Synthesis and Electrochemical Properties of Two-Dimensional RGO/Ti3C2Tx Nanocomposites
MXene is a new type of two-dimensional layered material. Herein, a GO/Ti3C2Tx nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti3C2Tx was transformed into RGO/Ti3C2Tx under high temperature with Ar/H2. The prepared samples were characterized using X-ray diffraction (X...
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| Published in | Nanomaterials (Basel, Switzerland) Vol. 8; no. 2; p. 80 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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31.01.2018
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| Abstract | MXene is a new type of two-dimensional layered material. Herein, a GO/Ti3C2Tx nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti3C2Tx was transformed into RGO/Ti3C2Tx under high temperature with Ar/H2. The prepared samples were characterized using X-ray diffraction (XRD), Raman measurement, scanning electron microscopy (SEM), energy disperse spectroscopy (EDS), and X-ray photoelectron spectroscopy (XPS). As an electrode material in lithium-ion batteries, the RGO/Ti3C2Tx nanocomposite exhibited an excellent electrochemical performance and an excellent rate performance. Compared to pure Ti3C2Tx, the nanocomposite had a better reversible capacity at different current densities and had no attenuation after 200 cycles, which is one time higher than pure Ti3C2Tx. The improvement in the specific capacity was due to the excellent electrical conductivity and the unique structure of RGO, in which a charge transfer bridge was built among the Ti3C2Tx flakes. Such a bridge shortened the transmission distance of the electrons and ions and effectively controlled the restacking of the laminated materials. |
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| AbstractList | MXene is a new type of two-dimensional layered material. Herein, a GO/Ti₃C₂Tx nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti₃C₂Tx was transformed into RGO/Ti₃C₂Tx under high temperature with Ar/H2. The prepared samples were characterized using X-ray diffraction (XRD), Raman measurement, scanning electron microscopy (SEM), energy disperse spectroscopy (EDS), and X-ray photoelectron spectroscopy (XPS). As an electrode material in lithium-ion batteries, the RGO/Ti₃C₂Tx nanocomposite exhibited an excellent electrochemical performance and an excellent rate performance. Compared to pure Ti₃C₂Tx, the nanocomposite had a better reversible capacity at different current densities and had no attenuation after 200 cycles, which is one time higher than pure Ti₃C₂Tx. The improvement in the specific capacity was due to the excellent electrical conductivity and the unique structure of RGO, in which a charge transfer bridge was built among the Ti₃C₂Tx flakes. Such a bridge shortened the transmission distance of the electrons and ions and effectively controlled the restacking of the laminated materials.MXene is a new type of two-dimensional layered material. Herein, a GO/Ti₃C₂Tx nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti₃C₂Tx was transformed into RGO/Ti₃C₂Tx under high temperature with Ar/H2. The prepared samples were characterized using X-ray diffraction (XRD), Raman measurement, scanning electron microscopy (SEM), energy disperse spectroscopy (EDS), and X-ray photoelectron spectroscopy (XPS). As an electrode material in lithium-ion batteries, the RGO/Ti₃C₂Tx nanocomposite exhibited an excellent electrochemical performance and an excellent rate performance. Compared to pure Ti₃C₂Tx, the nanocomposite had a better reversible capacity at different current densities and had no attenuation after 200 cycles, which is one time higher than pure Ti₃C₂Tx. The improvement in the specific capacity was due to the excellent electrical conductivity and the unique structure of RGO, in which a charge transfer bridge was built among the Ti₃C₂Tx flakes. Such a bridge shortened the transmission distance of the electrons and ions and effectively controlled the restacking of the laminated materials. MXene is a new type of two-dimensional layered material. Herein, a GO/Ti3C2Tx nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti3C2Tx was transformed into RGO/Ti3C2Tx under high temperature with Ar/H2. The prepared samples were characterized using X-ray diffraction (XRD), Raman measurement, scanning electron microscopy (SEM), energy disperse spectroscopy (EDS), and X-ray photoelectron spectroscopy (XPS). As an electrode material in lithium-ion batteries, the RGO/Ti3C2Tx nanocomposite exhibited an excellent electrochemical performance and an excellent rate performance. Compared to pure Ti3C2Tx, the nanocomposite had a better reversible capacity at different