Electrode/electrolyte interface and interface reactions of solid oxide cells: Recent development and advances

High temperature solid oxide cells (SOCs) consisted of solid oxide fuel cells (SOFCs) and solid oxide electrolysis cells (SOECs) are considered one of the most environmentally friendly and efficient energy conversion technology to store renewal energy from sun and wind in hydrogen and generate elect...

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Published inProgress in natural science Vol. 31; no. 3; pp. 341 - 372
Main Authors He, Shuai, Jiang, San Ping
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.06.2021
WA School of Mines: Minerals, Energy and Chemical Engineering, Curtin University, Perth, WA, 6102, Australia
Subjects
Effect of polarization
Electrode/electrolyte interface
High temperature sintering
Review
SOFCs and SOECs
Solid oxide cells
Solid oxide cells
Review
SOFCs and SOECs
High temperature sintering
Effect of polarization
Electrode/electrolyte interface
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Abstract High temperature solid oxide cells (SOCs) consisted of solid oxide fuel cells (SOFCs) and solid oxide electrolysis cells (SOECs) are considered one of the most environmentally friendly and efficient energy conversion technology to store renewal energy from sun and wind in hydrogen and generate electricity from the fuels such as hydrogen and natural gas with high efficiency and very low greenhouse gas emission. Over the last few decades, the development of SOC technologies in particularly SOFCs has experienced significant progress and much of the recent research have paid great efforts in understanding the processes occurring at the electrode/electrolyte interfaces. As electrochemical reactions mainly proceed at the gas, electrode and electrolyte three phase boundaries (TPBs), the microstructure and properties of the electrode/electrolyte interfaces thus play a crucial role in determining the overall cell performance and durability. Herein, we review the progress and achievements in the fundamental researches of the electrode/electrolyte (mainly oxygen-conducting) interface evolution behavior under open circuit and polarization conditions. Studies involving interfacial phenomena such as interface formation and reactions, element segregation and diffusion, micropore formation and delamination are summarized and discussed in detail. Besides, the state of the art characterization techniques that have been employed to examine the interface behavior are reviewed. Finally, the challenges and prospects of the interface research in the improvement of the performance and durability of a SOC device are discussed.
AbstractList High temperature solid oxide cells (SOCs) consisted of solid oxide fuel cells (SOFCs) and solid oxide electrolysis cells (SOECs) are considered one of the most environmentally friendly and efficient energy conversion technology to store renewal energy from sun and wind in hydrogen and generate electricity from the fuels such as hydrogen and natural gas with high efficiency and very low greenhouse gas emission. Over the last few decades, the development of SOC technologies in particularly SOFCs has experienced significant progress and much of the recent research have paid great efforts in understanding the processes occurring at the electrode/electrolyte in-terfaces. As electrochemical reactions mainly proceed at the gas, electrode and electrolyte three phase boundaries (TPBs), the microstructure and properties of the electrode/electrolyte interfaces thus play a crucial role in determining the overall cell performance and durability. Herein, we review the progress and achievements in the fundamental researches of the electrode/electrolyte (mainly oxygen-conducting) interface evolution behavior under open circuit and polarization conditions. Studies involving interfacial phenomena such as interface for-mation and reactions, element segregation and diffusion, micropore formation and delamination are summarized and discussed in detail. Besides, the state of the art characterization techniques that have been employed to examine the interface behavior are reviewed. Finally, the challenges and prospects of the interface research in the improvement of the performance and durability of a SOC device are discussed.
High temperature solid oxide cells (SOCs) consisted of solid oxide fuel cells (SOFCs) and solid oxide electrolysis cells (SOECs) are considered one of the most environmentally friendly and efficient energy conversion technology to store renewal energy from sun and wind in hydrogen and generate electricity from the fuels such as hydrogen and natural gas with high efficiency and very low greenhouse gas emission. Over the last few decades, the development of SOC technologies in particularly SOFCs has experienced significant progress and much of the recent research have paid great efforts in understanding the processes occurring at the electrode/electrolyte interfaces. As electrochemical reactions mainly proceed at the gas, electrode and electrolyte three phase boundaries (TPBs), the microstructure and properties of the electrode/electrolyte interfaces thus play a crucial role in determining the overall cell performance and durability. Herein, we review the progress and achievements in the fundamental researches of the electrode/electrolyte (mainly oxygen-conducting) interface evolution behavior under open circuit and polarization conditions. Studies involving interfacial phenomena such as interface formation and reactions, element segregation and diffusion, micropore formation and delamination are summarized and discussed in detail. Besides, the state of the art characterization techniques that have been employed to examine the interface behavior are reviewed. Finally, the challenges and prospects of the interface research in the improvement of the performance and durability of a SOC device are discussed.
Author Jiang, San Ping
He, Shuai
AuthorAffiliation WA School of Mines: Minerals, Energy and Chemical Engineering, Curtin University, Perth, WA, 6102, Australia
AuthorAffiliation_xml – name: WA School of Mines: Minerals, Energy and Chemical Engineering, Curtin University, Perth, WA, 6102, Australia
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Issue 3
Keywords Solid oxide cells
Review
SOFCs and SOECs
High temperature sintering
Effect of polarization
Electrode/electrolyte interface
Language English
License This is an open access article under the CC BY-NC-ND license.
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PublicationTitle Progress in natural science
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WA School of Mines: Minerals, Energy and Chemical Engineering, Curtin University, Perth, WA, 6102, Australia
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Snippet High temperature solid oxide cells (SOCs) consisted of solid oxide fuel cells (SOFCs) and solid oxide electrolysis cells (SOECs) are considered one of the most...
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SubjectTerms Effect of polarization
Electrode/electrolyte interface
High temperature sintering
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SOFCs and SOECs
Solid oxide cells
Title Electrode/electrolyte interface and interface reactions of solid oxide cells: Recent development and advances
URI https://dx.doi.org/10.1016/j.pnsc.2021.03.002
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