The influence of chromium substitution on an iron–titanium catalyst used in the selective catalytic reduction of NO
The selective catalytic reduction (SCR) of NO by NH3 over chromium-substituted Fe titanate catalysts with different amounts of chromium has been studied. The experiments revealed that the amount of chromium in the catalyst is a crucial factor for high activity. Fe0.5Cr0.5TiOx showed the highest acti...
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| Published in | Journal of catalysis Vol. 292; pp. 32 - 43 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier Inc
01.08.2012
Elsevier Elsevier BV |
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| Abstract | The selective catalytic reduction (SCR) of NO by NH3 over chromium-substituted Fe titanate catalysts with different amounts of chromium has been studied. The experiments revealed that the amount of chromium in the catalyst is a crucial factor for high activity. Fe0.5Cr0.5TiOx showed the highest activity.
A series of Cr-substituted Fe–Ti compounds were prepared by the co-precipitation method and were systematically investigated as catalysts for the selective catalytic reduction (SCR) of NO by NH3. A variety of analytical techniques revealed that the Cr substitution amount affects the N2 selectivity, SCR activity, redox behavior of NH3/NOx, adsorption ability, and structure of catalysts in terms of surface properties, porosity, mobility of lattice oxygen, oxidative ability of Cr species, ratio of Brønsted acid sites and Lewis acid sites, NOx adsorption capacity, and structural disorder and distortion. In a series of FeaCr1−aTiOx (a=1, 0.75, 0.5, 0.2, 0) catalysts, Fe0.5Cr0.5TiOx showed the highest activity because of the optimized interactions of Fe, Cr, and Ti species in this catalyst. |
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| AbstractList | The selective catalytic reduction (SCR) of NO by NH3 over chromium-substituted Fe titanate catalysts with different amounts of chromium has been studied. The experiments revealed that the amount of chromium in the catalyst is a crucial factor for high activity. Fe0.5Cr0.5TiOx showed the highest activity.
A series of Cr-substituted Fe–Ti compounds were prepared by the co-precipitation method and were systematically investigated as catalysts for the selective catalytic reduction (SCR) of NO by NH3. A variety of analytical techniques revealed that the Cr substitution amount affects the N2 selectivity, SCR activity, redox behavior of NH3/NOx, adsorption ability, and structure of catalysts in terms of surface properties, porosity, mobility of lattice oxygen, oxidative ability of Cr species, ratio of Brønsted acid sites and Lewis acid sites, NOx adsorption capacity, and structural disorder and distortion. In a series of FeaCr1−aTiOx (a=1, 0.75, 0.5, 0.2, 0) catalysts, Fe0.5Cr0.5TiOx showed the highest activity because of the optimized interactions of Fe, Cr, and Ti species in this catalyst. A series of Cr-substituted Fe–Ti compounds were prepared by the co-precipitation method and were systematically investigated as catalysts for the selective catalytic reduction (SCR) of NO by NH₃. A variety of analytical techniques revealed that the Cr substitution amount affects the N₂ selectivity, SCR activity, redox behavior of NH₃/NOₓ, adsorption ability, and structure of catalysts in terms of surface properties, porosity, mobility of lattice oxygen, oxidative ability of Cr species, ratio of Brønsted acid sites and Lewis acid sites, NOₓ adsorption capacity, and structural disorder and distortion. In a series of FeₐCr₁₋ ₐTiOₓ (a=1, 0.75, 0.5, 0.2, 0) catalysts, Fe₀.₅Cr₀.₅TiOₓ showed the highest activity because of the optimized interactions of Fe, Cr, and Ti species in this catalyst. The selective catalytic reduction (SCR) of NO by NH3 over chromium-substituted Fe titanate catalysts with different amounts of chromium has been studied. The experiments revealed that the amount of chromium in the catalyst is a crucial factor for high activity. Fe0.5 Cr0.5 TiO x showed the highest activity. A series of Cr-substituted Fe-Ti compounds were prepared by the co-precipitation method and were systematically investigated as catalysts for the selective catalytic reduction (SCR) of NO by NH3 . A variety of analytical techniques revealed that the Cr substitution amount affects the N2 selectivity, SCR activity, redox behavior of NH3 /NO x , adsorption ability, and structure of catalysts in terms of surface properties, porosity, mobility of lattice oxygen, oxidative ability of Cr species, ratio of Brønsted acid sites and Lewis acid sites, NO x adsorption capacity, and structural disorder and distortion. In a series of Fe a Cr1- a TiO x (a =1, 0.75, 0.5, 0.2, 0) catalysts, Fe0.5 Cr0.5 TiO x showed the highest activity because of the optimized interactions of Fe, Cr, and Ti species in this catalyst. [PUBLICATION ABSTRACT] |
| Author | Karami, Asghar Salehi, Vajiheh |
| Author_xml | – sequence: 1 givenname: Asghar surname: Karami fullname: Karami, Asghar email: asghar54@jdsharif.ac.ir organization: Department of Chemical Engineering, Amirkabir University of Technology (Tehran Polytechnic), 424 Hafez Ave., Tehran, Iran – sequence: 2 givenname: Vajiheh surname: Salehi fullname: Salehi, Vajiheh organization: Department of Chemistry, Sharif University of Technology, Azadi Ave., Tehran, Iran |
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| Copyright | 2012 Elsevier Inc. 2015 INIST-CNRS Copyright © 2012 Elsevier B.V. All rights reserved. |
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| Keywords | Cr substitution Redox behavior NOx adsorption Selective catalytic reduction NO Acidic site Adsorption capacity Mobility Distortion Iron Selectivity Chemical reduction Precipitation Brönsted acid Substitution Surface properties Adsorption structure Titanium Oxidation Lewis acid Nitrogen oxide Oxygen Catalytic reaction Lewis site Transition metal Bronsted site Ammonia Heterogeneous catalysis Adsorption Chromium Porosity Catalyst |
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| Snippet | The selective catalytic reduction (SCR) of NO by NH3 over chromium-substituted Fe titanate catalysts with different amounts of chromium has been studied. The... A series of Cr-substituted Fe–Ti compounds were prepared by the co-precipitation method and were systematically investigated as catalysts for the selective... |
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| SubjectTerms | adsorption ammonia analytical methods Catalysis Catalysts Chemistry Chromium Colloidal state and disperse state coprecipitation Cr substitution Exact sciences and technology General and physical chemistry Iron Lewis acids nitric oxide nitrogen NOx adsorption oxygen porosity Porous materials Redox behavior Selective catalytic reduction Surface physical chemistry Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry Titanium |
| Title | The influence of chromium substitution on an iron–titanium catalyst used in the selective catalytic reduction of NO |
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