The shadow of dichloroacetonitrile (DCAN), a typical nitrogenous disinfection by-product (N-DBP), in the waterworks and its backwash water reuse

Dichloroacetonitrile (DCAN) is one of nitrogenous disinfection by-products (N-DBPs) with strong cytotoxicity and genotoxicity. In this study, the formation potential (FP) of DCAN was investigated in the samples of six important water sources located in the Yangtze River Delta. The highest formation...

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Published inChemosphere (Oxford) Vol. 181; pp. 569 - 578
Main Authors Tan, Yiwen, Lin, Tao, Jiang, Fuchun, Dong, Jian, Chen, Wei, Zhou, Dongju
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 01.08.2017
Subjects
Acetonitriles - analysis
Acetonitriles - isolation & purification
Backwash water
Charcoal
Dichloroacetonitrile
Disinfection
Drinking Water - standards
Drinking water treatment
Filtration
Lakes
Nitrogen
Nitrogenous disinfection by-product
Reuse
Water Pollutants - analysis
Water Pollutants - isolation & purification
Water Pollutants, Chemical - analysis
Water Purification - methods
Drinking water treatment
Nitrogenous disinfection by-product
Dichloroacetonitrile
Backwash water
Reuse
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Abstract Dichloroacetonitrile (DCAN) is one of nitrogenous disinfection by-products (N-DBPs) with strong cytotoxicity and genotoxicity. In this study, the formation potential (FP) of DCAN was investigated in the samples of six important water sources located in the Yangtze River Delta. The highest formation concentration of DCAN was 9.05 μg/L in the water sample taken from Taihu Lake with the lowest SUVA value. After the NOM fractionation, the conversion rate of hydrophilic fraction to DCAN was found the highest. Subsequently, a waterworks using Taihu Lake as water source was chosen to research the FP variations of DCAN in the treatment process and backwash water. The results showed that, compared to the conventional treatment process, O/biological activated carbon (BAC) process increased the removal efficiency of DCAN from 21.89% to 50.58% by removing aromatic protein and soluble biological by-products as main precursors of DCAN. The DCAN FP in the effluent of BAC filters using old granular activated carbon was higher than that in the influent and the DCAN FP of its backwash water was lower than that in raw water. In the backwash water of sand filters, the DCAN FP higher than raw water required the recycle ratio less than 5% to avoid the accumulation of DCAN. •The DCAN FP's remove by conventional and advanced treatment process was investigated.•DCAN FP in effluent of old GAC filter increased due to the decreased adsorption.•The recycle ratio of sand filters' backwash water >5% may cause DCAN's accumulation.
AbstractList Dichloroacetonitrile (DCAN) is one of nitrogenous disinfection by-products (N-DBPs) with strong cytotoxicity and genotoxicity. In this study, the formation potential (FP) of DCAN was investigated in the samples of six important water sources located in the Yangtze River Delta. The highest formation concentration of DCAN was 9.05 μg/L in the water sample taken from Taihu Lake with the lowest SUVA value. After the NOM fractionation, the conversion rate of hydrophilic fraction to DCAN was found the highest. Subsequently, a waterworks using Taihu Lake as water source was chosen to research the FP variations of DCAN in the treatment process and backwash water. The results showed that, compared to the conventional treatment process, O/biological activated carbon (BAC) process increased the removal efficiency of DCAN from 21.89% to 50.58% by removing aromatic protein and soluble biological by-products as main precursors of DCAN. The DCAN FP in the effluent of BAC filters using old granular activated carbon was higher than that in the influent and the DCAN FP of its backwash water was lower than that in raw water. In the backwash water of sand filters, the DCAN FP higher than raw water required the recycle ratio less than 5% to avoid the accumulation of DCAN. •The DCAN FP's remove by conventional and advanced treatment process was investigated.•DCAN FP in effluent of old GAC filter increased due to the decreased adsorption.•The recycle ratio of sand filters' backwash water >5% may cause DCAN's accumulation.
Dichloroacetonitrile (DCAN) is one of nitrogenous disinfection by-products (N-DBPs) with strong cytotoxicity and genotoxicity. In this study, the formation potential (FP) of DCAN was investigated in the samples of six important water sources located in the Yangtze River Delta. The highest formation concentration of DCAN was 9.05 μg/L in the water sample taken from Taihu Lake with the lowest SUVA value. After the NOM fractionation, the conversion rate of hydrophilic fraction to DCAN was found the highest. Subsequently, a waterworks using Taihu Lake as water source was chosen to research the FP variations of DCAN in the treatment process and backwash water. The results showed that, compared to the conventional treatment process, O/biological activated carbon (BAC) process increased the removal efficiency of DCAN from 21.89% to 50.58% by removing aromatic protein and soluble biological by-products as main precursors of DCAN. The DCAN FP in the effluent of BAC filters using old granular activated carbon was higher than that in the influent and the DCAN FP of its backwash water was lower than that in raw water. In the backwash water of sand filters, the DCAN FP higher than raw water required the recycle ratio less than 5% to avoid the accumulation of DCAN.
Author Chen, Wei
Dong, Jian
Zhou, Dongju
Lin, Tao
Jiang, Fuchun
Tan, Yiwen
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Keywords Drinking water treatment
Nitrogenous disinfection by-product
Dichloroacetonitrile
Backwash water
Reuse
Language English
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Snippet Dichloroacetonitrile (DCAN) is one of nitrogenous disinfection by-products (N-DBPs) with strong cytotoxicity and genotoxicity. In this study, the formation...
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SubjectTerms Acetonitriles - analysis
Acetonitriles - isolation & purification
Backwash water
Charcoal
Dichloroacetonitrile
Disinfection
Drinking Water - standards
Drinking water treatment
Filtration
Lakes
Nitrogen
Nitrogenous disinfection by-product
Reuse
Water Pollutants - analysis
Water Pollutants - isolation & purification
Water Pollutants, Chemical - analysis
Water Purification - methods
Title The shadow of dichloroacetonitrile (DCAN), a typical nitrogenous disinfection by-product (N-DBP), in the waterworks and its backwash water reuse
URI https://dx.doi.org/10.1016/j.chemosphere.2017.04.118
https://www.ncbi.nlm.nih.gov/pubmed/28467950
https://search.proquest.com/docview/1895277811
Volume 181
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