Electrospun metal-organic framework based nanofibers for energy storage and environmental applications: current approaches and challenges

In recent years, a great deal of investigation has been performed based on the study of metal-organic frameworks (MOFs) combined with other materials, in order to overcome the tremendous challenge encountered by single MOFs in practical applications. Among them are MOF based composite nanofibers pre...

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Published inJournal of materials chemistry. A, Materials for energy and sustainability Vol. 1; no. 4; pp. 1642 - 1681
Main Authors Li, Xiangye, Zhou, Ruifeng, Wang, Zhenzhen, Zhang, Minghui, He, Tieshi
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 25.01.2022
Subjects
chemistry
coordination polymers
Electrospinning
energy
Energy conservation
Energy storage
Environmental protection
Fabrication
Functional materials
Metal-organic frameworks
Nanofibers
natural resources conservation
Porous materials
Online AccessGet full text
ISSN2050-7488
2050-7496
2050-7496
DOI10.1039/d1ta08413e

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Abstract In recent years, a great deal of investigation has been performed based on the study of metal-organic frameworks (MOFs) combined with other materials, in order to overcome the tremendous challenge encountered by single MOFs in practical applications. Among them are MOF based composite nanofibers prepared via electrospinning with the advantages of inorganic porous materials and polymeric nanofibers, which have witnessed intensive development and extensive applications in energy storage and environment conservation fields. Beyond that, preparing MOF based composite nanofibers is also considered to be an effective route to broaden the practical application of MOFs. Herein, a comprehensive review of the recent developments of MOF based composite nanofibers prepared via the electrospinning process, serving as functional materials, is provided. From the perspective of fabrication, the major routes reported so far for fabricating MOF based composite nanofibers are first systematically discussed. Furthermore, the fundamental applications of MOF based composite nanofibers in energy storage and environmental protection are introduced in detail. Finally, a series of critical challenges in the above research area, and some directions for future research are put forward. Schematic illustration of the morphology, structure and preparation route of MOF based nanofiber composites and their applications (LLA stands for layer-by-layer assembly; ALD stands for atomic layer deposition).
AbstractList In recent years, a great deal of investigation has been performed based on the study of metal-organic frameworks (MOFs) combined with other materials, in order to overcome the tremendous challenge encountered by single MOFs in practical applications. Among them are MOF based composite nanofibers prepared via electrospinning with the advantages of inorganic porous materials and polymeric nanofibers, which have witnessed intensive development and extensive applications in energy storage and environment conservation fields. Beyond that, preparing MOF based composite nanofibers is also considered to be an effective route to broaden the practical application of MOFs. Herein, a comprehensive review of the recent developments of MOF based composite nanofibers prepared via the electrospinning process, serving as functional materials, is provided. From the perspective of fabrication, the major routes reported so far for fabricating MOF based composite nanofibers are first systematically discussed. Furthermore, the fundamental applications of MOF based composite nanofibers in energy storage and environmental protection are introduced in detail. Finally, a series of critical challenges in the above research area, and some directions for future research are put forward. Schematic illustration of the morphology, structure and preparation route of MOF based nanofiber composites and their applications (LLA stands for layer-by-layer assembly; ALD stands for atomic layer deposition).
In recent years, a great deal of investigation has been performed based on the study of metal–organic frameworks (MOFs) combined with other materials, in order to overcome the tremendous challenge encountered by single MOFs in practical applications. Among them are MOF based composite nanofibers prepared via electrospinning with the advantages of inorganic porous materials and polymeric nanofibers, which have witnessed intensive development and extensive applications in energy storage and environment conservation fields. Beyond that, preparing MOF based composite nanofibers is also considered to be an effective route to broaden the practical application of MOFs. Herein, a comprehensive review of the recent developments of MOF based composite nanofibers prepared via the electrospinning process, serving as functional materials, is provided. From the perspective of fabrication, the major routes reported so far for fabricating MOF based composite nanofibers are first systematically discussed. Furthermore, the fundamental applications of MOF based composite nanofibers in energy storage and environmental protection are introduced in detail. Finally, a series of critical challenges in the above research area, and some directions for future research are put forward.
In recent years, a great deal of investigation has been performed based on the study of metal–organic frameworks (MOFs) combined with other materials, in order to overcome the tremendous challenge encountered by single MOFs in practical applications. Among them are MOF based composite nanofibers prepared via electrospinning with the advantages of inorganic porous materials and polymeric nanofibers, which have witnessed intensive development and extensive applications in energy storage and environment conservation fields. Beyond that, preparing MOF based composite nanofibers is also considered to be an effective route to broaden the practical application of MOFs. Herein, a comprehensive review of the recent developments of MOF based composite nanofibers prepared via the electrospinning process, serving as functional materials, is provided. From the perspective of fabrication, the major routes reported so far for fabricating MOF based composite nanofibers are first systematically discussed. Furthermore, the fundamental applications of MOF based composite nanofibers in energy storage and environmental protection are introduced in detail. Finally, a series of critical challenges in the above research area, and some directions for future research are put forward.
Author Wang, Zhenzhen
He, Tieshi
Li, Xiangye
Zhou, Ruifeng
Zhang, Minghui
AuthorAffiliation Bohai University
Liaoning Engineering Technology Center of Supercapacitor
Lanzhou University of Technology
College of Chemistry & Materials Engineering
School of Material Science and Engineering
AuthorAffiliation_xml – name: College of Chemistry & Materials Engineering
– name: Bohai University
– name: School of Material Science and Engineering
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Notes Minghui Zhang received her B.S. degrees from Bohai University. She is presently pursuing her master's degree at the School of Chemistry & Materials Engineering, Bohai University, China. Her research interests focus mainly on the design, fabrication, and application of organic metal frameworks for supercapacitors.
Ruifeng Zhou is now a post-graduate student majoring at the School of Chemistry and Materials Engineering, Bohai University, China. His scientific research directions are the preparation and application of environment-friendly materials.
Tieshi He received his Ph.D. degree in materials science from Hefei University of Technology, China in 2009. Since then, he has been working as an associate professor (2009-2019) and a professor (2019-) at the School of Chemical & Materials Engineering, Bohai University, China. His research interests involve advanced functional materials and devices for energy storage and conversion.
Zhenzhen Wang received her B.S. degrees from Anyang Normal University. She is currently studying for an M.Sc. degree at the School of Chemistry & Materials Engineering, Bohai University, China. Her research focuses on the design, optimization, and application of new energy storage materials.
Xiangye Li received his M.Sc. degree from Bohai University. He is currently pursuing his Ph.D. degree at the School of Materials Science and Engineering, Lanzhou University of Technology, China. His research interests focus mainly on the design and fabrication of new kinds of energy storage materials and the related mechanisms.
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  year: 2022
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Snippet In recent years, a great deal of investigation has been performed based on the study of metal-organic frameworks (MOFs) combined with other materials, in order...
In recent years, a great deal of investigation has been performed based on the study of metal–organic frameworks (MOFs) combined with other materials, in order...
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SubjectTerms chemistry
coordination polymers
Electrospinning
energy
Energy conservation
Energy storage
Environmental protection
Fabrication
Functional materials
Metal-organic frameworks
Nanofibers
natural resources conservation
Porous materials
Title Electrospun metal-organic framework based nanofibers for energy storage and environmental applications: current approaches and challenges
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