961917$$D View this record in MEDLINE/PubMed
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Snippet	A highly gas‐permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer... A highly gas-permeable polymer with enhanced selectivities is prepared using spirobifluorene as the main structural unit. The greater rigidity of this polymer...
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StartPage	5930
SubjectTerms	Fluorenes - chemistry gas separation Gases - isolation & purification intrinsic microporosity Membranes, Artificial polymer membranes Polymers - chemistry Porosity Spiro Compounds - chemistry spirobifluorene Ultrafiltration - methods
Title	A Spirobifluorene-Based Polymer of Intrinsic Microporosity with Improved Performance for Gas Separation
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