Research on the sustainable efficacy of g-MoS2 decorated biochar nanocomposites for removing tetracycline hydrochloride from antibiotic-polluted aqueous solution
Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach with potential efficiency, sustainability and eco-friendliness to remove antibiotic pollutants. A novel biochar-based nanomaterial was synthesiz...
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| Published in | The Science of the total environment Vol. 648; pp. 206 - 217 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.01.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach with potential efficiency, sustainability and eco-friendliness to remove antibiotic pollutants. A novel biochar-based nanomaterial was synthesized by hydrothermal synthesis and was investigated for its removal potential for tetracycline hydrochloride (TC) from both artificial and real wastewater. The associative facilitation between biochar and g-MoS2 nanosheets was proposed, revealing the favorable surface structures and adsorption properties of the composite. The related adsorption kinetics, isotherms and thermodynamics were studied by several models with adsorption experimental data, turning out that biochar decorated by g-MoS2 exhibited optimum TC removal with adsorption capacity up to 249.45 mg/g at 298 K. The adsorption behavior of TC molecules on g-MoS2-BC can be interpreted well by three-step process, and it is dominated by several mechanisms containing pore-filling, electrostatic force, hydrogen bond and π-π interaction. In addition, the cost-effective g-MoS2-BC nanocomposites demonstrated excellent adsorption and recycling performance in TC-contaminated river water, which might provide the underlying insights needed to guide the design of promising approach for contaminant removal on a large scale in practical application.
[Display omitted]
•Hierarchical g-MoS2 nanosheets were successfully loaded onto the surface of biochar.•Pore structures and surface properties of biochar were improved by decorated with g-MoS2.•Sustainable efficient removal for TC by novel g-MoS2-biochar nanocomposite was confirmed.•Several mechanisms participated in the antibiotic removal were also discussed.•Further research focuses on the catalytic degradation ability of nanocomposite for its regeneration. |
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| AbstractList | Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach with potential efficiency, sustainability and eco-friendliness to remove antibiotic pollutants. A novel biochar-based nanomaterial was synthesized by hydrothermal synthesis and was investigated for its removal potential for tetracycline hydrochloride (TC) from both artificial and real wastewater. The associative facilitation between biochar and g-MoS2 nanosheets was proposed, revealing the favorable surface structures and adsorption properties of the composite. The related adsorption kinetics, isotherms and thermodynamics were studied by several models with adsorption experimental data, turning out that biochar decorated by g-MoS2 exhibited optimum TC removal with adsorption capacity up to 249.45 mg/g at 298 K. The adsorption behavior of TC molecules on g-MoS2-BC can be interpreted well by three-step process, and it is dominated by several mechanisms containing pore-filling, electrostatic force, hydrogen bond and π-π interaction. In addition, the cost-effective g-MoS2-BC nanocomposites demonstrated excellent adsorption and recycling performance in TC-contaminated river water, which might provide the underlying insights needed to guide the design of promising approach for contaminant removal on a large scale in practical application.Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach with potential efficiency, sustainability and eco-friendliness to remove antibiotic pollutants. A novel biochar-based nanomaterial was synthesized by hydrothermal synthesis and was investigated for its removal potential for tetracycline hydrochloride (TC) from both artificial and real wastewater. The associative facilitation between biochar and g-MoS2 nanosheets was proposed, revealing the favorable surface structures and adsorption properties of the composite. The related adsorption kinetics, isotherms and thermodynamics were studied by several models with adsorption experimental data, turning out that biochar decorated by g-MoS2 exhibited optimum TC removal with adsorption capacity up to 249.45 mg/g at 298 K. The adsorption behavior of TC molecules on g-MoS2-BC can be interpreted well by three-step process, and it is dominated by several mechanisms containing pore-filling, electrostatic force, hydrogen bond and π-π interaction. In addition, the cost-effective g-MoS2-BC nanocomposites demonstrated excellent adsorption and recycling performance in TC-contaminated river water, which might provide the underlying insights needed to guide the design of promising approach for contaminant removal on a large scale in practical application. Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach with potential efficiency, sustainability and eco-friendliness to remove antibiotic pollutants. A novel biochar-based nanomaterial was synthesized by hydrothermal synthesis and was investigated for its removal potential for tetracycline hydrochloride (TC) from both artificial and real wastewater. The associative facilitation between biochar and g-MoS2 nanosheets was proposed, revealing the favorable surface structures and adsorption properties of the composite. The related adsorption kinetics, isotherms and thermodynamics were studied by several models with adsorption experimental data, turning out that biochar decorated by g-MoS2 exhibited optimum TC removal with adsorption capacity up to 249.45 mg/g at 298 K. The adsorption behavior of TC molecules on g-MoS2-BC can be interpreted well by three-step process, and it is dominated by several mechanisms containing pore-filling, electrostatic force, hydrogen bond and π-π interaction. In addition, the cost-effective g-MoS2-BC nanocomposites demonstrated excellent adsorption and recycling performance in TC-contaminated river water, which might provide the underlying insights needed to guide the design of promising approach for contaminant removal on a large scale in practical application. [Display omitted] •Hierarchical g-MoS2 nanosheets were successfully loaded onto the surface of biochar.•Pore structures and surface properties of biochar were improved by decorated with g-MoS2.•Sustainable efficient removal for TC by novel g-MoS2-biochar nanocomposite was confirmed.•Several mechanisms participated in the antibiotic removal were also discussed.•Further research focuses on the catalytic degradation ability of nanocomposite for its regeneration. Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach with potential efficiency, sustainability and eco-friendliness to remove antibiotic pollutants. A novel biochar-based nanomaterial was synthesized by hydrothermal synthesis and was investigated for its removal potential for tetracycline hydrochloride (TC) from both artificial and real wastewater. The associative facilitation between biochar and g-MoS₂ nanosheets was proposed, revealing the favorable surface structures and adsorption properties of the composite. The related adsorption kinetics, isotherms and thermodynamics were studied by several models with adsorption experimental data, turning out that biochar decorated by g-MoS₂ exhibited optimum TC removal with adsorption capacity up to 249.45 mg/g at 298 K. The adsorption behavior of TC molecules on g-MoS₂-BC can be interpreted well by three-step process, and it is dominated by several mechanisms containing pore-filling, electrostatic force, hydrogen bond and π-π interaction. In addition, the cost-effective g-MoS₂-BC nanocomposites demonstrated excellent adsorption and recycling performance in TC-contaminated river water, which might provide the underlying insights needed to guide the design of promising approach for contaminant removal on a large scale in practical application. |
| Author | Zeng, Guangming Fang, Yilong Yu, Jiangfang Zeng, Zhuotong Wu, Haipeng Liang, Jie Song, Biao Zhang, Chang Ye, Shujing Xiao, Rong |
| Author_xml | – sequence: 1 givenname: Zhuotong surname: Zeng fullname: Zeng, Zhuotong organization: Department of Dermatology, Second Xiangya Hospital, Central South University, Changsha 410011, PR China – sequence: 2 givenname: Shujing surname: Ye fullname: Ye, Shujing organization: College of Environmental Science and Engineering, Hunan University, Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 3 givenname: Haipeng surname: Wu fullname: Wu, Haipeng organization: Department of Dermatology, Second Xiangya Hospital, Central South University, Changsha 410011, PR China – sequence: 4 givenname: Rong surname: Xiao fullname: Xiao, Rong email: xiaorong65@csu.edu.cn organization: Department of Dermatology, Second Xiangya Hospital, Central South University, Changsha 410011, PR China – sequence: 5 givenname: Guangming orcidid: 0000-0002-4230-7647 surname: Zeng fullname: Zeng, Guangming email: zgming@hnu.edu.cn organization: Department of Dermatology, Second Xiangya Hospital, Central South University, Changsha 410011, PR China – sequence: 6 givenname: Jie surname: Liang fullname: Liang, Jie organization: College of Environmental Science and Engineering, Hunan University, Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 7 givenname: Chang surname: Zhang fullname: Zhang, Chang organization: College of Environmental Science and Engineering, Hunan University, Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 8 givenname: Jiangfang surname: Yu fullname: Yu, Jiangfang organization: College of Environmental Science and Engineering, Hunan University, Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 9 givenname: Yilong surname: Fang fullname: Fang, Yilong organization: College of Environmental Science and Engineering, Hunan University, Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China – sequence: 10 givenname: Biao surname: Song fullname: Song, Biao organization: College of Environmental Science and Engineering, Hunan University, Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha 410082, PR China |
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| Snippet | Antibiotic concentrations in surface waters far exceed the pollution limit due to the abuse of pharmaceuticals, resulting in an urgent need for an approach... |
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| SubjectTerms | adsorption aqueous solutions biochar Biochar-based nanocomposite cost effectiveness drugs electrostatic interactions g-MoS2 hydrogen bonding nanocomposites nanosheets pollutants pollution pollution control Removal mechanisms river water surface water Sustainable application tetracycline Tetracycline hydrochloride thermodynamics wastewater |
| Title | Research on the sustainable efficacy of g-MoS2 decorated biochar nanocomposites for removing tetracycline hydrochloride from antibiotic-polluted aqueous solution |
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