High-performance lead-free bulk ceramics for electrical energy storage applications: design strategies and challenges

Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power systems due to their fast charge/discharge rates and ultrahigh power density. Dielectric materials are core components of dielectric capacitors...

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Published in	Journal of materials chemistry. A, Materials for energy and sustainability Vol. 9; no. 34; pp. 1826 - 1885
Main Authors	Yang, Zetian, Du, Hongliang, Jin, Li, Poelman, Dirk
Format	Journal Article
Language	English
Published	Cambridge Royal Society of Chemistry 31.08.2021
Subjects	Barium titanates Capacitors Ceramics Chemical composition electric power Electric power systems Electrochemistry energy Energy storage Fuel cells Lead free Physical properties Strontium titanates
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Abstract	Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power systems due to their fast charge/discharge rates and ultrahigh power density. Dielectric materials are core components of dielectric capacitors and directly determine their performance. Over the past decade, extensive efforts have been devoted to develop high-performance dielectric materials for electrical energy storage applications and great progress has been achieved. Here, we present an overview on the current state-of-the-art lead-free bulk ceramics for electrical energy storage applications, including SrTiO 3 , CaTiO 3 , BaTiO 3 , (Bi 0.5 Na 0.5 )TiO 3 , (K 0.5 Na 0.5 )NbO 3 , BiFeO 3 , AgNbO 3 and NaNbO 3 -based ceramics. This review starts with a brief introduction of the research background, the development history and the basic fundamentals of dielectric materials for energy storage applications as well as the universal strategies to optimize their energy storage performance. Emphases are placed on the design strategies for each type of dielectric ceramic based on their special physical properties with a summary of their respective advantages and disadvantages. Challenges along with future prospects are presented at the end of this review. This review will not only accelerate the exploration of higher performance lead-free dielectric materials, but also provides a deeper understanding of the relationship among chemical composition, physical properties and energy storage performance. This review summarizes the development history of lead-free bulk ceramics for electrical energy storage applications and stress the design strategies for each type of dielectric ceramic based on their special physical properties.
AbstractList	Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power systems due to their fast charge/discharge rates and ultrahigh power density. Dielectric materials are core components of dielectric capacitors and directly determine their performance. Over the past decade, extensive efforts have been devoted to develop high-performance dielectric materials for electrical energy storage applications and great progress has been achieved. Here, we present an overview on the current state-of-the-art lead-free bulk ceramics for electrical energy storage applications, including SrTiO 3 , CaTiO 3 , BaTiO 3 , (Bi 0.5 Na 0.5 )TiO 3 , (K 0.5 Na 0.5 )NbO 3 , BiFeO 3 , AgNbO 3 and NaNbO 3 -based ceramics. This review starts with a brief introduction of the research background, the development history and the basic fundamentals of dielectric materials for energy storage applications as well as the universal strategies to optimize their energy storage performance. Emphases are placed on the design strategies for each type of dielectric ceramic based on their special physical properties with a summary of their respective advantages and disadvantages. Challenges along with future prospects are presented at the end of this review. This review will not only accelerate the exploration of higher performance lead-free dielectric materials, but also provides a deeper understanding of the relationship among chemical composition, physical properties and energy storage performance. This review summarizes the development history of lead-free bulk ceramics for electrical energy storage applications and stress the design strategies for each type of dielectric ceramic based on their special physical properties. Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power systems due to their fast charge/discharge rates and ultrahigh power density. Dielectric materials are core components of dielectric capacitors and directly determine their performance. Over the past decade, extensive efforts have been devoted to develop high-performance dielectric materials for electrical energy storage applications and great progress has been achieved. Here, we present an overview on the current state-of-the-art lead-free bulk ceramics for electrical energy storage applications, including SrTiO 3 , CaTiO 3 , BaTiO 3 , (Bi 0.5 Na 0.5 )TiO 3 , (K 0.5 Na 0.5 )NbO 3 , BiFeO 3 , AgNbO 3 and NaNbO 3 -based ceramics. This review starts with a brief introduction of the research background, the development history and the basic fundamentals of dielectric materials for energy storage applications as well as the universal strategies to optimize their energy storage performance. Emphases are placed on the design strategies for each type of dielectric ceramic based on their special physical properties with a summary of their respective advantages and disadvantages. Challenges along with future prospects are presented at the end of this review. This review will not only accelerate the exploration of higher performance lead-free dielectric materials, but also provides a deeper understanding of the relationship among chemical composition, physical properties and energy storage performance. Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power systems due to their fast charge/discharge rates and ultrahigh power density. Dielectric materials are core components of dielectric capacitors and directly determine their performance. Over the past decade, extensive efforts have been devoted to develop high-performance dielectric materials for electrical energy storage applications and great progress has been achieved. Here, we present an overview on the current state-of-the-art lead-free bulk ceramics for electrical energy storage applications, including SrTiO3, CaTiO3, BaTiO3, (Bi0.5Na0.5)TiO3, (K0.5Na0.5)NbO3, BiFeO3, AgNbO3 and NaNbO3-based ceramics. This review starts with a brief introduction of the research background, the development history and the basic fundamentals of dielectric materials for energy storage applications as well as the universal strategies to optimize their energy storage performance. Emphases are placed on the design strategies for each type of dielectric ceramic based on their special physical properties with a summary of their respective advantages and disadvantages. Challenges along with future prospects are presented at the end of this review. This review will not only accelerate the exploration of higher performance lead-free dielectric materials, but also provides a deeper understanding of the relationship among chemical composition, physical properties and energy storage performance. Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power systems due to their fast charge/discharge rates and ultrahigh power density. Dielectric materials are core components of dielectric capacitors and directly determine their performance. Over the past decade, extensive efforts have been devoted to develop high-performance dielectric materials for electrical energy storage applications and great progress has been achieved. Here, we present an overview on the current state-of-the-art lead-free bulk ceramics for electrical energy storage applications, including SrTiO₃, CaTiO₃, BaTiO₃, (Bi₀.₅Na₀.₅)TiO₃, (K₀.₅Na₀.₅)NbO₃, BiFeO₃, AgNbO₃ and NaNbO₃-based ceramics. This review starts with a brief introduction of the research background, the development history and the basic fundamentals of dielectric materials for energy storage applications as well as the universal strategies to optimize their energy storage performance. Emphases are placed on the design strategies for each type of dielectric ceramic based on their special physical properties with a summary of their respective advantages and disadvantages. Challenges along with future prospects are presented at the end of this review. This review will not only accelerate the exploration of higher performance lead-free dielectric materials, but also provides a deeper understanding of the relationship among chemical composition, physical properties and energy storage performance.
