Two-dimensional metal-organic framework materials for energy conversion and storage

Selecting and assembling metal ions and bridging ligands can fabricate two-dimensional metal-organic framework nanosheets, which can act as prospective materials for efficient energy applications. Thanks to large surface area and more porosity, ultrathin 2D MOFs nanosheets and their derived two-dime...

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Published inJournal of power sources Vol. 477; p. 228919
Main Authors Tang, Xuxu, Zhao, Lu, Sun, Weiwei, Wang, Yong
Format Journal Article
LanguageEnglish
Published Elsevier B.V 30.11.2020
Subjects
Energy storage/conversion
Metal-organic frameworks
Nanosheets
Two-dimensional
Nanosheets
Energy storage/conversion
Metal-organic frameworks
Two-dimensional
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Abstract Selecting and assembling metal ions and bridging ligands can fabricate two-dimensional metal-organic framework nanosheets, which can act as prospective materials for efficient energy applications. Thanks to large surface area and more porosity, ultrathin 2D MOFs nanosheets and their derived two-dimensional nanosheet materials exhibit more highly approachable active sites uncovered on the surface, decreased ion diffusion distance and fast electron transfer for energy storage/conversion applications. Herein, this review will summarize the latest developments with discussion of design, fabrication, energy storage as well as conversion performance of 2D MOFs and their-derived two-dimensional materials. Moreover, the development of exfoliated two-dimensional MOFs and their derivatives, as well as the promising trends and prospects in application as excellent-performance electrode materials in batteries, supercapacitors, and electrocatalysis are also present. [Display omitted] •Recent developments of 2D MOF materials for energy applications are reviewed.•Design strategies of 2D MOF related materials are summarized.•Relationship between the structure and performance is discussed in details.•Future research tendency of 2D MOF-related materials is highlighted.
AbstractList Selecting and assembling metal ions and bridging ligands can fabricate two-dimensional metal-organic framework nanosheets, which can act as prospective materials for efficient energy applications. Thanks to large surface area and more porosity, ultrathin 2D MOFs nanosheets and their derived two-dimensional nanosheet materials exhibit more highly approachable active sites uncovered on the surface, decreased ion diffusion distance and fast electron transfer for energy storage/conversion applications. Herein, this review will summarize the latest developments with discussion of design, fabrication, energy storage as well as conversion performance of 2D MOFs and their-derived two-dimensional materials. Moreover, the development of exfoliated two-dimensional MOFs and their derivatives, as well as the promising trends and prospects in application as excellent-performance electrode materials in batteries, supercapacitors, and electrocatalysis are also present. [Display omitted] •Recent developments of 2D MOF materials for energy applications are reviewed.•Design strategies of 2D MOF related materials are summarized.•Relationship between the structure and performance is discussed in details.•Future research tendency of 2D MOF-related materials is highlighted.
ArticleNumber 228919
Author Tang, Xuxu
Zhao, Lu
Wang, Yong
Sun, Weiwei
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  givenname: Lu
  surname: Zhao
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  givenname: Weiwei
  surname: Sun
  fullname: Sun, Weiwei
  email: vivisun@shu.edu.cn
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  email: yongwang@shu.edu.cn
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  publication-title: ACS Appl. Mater. Interfaces
  doi: 10.1021/acsami.8b09812
– volume: 6
  issue: 4
  year: 2019
  ident: 10.1016/j.jpowsour.2020.228919_bib100
  publication-title: 2D Mater.
  doi: 10.1088/2053-1583/ab2efc
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Snippet Selecting and assembling metal ions and bridging ligands can fabricate two-dimensional metal-organic framework nanosheets, which can act as prospective...
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elsevier
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StartPage 228919
SubjectTerms Energy storage/conversion
Metal-organic frameworks
Nanosheets
Two-dimensional
Title Two-dimensional metal-organic framework materials for energy conversion and storage
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