Effect of organic additives on positive electrolyte for vanadium redox battery

► Four organics as electrolyte additives of vanadium redox battery. ► Changes are examined in the electrochemical properties of vanadium redox battery. ► d-sorbitol is a suitable additive to the electrolyte for the vanadium redox battery. ► The mechanism of improvement is discussed in detail. Fructo...

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Published in	Electrochimica acta Vol. 56; no. 16; pp. 5483 - 5487
Main Authors	Li, Sha, Huang, Kelong, Liu, Suqin, Fang, Dong, Wu, Xiongwei, Lu, Dan, Wu, Tao
Format	Journal Article
Language	English
Published	Kidlington Elsevier Ltd 30.06.2011 Elsevier
Subjects	Additives Applied sciences Battery d-sorbitol Direct energy conversion and energy accumulation Electric batteries Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Electrochemical impedance spectroscopy Electrolyte Electrolytes Exact sciences and technology Fructose Redox cells Solubility Vanadium Vanadium redox flow batteries Additives Vanadium redox flow batteries Electrolyte d-sorbitol Sorbitol Flow battery Vanadyl Sulfates Transition metal Secondary cell Discharge charge cycle Acidic solution Sulfuric acid Electrodes Additive Alditol Redox couple Medium effect Graphite Raman spectrometry D-sorbitol Electrical characteristic Electrochemical impedance spectroscopy
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Abstract	► Four organics as electrolyte additives of vanadium redox battery. ► Changes are examined in the electrochemical properties of vanadium redox battery. ► d-sorbitol is a suitable additive to the electrolyte for the vanadium redox battery. ► The mechanism of improvement is discussed in detail. Fructose, mannitol, glucose, d-sorbitol are explored as additives in electrolyte for vanadium redox battery (VRB), respectively. The effects of additives on electrolyte are studied by cyclic voltammetry (CV), charge–discharge technique, electrochemical impedance spectroscopy (EIS) and Raman spectroscopy. The results indicate that the vanadium redox cell using the electrolyte with the additive of d-sorbitol exhibits the best electrochemical performance (the energy efficiency 81.8%). The EIS results indicate that the electrochemical activity of the electrolyte is improved by adding d-sorbitol, which can be interpreted as the increase of available (–OH) groups providing active sites for electron transfer. The Raman spectra show that VO 2+ ions take part in forming a complex with the d-sorbitol, which not only improve solubility of V(V) electrolyte, but also provide more activity sites for the V(IV)/V(V) redox reaction.
AbstractList	► Four organics as electrolyte additives of vanadium redox battery. ► Changes are examined in the electrochemical properties of vanadium redox battery. ► d-sorbitol is a suitable additive to the electrolyte for the vanadium redox battery. ► The mechanism of improvement is discussed in detail. Fructose, mannitol, glucose, d-sorbitol are explored as additives in electrolyte for vanadium redox battery (VRB), respectively. The effects of additives on electrolyte are studied by cyclic voltammetry (CV), charge–discharge technique, electrochemical impedance spectroscopy (EIS) and Raman spectroscopy. The results indicate that the vanadium redox cell using the electrolyte with the additive of d-sorbitol exhibits the best electrochemical performance (the energy efficiency 81.8%). The EIS results indicate that the electrochemical activity of the electrolyte is improved by adding d-sorbitol, which can be interpreted as the increase of available (–OH) groups providing active sites for electron transfer. The Raman spectra show that VO 2+ ions take part in forming a complex with the d-sorbitol, which not only improve solubility of V(V) electrolyte, but also provide more activity sites for the V(IV)/V(V) redox reaction. Fructose, mannitol, glucose, d-sorbitol are explored as additives in electrolyte for vanadium redox battery (VRB), respectively. The effects of additives on electrolyte are studied by cyclic voltammetry (CV), charge-discharge technique, electrochemical impedance spectroscopy (EIS) and Raman spectroscopy. The results indicate that the vanadium redox cell using the electrolyte with the additive of d-sorbitol exhibits the best electrochemical performance (the energy efficiency 81.8%). The EIS results indicate that the electrochemical activity of the electrolyte is improved by adding d-sorbitol, which can be interpreted as the increase of available (-OH) groups providing active sites for electron transfer. The Raman spectra show that VO[super]2+ ions take part in forming a complex with the d-sorbitol, which not only improve solubility of V(V) electrolyte, but also provide more activity sites for the V(IV)/V(V) redox reaction. Four organics as electrolyte additives of vanadium redox battery. Changes are examined in the electrochemical properties of vanadium redox battery. d-sorbitol is a suitable additive to the electrolyte for the vanadium redox battery. The mechanism of improvement is discussed in detail.
Author	Wu, Tao Fang, Dong Huang, Kelong Liu, Suqin Wu, Xiongwei Lu, Dan Li, Sha
Author_xml	– sequence: 1 givenname: Sha surname: Li fullname: Li, Sha – sequence: 2 givenname: Kelong surname: Huang fullname: Huang, Kelong email: lisha_csu@163.com, huangkelong@yahoo.com.cn – sequence: 3 givenname: Suqin surname: Liu fullname: Liu, Suqin – sequence: 4 givenname: Dong surname: Fang fullname: Fang, Dong – sequence: 5 givenname: Xiongwei surname: Wu fullname: Wu, Xiongwei – sequence: 6 givenname: Dan surname: Lu fullname: Lu, Dan – sequence: 7 givenname: Tao surname: Wu fullname: Wu, Tao
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Keywords	Additives Vanadium redox flow batteries Electrolyte d-sorbitol Sorbitol Flow battery Vanadyl Sulfates Transition metal Secondary cell Discharge charge cycle Acidic solution Sulfuric acid Electrodes Additive Alditol Redox couple Medium effect Graphite Raman spectrometry D-sorbitol Electrical characteristic Electrochemical impedance spectroscopy
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Snippet	► Four organics as electrolyte additives of vanadium redox battery. ► Changes are examined in the electrochemical properties of vanadium redox battery. ►... Fructose, mannitol, glucose, d-sorbitol are explored as additives in electrolyte for vanadium redox battery (VRB), respectively. The effects of additives on...
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SubjectTerms	Additives Applied sciences Battery d-sorbitol Direct energy conversion and energy accumulation Electric batteries Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Electrochemical impedance spectroscopy Electrolyte Electrolytes Exact sciences and technology Fructose Redox cells Solubility Vanadium Vanadium redox flow batteries
Title	Effect of organic additives on positive electrolyte for vanadium redox battery
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