Author	Du, Hongliang Yang, Zetian Jin, Li Poelman, Dirk
AuthorAffiliation	Ghent University College of Engineering Key Laboratory of the Ministry of Education LumiLab School of Electronic Science and Engineering International Center for Dielectric Research Electronic Materials Research Laboratory Xi'an Jiaotong University Xi'an International University Department of Solid State Sciences
AuthorAffiliation_xml	– name: Ghent University – name: Xi'an International University – name: Key Laboratory of the Ministry of Education – name: Xi'an Jiaotong University – name: LumiLab – name: College of Engineering – name: Electronic Materials Research Laboratory – name: International Center for Dielectric Research – name: Department of Solid State Sciences – name: School of Electronic Science and Engineering
Author_xml	– sequence: 1 givenname: Zetian surname: Yang fullname: Yang, Zetian – sequence: 2 givenname: Hongliang surname: Du fullname: Du, Hongliang – sequence: 3 givenname: Li surname: Jin fullname: Jin, Li – sequence: 4 givenname: Dirk surname: Poelman fullname: Poelman, Dirk
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Notes	Li Jin is a full professor in the School of Electronic Science and Engineering at Xi'an Jiaotong University (XJTU), China. He received his BEng and MEng degrees in Electronics Science and Technology from the XJTU in 2003 and 2006, respectively. He received his PhD degree in Materials Science and Engineering from the Swiss Federal Institute of Technology in Lausanne (EPFL), Switzerland in 2011. Subsequently, he completed his postdoctoral research at the Ceramics Laboratory of EPFL. His interests include ferroelectric/electrostrictive/dielectric materials and their applications in actuators, energy storage devices and other electronic devices. He has published more than 110+ papers in peer-reviewed journals with 6000+ citations. One of his paper has been selected as the 100 Most Influential International Academic Papers in China, in 2014. He has received the First Prize of Natural Science Award by the Ministry of Education of China (2015). Hongliang Du is currently a full professor at college of Engineering, Xi'an International University (XAIU), China. He received his Ph.D. degree from Northwestern Polytechnical University in 2011, and he was a visiting scholar in Technische Universitat Darmstadt (Germany) in 2016. His research interests mainly include lead-free piezoelectric materials, high-temperature piezoelectric ceramics, transparent ferroelectric ceramics and dielectric materials for energy storage applications. He received several awards including Natural Science Second Class Award from Ministry of Education (2010), Excellent Paper Award for Young Scientists from the 11th IUMRS International Conference in Asia (2010), and the First Prize of Scientific and Technological Award from Shaanxi Universities (2021). He has published more than 80 papers in the field of ferro/piezoelectric materials. He was identified as one of the top 1% of highly cited authors in Royal Society of Chemistry (RSC) journals in 2019. Zetian Yang is a Ph.D. student in LumiLab, Department of Solid State Sciences, Ghent University. His research interests mainly include piezoresistive properties of samarium monosulfide, inorganic photochromic materials for optical information storage and anti-counterfeiting applications, and ferroelectric ceramics for electrical energy storage. He has authored/co-authored 17 referred papers with three highly cited papers and one hot paper, and his work has been cited about 1000 times. Dirk Poelman is a full professor in the Department of Solid State Sciences at Ghent University, Belgium since 2012. He obtained his PhD in Ghent University on electroluminescent thin films in 1994. His recent interests include photocatalysis for air purification, luminescent materials for lighting and displays, persistent luminescent compounds for safety applications and near-infrared bio-imaging. He has published over 230 international publications in these fields. Currently, he is working on the relation between the persistent luminescent behaviour of materials, their thermoluminescence characteristics and their photo- and thermochromic properties. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23
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Snippet	Compared with fuel cells and electrochemical capacitors, dielectric capacitors are regarded as promising devices to store electrical energy for pulsed power...
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SubjectTerms	Barium titanates Capacitors Ceramics Chemical composition electric power Electric power systems Electrochemistry energy Energy storage Fuel cells Lead free Physical properties Strontium titanates
Title	High-performance lead-free bulk ceramics for electrical energy storage applications: design strategies and challenges
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