A magnetic continuum in the cobalt-based honeycomb magnet BaCo2(AsO4)2
Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all h...
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| Published in | Nature materials Vol. 22; no. 1; pp. 58 - 63 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.01.2023
Nature Publishing Group Springer Nature |
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| Abstract | Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all have appreciable non-Kitaev interactions. Using time-domain terahertz spectroscopy, we observed a broad magnetic continuum over a wide range of temperatures and fields in the honeycomb cobalt-based magnet BaCo
2
(AsO
4
)
2
, which has been proposed to be a more ideal version of a Kitaev QSL. Applying an in-plane magnetic field of ~0.5 T suppresses the magnetic order, and at higher fields, applying the field gives rise to a spin-polarized state. Under a 4 T magnetic field that was oriented principally out of plane, a broad magnetic continuum was observed that may be consistent with a field-induced QSL. Our results indicate BaCo
2
(AsO
4
)
2
is a promising QSL candidate.
The authors present time-domain terahertz spectroscopy measurements on BaCo
2
(AsO
4
)
2
, a promising 3
d
transition-metal-based quantum spin liquid candidate. |
|---|---|
| AbstractList | Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all have appreciable non-Kitaev interactions. Using time-domain terahertz spectroscopy, we observed a broad magnetic continuum over a wide range of temperatures and fields in the honeycomb cobalt-based magnet BaCo2(AsO4)2, which has been proposed to be a more ideal version of a Kitaev QSL. Applying an in-plane magnetic field of ~0.5 T suppresses the magnetic order, and at higher fields, applying the field gives rise to a spin-polarized state. Under a 4 T magnetic field that was oriented principally out of plane, a broad magnetic continuum was observed that may be consistent with a field-induced QSL. Our results indicate BaCo2(AsO4)2 is a promising QSL candidate.The authors present time-domain terahertz spectroscopy measurements on BaCo2(AsO4)2, a promising 3d transition-metal-based quantum spin liquid candidate. Not provided. Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all have appreciable non-Kitaev interactions. Using time-domain terahertz spectroscopy, we observed a broad magnetic continuum over a wide range of temperatures and fields in the honeycomb cobalt-based magnet BaCo 2 (AsO 4 ) 2 , which has been proposed to be a more ideal version of a Kitaev QSL. Applying an in-plane magnetic field of ~0.5 T suppresses the magnetic order, and at higher fields, applying the field gives rise to a spin-polarized state. Under a 4 T magnetic field that was oriented principally out of plane, a broad magnetic continuum was observed that may be consistent with a field-induced QSL. Our results indicate BaCo 2 (AsO 4 ) 2 is a promising QSL candidate. The authors present time-domain terahertz spectroscopy measurements on BaCo 2 (AsO 4 ) 2 , a promising 3 d transition-metal-based quantum spin liquid candidate. Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all have appreciable non-Kitaev interactions. Using time-domain terahertz spectroscopy, we observed a broad magnetic continuum over a wide range of temperatures and fields in the honeycomb cobalt-based magnet BaCo2(AsO4)2, which has been proposed to be a more ideal version of a Kitaev QSL. Applying an in-plane magnetic field of ~0.5 T suppresses the magnetic order, and at higher fields, applying the field gives rise to a spin-polarized state. Under a 4 T magnetic field that was oriented principally out of plane, a broad magnetic continuum was observed that may be consistent with a field-induced QSL. Our results indicate BaCo2(AsO4)2 is a promising QSL candidate.Quantum spin liquids (QSLs) are topologically ordered states of matter that host fractionalized excitations. A particular route towards a QSL is via strongly bond-dependent interactions on the hexagonal lattice. A number of Ru- and Ir-based candidate Kitaev QSL materials have been pursued, but all have appreciable non-Kitaev interactions. Using time-domain terahertz spectroscopy, we observed a broad magnetic continuum over a wide range of temperatures and fields in the honeycomb cobalt-based magnet BaCo2(AsO4)2, which has been proposed to be a more ideal version of a Kitaev QSL. Applying an in-plane magnetic field of ~0.5 T suppresses the magnetic order, and at higher fields, applying the field gives rise to a spin-polarized state. Under a 4 T magnetic field that was oriented principally out of plane, a broad magnetic continuum was observed that may be consistent with a field-induced QSL. Our results indicate BaCo2(AsO4)2 is a promising QSL candidate. |
| Author | Armitage, N. P. Xu, Yuanyuan Drichko, N. Broholm, C. Zhang, Xinshu Cava, R. J. Halloran, T. Zhong, Ruidan |
| Author_xml | – sequence: 1 givenname: Xinshu surname: Zhang fullname: Zhang, Xinshu organization: Institute for Quantum Matter, Department of Physics and Astronomy, Johns Hopkins University – sequence: 2 givenname: Yuanyuan surname: Xu fullname: Xu, Yuanyuan organization: Institute for Quantum Matter, Department of Physics and Astronomy, Johns Hopkins University – sequence: 3 givenname: T. orcidid: 0000-0001-5284-2339 surname: Halloran fullname: Halloran, T. organization: Institute for Quantum Matter, Department of Physics and Astronomy, Johns Hopkins University – sequence: 4 givenname: Ruidan surname: Zhong fullname: Zhong, Ruidan organization: Department of Chemistry, Princeton University – sequence: 5 givenname: C. orcidid: 0000-0002-1569-9892 surname: Broholm fullname: Broholm, C. organization: Institute for Quantum Matter, Department of Physics and Astronomy, Johns Hopkins University, NIST Center for Neutron Research, National Institute of Standards and Technology, Department of Materials Science and Engineering, Johns Hopkins University – sequence: 6 givenname: R. J. surname: Cava fullname: Cava, R. J. organization: Department of Chemistry, Princeton University – sequence: 7 givenname: N. surname: Drichko fullname: Drichko, N. organization: Institute for Quantum Matter, Department of Physics and Astronomy, Johns Hopkins University – sequence: 8 givenname: N. P. orcidid: 0000-0001-7568-2059 surname: Armitage fullname: Armitage, N. P. email: npa@jhu.edu organization: Institute for Quantum Matter, Department of Physics and Astronomy, Johns Hopkins University, Canadian Institute for Advanced Research |
| BackLink | https://www.osti.gov/biblio/2421157$$D View this record in Osti.gov |
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| SubjectTerms | 639/766/119/2795 639/766/119/997 Biomaterials Chemistry Chemistry and Materials Science Cobalt Condensed Matter Physics Hexagonal lattice Magnetic fields Materials Science Nanotechnology Optical and Electronic Materials Physics Spectroscopy Spectrum analysis Spin liquid Time domain analysis Transition metals |
| Title | A magnetic continuum in the cobalt-based honeycomb magnet BaCo2(AsO4)2 |
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