Core-shell structured Fe2O3@Fe3C@C nanochains and Ni–Co carbonate hydroxide hybridized microspheres for high-performance battery-type supercapacitor
Battery-supercapacitor hybrid (BSH) device is one of the most promising candidates for next advanced energy storage systems because it can bridge the performance gap between lithium ion batteries and conventional capacitors. Herein, we report a novel porous core-shell structured Fe2O3@Fe3C@C nanocha...
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| Published in | Journal of power sources Vol. 482; p. 228915 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.01.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Battery-supercapacitor hybrid (BSH) device is one of the most promising candidates for next advanced energy storage systems because it can bridge the performance gap between lithium ion batteries and conventional capacitors. Herein, we report a novel porous core-shell structured Fe2O3@Fe3C@C nanochains and urchin-like Ni–Co carbonate hydroxide hybridized (denoted as NiCo–CHH) microspheres for advanced battery-type supercapacitors. The as-obtained Fe2O3@Fe3C@C anode shows high specific capacity (611 C g−1) and good rate capability. The fabricated NiCo–CHH cathode delivers high specific capacity (814 C g−1) and excellent cycling stability. When assembled into a battery-type supercapacitor, the NiCo–CHH//Fe2O3@Fe3C@C device delivers a high energy density (95.2 Wh kg−1) and excellent cycling stability. Moreover, In situ Raman spectroscopy proves the reversibility of the NiCo–CHH electrode, and the synergistic effects of Ni and Co ions, further revealing its energy storage mechanism. These findings provide a novel insight on high-performance battery-type supercapacitors.
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•The Fe2O3@Fe3C@C nanochains are successfully constructed, exhibiting high capacity.•The NiCo–CHH electrode exhibits outstanding electrochemical performance.•The charge storage behaviour of NiCo–CHH is probed by in situ Raman spectroscopy.•The battery-type supercapacitor demonstrates high energy storage capability. |
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| AbstractList | Battery-supercapacitor hybrid (BSH) device is one of the most promising candidates for next advanced energy storage systems because it can bridge the performance gap between lithium ion batteries and conventional capacitors. Herein, we report a novel porous core-shell structured Fe2O3@Fe3C@C nanochains and urchin-like Ni–Co carbonate hydroxide hybridized (denoted as NiCo–CHH) microspheres for advanced battery-type supercapacitors. The as-obtained Fe2O3@Fe3C@C anode shows high specific capacity (611 C g−1) and good rate capability. The fabricated NiCo–CHH cathode delivers high specific capacity (814 C g−1) and excellent cycling stability. When assembled into a battery-type supercapacitor, the NiCo–CHH//Fe2O3@Fe3C@C device delivers a high energy density (95.2 Wh kg−1) and excellent cycling stability. Moreover, In situ Raman spectroscopy proves the reversibility of the NiCo–CHH electrode, and the synergistic effects of Ni and Co ions, further revealing its energy storage mechanism. These findings provide a novel insight on high-performance battery-type supercapacitors.
[Display omitted]
•The Fe2O3@Fe3C@C nanochains are successfully constructed, exhibiting high capacity.•The NiCo–CHH electrode exhibits outstanding electrochemical performance.•The charge storage behaviour of NiCo–CHH is probed by in situ Raman spectroscopy.•The battery-type supercapacitor demonstrates high energy storage capability. |
| ArticleNumber | 228915 |
| Author | Liu, Meilin Zhang, Sen Shen, Weixia Dai, Shuge Hu, Hao Wang, Xinchang Fu, Jianwei Hu, Chenguo Bai, Yucheng |
| Author_xml | – sequence: 1 givenname: Shuge surname: Dai fullname: Dai, Shuge email: shugedai@zzu.edu.cn organization: Key Laboratory of Material Physics of Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou, 450052, PR China – sequence: 2 givenname: Yucheng surname: Bai fullname: Bai, Yucheng organization: Key Laboratory of Material Physics of Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou, 450052, PR China – sequence: 3 givenname: Weixia surname: Shen fullname: Shen, Weixia organization: Key Laboratory of Material Physics of Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou, 450052, PR China – sequence: 4 givenname: Sen surname: Zhang fullname: Zhang, Sen organization: Key Laboratory of Material Physics of Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou, 450052, PR China – sequence: 5 givenname: Hao surname: Hu fullname: Hu, Hao organization: School of Materials Science and Engineering, Henan University of Science and Technology, Luoyang, Henan, 471023, PR China – sequence: 6 givenname: Jianwei orcidid: 0000-0002-2570-2610 surname: Fu fullname: Fu, Jianwei email: jwfu@zzu.edu.cn organization: School of Materials Science and Engineering, Zhengzhou University, Zhengzhou, 450052, PR China – sequence: 7 givenname: Xinchang surname: Wang fullname: Wang, Xinchang organization: Key Laboratory of Material Physics of Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou, 450052, PR China – sequence: 8 givenname: Chenguo surname: Hu fullname: Hu, Chenguo email: hucg@cqu.edu.cn organization: Department of Applied Physics, Chongqing University, Chongqing, 400044, PR China – sequence: 9 givenname: Meilin surname: Liu fullname: Liu, Meilin organization: School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA, 30332-0245, USA |
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| Snippet | Battery-supercapacitor hybrid (BSH) device is one of the most promising candidates for next advanced energy storage systems because it can bridge the... |
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| SubjectTerms | Battery-type supercapacitors Fe2O3@Fe3C@C nanochains In-situ Raman NiCo–CHH microspheres |
| Title | Core-shell structured Fe2O3@Fe3C@C nanochains and Ni–Co carbonate hydroxide hybridized microspheres for high-performance battery-type supercapacitor |
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