Cross-dehydrogenative coupling: a sustainable reaction for C-C bond formations

We are entering an era that emphasizes greenness and sustainability. Based on such a philosophy, it is critical to uncover novel and original sustainable reaction modes for future green chemical syntheses. The cross-dehydrogenative coupling (CDC) reaction has thus been widely developed as one of the...

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Published inGreen chemistry : an international journal and green chemistry resource : GC Vol. 23; no. 18; pp. 6789 - 6862
Main Authors Tian, Tian, Li, Zhiping, Li, Chao-Jun
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 20.09.2021
Subjects
Alternative energy sources
Chemical reactions
Continuous flow
Coupling
Covalent bonds
Dehydrogenation
Electrochemistry
Green chemistry
philosophy
Quantum dots
Sustainability
Thermal energy
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Abstract We are entering an era that emphasizes greenness and sustainability. Based on such a philosophy, it is critical to uncover novel and original sustainable reaction modes for future green chemical syntheses. The cross-dehydrogenative coupling (CDC) reaction has thus been widely developed as one of the most sustainable and efficient synthesis strategies for constructing C-C bonds. This review summarizes the development of this field over the past 20 years, with a discussion on future trends and directions: from the original reaction model at the beginning and its development in the first decade, to extensive research in the second decade. The latest development sees the emergence of alternative forms of energy inputs (photoredox, mechano, microwave, electrochemical, continuous-flow and solar quantum dots) to facilitate CDC reactions, gradually replacing the classical form of thermal energy, which will inspire broader applications and innovations in the future. We provide a review of the progress of cross-dehydrogenative coupling reactions in constructing a wide variety of C-C bonds. Sustainable cross-dehydrogenative coupling reactions can be combined with multiple forms of energy output.
AbstractList We are entering an era that emphasizes greenness and sustainability. Based on such a philosophy, it is critical to uncover novel and original sustainable reaction modes for future green chemical syntheses. The cross-dehydrogenative coupling (CDC) reaction has thus been widely developed as one of the most sustainable and efficient synthesis strategies for constructing C–C bonds. This review summarizes the development of this field over the past 20 years, with a discussion on future trends and directions: from the original reaction model at the beginning and its development in the first decade, to extensive research in the second decade. The latest development sees the emergence of alternative forms of energy inputs (photoredox, mechano, microwave, electrochemical, continuous-flow and solar quantum dots) to facilitate CDC reactions, gradually replacing the classical form of thermal energy, which will inspire broader applications and innovations in the future.
We are entering an era that emphasizes greenness and sustainability. Based on such a philosophy, it is critical to uncover novel and original sustainable reaction modes for future green chemical syntheses. The cross-dehydrogenative coupling (CDC) reaction has thus been widely developed as one of the most sustainable and efficient synthesis strategies for constructing C-C bonds. This review summarizes the development of this field over the past 20 years, with a discussion on future trends and directions: from the original reaction model at the beginning and its development in the first decade, to extensive research in the second decade. The latest development sees the emergence of alternative forms of energy inputs (photoredox, mechano, microwave, electrochemical, continuous-flow and solar quantum dots) to facilitate CDC reactions, gradually replacing the classical form of thermal energy, which will inspire broader applications and innovations in the future. We provide a review of the progress of cross-dehydrogenative coupling reactions in constructing a wide variety of C-C bonds. Sustainable cross-dehydrogenative coupling reactions can be combined with multiple forms of energy output.
Author Li, Chao-Jun
Tian, Tian
Li, Zhiping
AuthorAffiliation Department of Chemistry
McGill University
Renmin University of China
Department of Chemistry and FQRNT Center for Green Chemistry and Catalysis
AuthorAffiliation_xml – name: Department of Chemistry
– name: McGill University
– name: Department of Chemistry and FQRNT Center for Green Chemistry and Catalysis
– name: Renmin University of China
Author_xml – sequence: 1
  givenname: Tian
  surname: Tian
  fullname: Tian, Tian
– sequence: 2
  givenname: Zhiping
  surname: Li
  fullname: Li, Zhiping
– sequence: 3
  givenname: Chao-Jun
  surname: Li
  fullname: Li, Chao-Jun
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Snippet We are entering an era that emphasizes greenness and sustainability. Based on such a philosophy, it is critical to uncover novel and original sustainable...
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SubjectTerms Alternative energy sources
Chemical reactions
Continuous flow
Coupling
Covalent bonds
Dehydrogenation
Electrochemistry
Green chemistry
philosophy
Quantum dots
Sustainability
Thermal energy
Title Cross-dehydrogenative coupling: a sustainable reaction for C-C bond formations
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