Metallocene-Catalyzed C7-Linkage in the Hydrooligomerization of Norbornene by σ-Bond Metathesis: Insight into the Microstructure of Polynorbornene

An unusual linkage: The zirconocene‐catalyzed hydrooligomerization of norbornene proceeds by σ‐bond metathesis to form a 2‐exo,7′‐syn linkage (as evident in the pentamer shown). The oligomers were characterized by gas chromatography, NMR spectroscopy , X‐ray crystallography, and DFT calculations....

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Published in	Angewandte Chemie (International ed.) Vol. 43; no. 18; pp. 2444 - 2446
Main Authors	Karafilidis, Christos, Hermann, Holger, Rufiñska, Anna, Gabor, Barbara, Mynott, Richard J., Breitenbruch, Georg, Weidenthaler, Claudia, Rust, Jörg, Joppek, Werner, Brookhart, Maurice S., Thiel, Walter, Fink, Gerhard
Format	Journal Article
Language	English
Published	Weinheim WILEY-VCH Verlag 26.04.2004 WILEY‐VCH Verlag
Subjects	density functional calculations metathesis oligomerization polynorbornene zirconocene
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Abstract	An unusual linkage: The zirconocene‐catalyzed hydrooligomerization of norbornene proceeds by σ‐bond metathesis to form a 2‐exo,7′‐syn linkage (as evident in the pentamer shown). The oligomers were characterized by gas chromatography, NMR spectroscopy , X‐ray crystallography, and DFT calculations.
AbstractList	An unusual linkage: The zirconocene‐catalyzed hydrooligomerization of norbornene proceeds by σ‐bond metathesis to form a 2‐exo,7′‐syn linkage (as evident in the pentamer shown). The oligomers were characterized by gas chromatography, NMR spectroscopy , X‐ray crystallography, and DFT calculations.
Author	Fink, Gerhard Gabor, Barbara Rufiñska, Anna Thiel, Walter Breitenbruch, Georg Brookhart, Maurice S. Mynott, Richard J. Weidenthaler, Claudia Joppek, Werner Karafilidis, Christos Hermann, Holger Rust, Jörg
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Snippet	An unusual linkage: The zirconocene‐catalyzed hydrooligomerization of norbornene proceeds by σ‐bond metathesis to form a 2‐exo,7′‐syn linkage (as evident in...
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SubjectTerms	density functional calculations metathesis oligomerization polynorbornene zirconocene
Title	Metallocene-Catalyzed C7-Linkage in the Hydrooligomerization of Norbornene by σ-Bond Metathesis: Insight into the Microstructure of Polynorbornene
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