Enhanced photocatalytic performance through the ferroelectric synergistic effect of p-n heterojunction BiFeO3/TiO2 under visible-light irradiation
A BiFeO3/TiO2 p-n heterojunction photocatalyst with ferroelectric synergistic effect under visible-light irradiation was developed through facile hydrolysis and precipitation by forming nanospheres of TiO2 on BiFeO3 nanocube to improve the photocatalytic efficiency. Analyses of the microstructure, o...
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| Published in | Ceramics international Vol. 47; no. 8; pp. 10786 - 10795 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
15.04.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | A BiFeO3/TiO2 p-n heterojunction photocatalyst with ferroelectric synergistic effect under visible-light irradiation was developed through facile hydrolysis and precipitation by forming nanospheres of TiO2 on BiFeO3 nanocube to improve the photocatalytic efficiency. Analyses of the microstructure, optical properties, and photoelectrochemical performance indicate the formation of a core–shell heterostructure of BiFeO3/TiO2 with excellent energy band matching. The BiFeO3/TiO2 p-n heterojunction has enlarged specific surface area, higher sensitivity to visible-light, and improved separation and transfer efficiency of photoelectron-hole pairs than single TiO2 and BiFeO3. Moreover, the composite exhibits superior photocatalytic degradation performance for methylene blue (MB) and common antibiotic tetracycline (TC) under UV and visible-light irradiation. The MB degradation rate within 180 min reaches 78.4% and 90.4% under UV and visible-light irradiation, respectively. Furthermore, the enhanced photocatalytic mechanism of BiFeO3/TiO2 is explored by photoluminescence (PL), electrochemical impedance spectroscopy (EIS), transient photocurrent analysis, radical quenching, and band structure characterization. |
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| AbstractList | A BiFeO3/TiO2 p-n heterojunction photocatalyst with ferroelectric synergistic effect under visible-light irradiation was developed through facile hydrolysis and precipitation by forming nanospheres of TiO2 on BiFeO3 nanocube to improve the photocatalytic efficiency. Analyses of the microstructure, optical properties, and photoelectrochemical performance indicate the formation of a core–shell heterostructure of BiFeO3/TiO2 with excellent energy band matching. The BiFeO3/TiO2 p-n heterojunction has enlarged specific surface area, higher sensitivity to visible-light, and improved separation and transfer efficiency of photoelectron-hole pairs than single TiO2 and BiFeO3. Moreover, the composite exhibits superior photocatalytic degradation performance for methylene blue (MB) and common antibiotic tetracycline (TC) under UV and visible-light irradiation. The MB degradation rate within 180 min reaches 78.4% and 90.4% under UV and visible-light irradiation, respectively. Furthermore, the enhanced photocatalytic mechanism of BiFeO3/TiO2 is explored by photoluminescence (PL), electrochemical impedance spectroscopy (EIS), transient photocurrent analysis, radical quenching, and band structure characterization. |
| Author | Zhang, Xuefei Lou, Ching-Wen Lin, Jia-Horng Liao, Xilin Ren, Hai-Tao Mao, Zhiyong Li, Ting-Ting |
| Author_xml | – sequence: 1 givenname: Xilin surname: Liao fullname: Liao, Xilin organization: Innovation Platform of Intelligent and Energy-Saving Textiles, School of Textile Science and Engineering, Tiangong University, Tianjin, 300387, China – sequence: 2 givenname: Ting-Ting surname: Li fullname: Li, Ting-Ting email: tingtingli@tiangong.edu.cn organization: Innovation Platform of Intelligent and Energy-Saving Textiles, School of Textile Science and Engineering, Tiangong University, Tianjin, 300387, China – sequence: 3 givenname: Hai-Tao surname: Ren fullname: Ren, Hai-Tao organization: Innovation Platform of Intelligent and Energy-Saving Textiles, School of Textile Science and Engineering, Tiangong University, Tianjin, 300387, China – sequence: 4 givenname: Zhiyong surname: Mao fullname: Mao, Zhiyong organization: School of Materials Science and Engineering and Tianjin Key Laboratory for Photoelectric Materials and Devices, Tianjin University of Technology, Tianjin, 300384, PR China – sequence: 5 givenname: Xuefei surname: Zhang fullname: Zhang, Xuefei organization: Innovation Platform of Intelligent and Energy-Saving Textiles, School of Textile Science and Engineering, Tiangong University, Tianjin, 300387, China – sequence: 6 givenname: Jia-Horng surname: Lin fullname: Lin, Jia-Horng email: jhlin@fcu.edu.tw organization: Innovation Platform of Intelligent and Energy-Saving Textiles, School of Textile Science and Engineering, Tiangong University, Tianjin, 300387, China – sequence: 7 givenname: Ching-Wen surname: Lou fullname: Lou, Ching-Wen email: cwlou@asia.edu.tw organization: Innovation Platform of Intelligent and Energy-Saving Textiles, School of Textile Science and Engineering, Tiangong University, Tianjin, 300387, China |
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| Keywords | Synergistic Ferroelectric Photocatalytic BiFeO3/TiO2 Visible light p-n heterojunctions |
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