Liquid, glass and amorphous solid states of coordination polymers and metal–organic frameworks
The field of coordination polymers and metal–organic frameworks has to date focused on the crystalline state. More than 60,000 crystalline metal–organic framework structures, formed from highly ordered arrays of metal nodes connected by organic ligands in at least one dimension, have been identified...
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| Published in | Nature reviews. Materials Vol. 3; no. 11; pp. 431 - 440 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.11.2018
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The field of coordination polymers and metal–organic frameworks has to date focused on the crystalline state. More than 60,000 crystalline metal–organic framework structures, formed from highly ordered arrays of metal nodes connected by organic ligands in at least one dimension, have been identified. However, interest in non-crystalline systems is growing, with amorphous solids, glasses and liquids identified as possessing similar metal–ligand bonding motifs to their crystalline cousins. In this Review, we provide an overview of the structural design, properties and potential applications of non-crystalline coordination polymers and metal–organic frameworks. In particular, we highlight recent reports of glasses that result from the melt quenching of the liquid states of these topical classes of materials. Finally, we provide a perspective on the future of the non-crystalline domain of coordination polymers and metal–organic frameworks.
There is increasing interest in the liquid, glass and amorphous solid states of coordination polymers and metal–organic frameworks. In this Review, we discuss the background and terminology of this emerging field, categorize example structures and provide an outlook for the future direction of the field. |
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| AbstractList | The field of coordination polymers and metal–organic frameworks has to date focused on the crystalline state. More than 60,000 crystalline metal–organic framework structures, formed from highly ordered arrays of metal nodes connected by organic ligands in at least one dimension, have been identified. However, interest in non-crystalline systems is growing, with amorphous solids, glasses and liquids identified as possessing similar metal–ligand bonding motifs to their crystalline cousins. In this Review, we provide an overview of the structural design, properties and potential applications of non-crystalline coordination polymers and metal–organic frameworks. In particular, we highlight recent reports of glasses that result from the melt quenching of the liquid states of these topical classes of materials. Finally, we provide a perspective on the future of the non-crystalline domain of coordination polymers and metal–organic frameworks. The field of coordination polymers and metal–organic frameworks has to date focused on the crystalline state. More than 60,000 crystalline metal–organic framework structures, formed from highly ordered arrays of metal nodes connected by organic ligands in at least one dimension, have been identified. However, interest in non-crystalline systems is growing, with amorphous solids, glasses and liquids identified as possessing similar metal–ligand bonding motifs to their crystalline cousins. In this Review, we provide an overview of the structural design, properties and potential applications of non-crystalline coordination polymers and metal–organic frameworks. In particular, we highlight recent reports of glasses that result from the melt quenching of the liquid states of these topical classes of materials. Finally, we provide a perspective on the future of the non-crystalline domain of coordination polymers and metal–organic frameworks. There is increasing interest in the liquid, glass and amorphous solid states of coordination polymers and metal–organic frameworks. In this Review, we discuss the background and terminology of this emerging field, categorize example structures and provide an outlook for the future direction of the field. |
| Author | Horike, Satoshi Bennett, Thomas D. |
| Author_xml | – sequence: 1 givenname: Thomas D. orcidid: 0000-0003-3717-3119 surname: Bennett fullname: Bennett, Thomas D. email: tdb35@cam.ac.uk organization: Department of Materials Science and Metallurgy, University of Cambridge – sequence: 2 givenname: Satoshi surname: Horike fullname: Horike, Satoshi email: horike@icems.kyoto-u.ac.jp organization: Institute for Integrated Cell-Material Sciences, Institute for Advanced Study, and AIST-Kyoto University Chemical Energy Materials Open Innovation Laboratory (ChEM-OIL), Kyoto University, Department of Synthetic Chemistry and Biological Chemistry, Graduate School of Engineering, Kyoto University |
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| Title | Liquid, glass and amorphous solid states of coordination polymers and metal–organic frameworks |
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