current densities and had no attenuation after 200 cycles, which is one time higher than pure Ti3C2Tx. The improvement in the specific capacity was due to the excellent electrical conductivity and the unique structure of RGO, in which a charge transfer bridge was built among the Ti3C2Tx flakes. Such a bridge shortened the transmission distance of the electrons and ions and effectively controlled the restacking of the laminated materials. MXene is a new type of two-dimensional layered material. Herein, a GO/Ti 3 C 2 T x nanocomposite was prepared by a simple liquid phase method, and the obtained GO/Ti 3 C 2 T x was transformed into RGO/Ti 3 C 2 T x under high temperature with Ar/H 2. The prepared samples were characterized using X-ray diffraction (XRD), Raman measurement, scanning electron microscopy (SEM), energy disperse spectroscopy (EDS), and X-ray photoelectron spectroscopy (XPS). As an electrode material in lithium-ion batteries, the RGO/Ti 3 C 2 T x nanocomposite exhibited an excellent electrochemical performance and an excellent rate performance. Compared to pure Ti 3 C 2 T x , the nanocomposite had a better reversible capacity at different current densities and had no attenuation after 200 cycles, which is one time higher than pure Ti 3 C 2 T x . The improvement in the specific capacity was due to the excellent electrical conductivity and the unique structure of RGO, in which a charge transfer bridge was built among the Ti 3 C 2 T x flakes. Such a bridge shortened the transmission distance of the electrons and ions and effectively controlled the restacking of the laminated materials. |
| Author | Wang, Libo Wang, Bo Wang, Xiaolong Qin, Gang Shen, Changjie Zhou, Aiguo Hu, Qianku Lian, Weiwei Liu, Xuqing |
| AuthorAffiliation | 2 State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China; bowang@licp.cas.cn 3 School of Materials, University of Manchester, Oxford Road, Manchester M13 9PL, UK; xuqing.liu@manchester.ac.uk 1 School of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, Henan, China; shenchangjie92@163.com (C.S.); zhouag@hpu.edu.cn (A.Z.); wangxiaolong@163.com (X.W.); WWL2116060@163.com (W.L.); hqk@hpu.edu.cn (Q.H.); clqingang@126.com (G.Q.) |
| AuthorAffiliation_xml | – name: 1 School of Materials Science and Engineering, Henan Polytechnic University, Jiaozuo 454000, Henan, China; shenchangjie92@163.com (C.S.); zhouag@hpu.edu.cn (A.Z.); wangxiaolong@163.com (X.W.); WWL2116060@163.com (W.L.); hqk@hpu.edu.cn (Q.H.); clqingang@126.com (G.Q.) – name: 3 School of Materials, University of Manchester, Oxford Road, Manchester M13 9PL, UK; xuqing.liu@manchester.ac.uk – name: 2 State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China; bowang@licp.cas.cn |
| Author_xml | – sequence: 1 givenname: Changjie surname: Shen fullname: Shen, Changjie – sequence: 2 givenname: Libo orcidid: 0000-0002-5858-397X surname: Wang fullname: Wang, Libo – sequence: 3 givenname: Aiguo surname: Zhou fullname: Zhou, Aiguo – sequence: 4 givenname: Bo surname: Wang fullname: Wang, Bo – sequence: 5 givenname: Xiaolong surname: Wang fullname: Wang, Xiaolong – sequence: 6 givenname: Weiwei surname: Lian fullname: Lian, Weiwei – sequence: 7 givenname: Qianku surname: Hu fullname: Hu, Qianku – sequence: 8 givenname: Gang surname: Qin fullname: Qin, Gang – sequence: 9 givenname: Xuqing orcidid: 0000-0001-5998-6546 surname: Liu fullname: Liu, Xuqing |
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| Snippet | MXene is a new type of two-dimensional layered material. Herein, a GO/Ti3C2Tx nanocomposite was prepared by a simple liquid phase method, and the obtained... MXene is a new type of two-dimensional layered material. Herein, a GO/Ti₃C₂Tx nanocomposite was prepared by a simple liquid phase method, and the obtained... MXene is a new type of two-dimensional layered material. Herein, a GO/Ti 3 C 2 T x nanocomposite was prepared by a simple liquid phase method, and the obtained... |
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| SubjectTerms | Batteries Charge transfer Electric bridges Electrical conductivity Electrical resistivity Electrochemical analysis Electrochemistry Electrode materials Electron microscopy Energy measurement exfoliation Flakes graphene High temperature Lithium Lithium-ion batteries lithium-ion battery Movable bridges MXene nanocomposite Nanocomposites Photoelectron spectroscopy Rechargeable batteries Scanning electron microscopy Specific capacity Spectroscopy Spectrum analysis X ray photoelectron spectroscopy X-ray diffraction X-rays |
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| Title | Synthesis and Electrochemical Properties of Two-Dimensional RGO/Ti3C2Tx Nanocomposites |
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