Green Ionic Liquid Lubricants Prepared from Anti-Inflammatory Drug

1-Alkyl-3-methylimidazolium ibuprofen ionic liquids (ILs, L-Ibu104, L-Ibu106 and L-Ibu108) were synthesized from an anti-inflammatory drug, sodium ibuprofen. The physicochemical and tribological properties of these ILs as neat lubricants for steel/steel and steel/copper contacts were measured. The r...

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Published in	Tribology letters Vol. 60; no. 3; pp. 1 - 11
Main Authors	Song, Zenghong, Yu, Qiangliang, Cai, Meirong, Huang, Guowei, Yao, Meihuan, Li, Dongmei, Liang, Yongmin, Fan, Mingjin, Zhou, Feng
Format	Journal Article
Language	English
Published	New York Springer US 01.12.2015 Springer Nature B.V
Subjects	Adsorption Anions Chemistry and Materials Science Copper Corrosion and Coatings Corrosion tests Friction reduction Hydrolysis Ibuprofen Ionic liquids Ions Lubricants Lubrication Materials Science Nanotechnology Nonsteroidal anti-inflammatory drugs Original Paper Photoelectrons Physical Chemistry Rubbing Stability analysis Surfaces and Interfaces Theoretical and Applied Mechanics Thin Films Tribology Ultrasonic testing Wear No corrosion Hydrolysis stable Ibuprofen Ionic liquid Lubricant
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Abstract	1-Alkyl-3-methylimidazolium ibuprofen ionic liquids (ILs, L-Ibu104, L-Ibu106 and L-Ibu108) were synthesized from an anti-inflammatory drug, sodium ibuprofen. The physicochemical and tribological properties of these ILs as neat lubricants for steel/steel and steel/copper contacts were measured. The results of hydrolysis stability evaluation and copper strip corrosion test show that these kinds of ILs are hydrolysis stable and have no corrosion to the metal contacts because of stability of anion. The friction and wear test results exhibit that these ibuprofen ILs have more effective friction-reducing and anti-wear properties than poly-alpha-olefin (PAO40) and 1-hexyl-3-methylimidazolium bis(trifluoromethylsulphonyl)imide (L-F106) at 100 °C. According to the X-ray photoelectron spectrometer analytical results, we speculated that physical adsorption films can easily formed on the metal worn surfaces during the rubbing process because of the high adsorption ability of Ibu − anion, which play an important role in the good lubricating behaviours of ibuprofen ILs. Graphical Abstract
AbstractList	1-Alkyl-3-methylimidazolium ibuprofen ionic liquids (ILs, L-Ibu104, L-Ibu106 and L-Ibu108) were synthesized from an anti-inflammatory drug, sodium ibuprofen. The physicochemical and tribological properties of these ILs as neat lubricants for steel/steel and steel/copper contacts were measured. The results of hydrolysis stability evaluation and copper strip corrosion test show that these kinds of ILs are hydrolysis stable and have no corrosion to the metal contacts because of stability of anion. The friction and wear test results exhibit that these ibuprofen ILs have more effective friction-reducing and anti-wear properties than poly-alpha-olefin (PAO40) and 1-hexyl-3-methylimidazolium bis(trifluoromethylsulphonyl)imide (L-F106) at 100 °C. According to the X-ray photoelectron spectrometer analytical results, we speculated that physical adsorption films can easily formed on the metal worn surfaces during the rubbing process because of the high adsorption ability of Ibu − anion, which play an important role in the good lubricating behaviours of ibuprofen ILs. Graphical Abstract 1-Alkyl-3-methylimidazolium ibuprofen ionic liquids (ILs, L-Ibu104, L-Ibu106 and L-Ibu108) were synthesized from an anti-inflammatory drug, sodium ibuprofen. The physicochemical and tribological properties of these ILs as neat lubricants for steel/steel and steel/copper contacts were measured. The results of hydrolysis stability evaluation and copper strip corrosion test show that these kinds of ILs are hydrolysis stable and have no corrosion to the metal contacts because of stability of anion. The friction and wear test results exhibit that these ibuprofen ILs have more effective friction-reducing and anti-wear properties than poly-alpha-olefin (PAO40) and 1-hexyl-3-methylimidazolium bis(trifluoromethylsulphonyl)imide (L-F106) at 100 °C. According to the X-ray photoelectron spectrometer analytical results, we speculated that physical adsorption films can easily formed on the metal worn surfaces during the rubbing process because of the high adsorption ability of Ibu− anion, which play an important role in the good lubricating behaviours of ibuprofen ILs.Graphical Abstract
ArticleNumber	38
Author	Liang, Yongmin Li, Dongmei Song, Zenghong Zhou, Feng Yu, Qiangliang Huang, Guowei Cai, Meirong Yao, Meihuan Fan, Mingjin
Author_xml	– sequence: 1 givenname: Zenghong surname: Song fullname: Song, Zenghong organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, University of Chinese Academy of Sciences – sequence: 2 givenname: Qiangliang surname: Yu fullname: Yu, Qiangliang organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, University of Chinese Academy of Sciences – sequence: 3 givenname: Meirong surname: Cai fullname: Cai, Meirong organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences – sequence: 4 givenname: Guowei surname: Huang fullname: Huang, Guowei organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, University of Chinese Academy of Sciences – sequence: 5 givenname: Meihuan surname: Yao fullname: Yao, Meihuan organization: Henan Normal University – sequence: 6 givenname: Dongmei surname: Li fullname: Li, Dongmei email: dmli@licp.cas.cn organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences – sequence: 7 givenname: Yongmin surname: Liang fullname: Liang, Yongmin organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences – sequence: 8 givenname: Mingjin surname: Fan fullname: Fan, Mingjin email: fanmingjin@licp.cas.cn organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences – sequence: 9 givenname: Feng surname: Zhou fullname: Zhou, Feng email: zhouf@lzb.ac.cn organization: State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences
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Snippet	1-Alkyl-3-methylimidazolium ibuprofen ionic liquids (ILs, L-Ibu104, L-Ibu106 and L-Ibu108) were synthesized from an anti-inflammatory drug, sodium ibuprofen....
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SubjectTerms	Adsorption Anions Chemistry and Materials Science Copper Corrosion and Coatings Corrosion tests Friction reduction Hydrolysis Ibuprofen Ionic liquids Ions Lubricants Lubrication Materials Science Nanotechnology Nonsteroidal anti-inflammatory drugs Original Paper Photoelectrons Physical Chemistry Rubbing Stability analysis Surfaces and Interfaces Theoretical and Applied Mechanics Thin Films Tribology Ultrasonic testing Wear
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Title	Green Ionic Liquid Lubricants Prepared from Anti-Inflammatory Drug
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