Structure-function relationships of deep eutectic solvents for lignin extraction and chemical transformation
Lignin is the most abundant natural aromatic feedstock, and the conversion of lignin to value-added chemicals has drawn immense attention in biorefineries. Deep eutectic solvents (DESs) have been used for lignocellulosic biomass fractionation and lignin extraction due to their simple procedure, sele...
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| Published in | Green chemistry : an international journal and green chemistry resource : GC Vol. 22; no. 21; pp. 7219 - 7232 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
02.11.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Lignin is the most abundant natural aromatic feedstock, and the conversion of lignin to value-added chemicals has drawn immense attention in biorefineries. Deep eutectic solvents (DESs) have been used for lignocellulosic biomass fractionation and lignin extraction due to their simple procedure, selective solubility of lignin, low cost, and high recyclability. The nature and number of functional groups in DESs remarkably influence the delignification and structural changes of lignin during treatment. Although many studies have investigated lignin extraction and the following chemical transformations during DES treatment, no review has illuminated the structure-function relationships between DESs and lignin. This review presents a systematic overview of important studies to provide insights into lignin extraction and chemical transformations by examining the relationship between the type and number of functional groups in DES constituents during pretreatment. Furthermore, various challenges and opportunities in the development of more sustainable and efficient lignin extraction are provided according to the remaining problems in this field.
The effect of the structure and properties of DESs on lignin extraction and chemical transformations. |
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| AbstractList | Lignin is the most abundant natural aromatic feedstock, and the conversion of lignin to value-added chemicals has drawn immense attention in biorefineries. Deep eutectic solvents (DESs) have been used for lignocellulosic biomass fractionation and lignin extraction due to their simple procedure, selective solubility of lignin, low cost, and high recyclability. The nature and number of functional groups in DESs remarkably influence the delignification and structural changes of lignin during treatment. Although many studies have investigated lignin extraction and the following chemical transformations during DES treatment, no review has illuminated the structure–function relationships between DESs and lignin. This review presents a systematic overview of important studies to provide insights into lignin extraction and chemical transformations by examining the relationship between the type and number of functional groups in DES constituents during pretreatment. Furthermore, various challenges and opportunities in the development of more sustainable and efficient lignin extraction are provided according to the remaining problems in this field. Lignin is the most abundant natural aromatic feedstock, and the conversion of lignin to value-added chemicals has drawn immense attention in biorefineries. Deep eutectic solvents (DESs) have been used for lignocellulosic biomass fractionation and lignin extraction due to their simple procedure, selective solubility of lignin, low cost, and high recyclability. The nature and number of functional groups in DESs remarkably influence the delignification and structural changes of lignin during treatment. Although many studies have investigated lignin extraction and the following chemical transformations during DES treatment, no review has illuminated the structure-function relationships between DESs and lignin. This review presents a systematic overview of important studies to provide insights into lignin extraction and chemical transformations by examining the relationship between the type and number of functional groups in DES constituents during pretreatment. Furthermore, various challenges and opportunities in the development of more sustainable and efficient lignin extraction are provided according to the remaining problems in this field. The effect of the structure and properties of DESs on lignin extraction and chemical transformations. |
| Author | Xue, Zhimin Yuan, Tong-Qi Hong, Si Shen, Xiao-Jun Sun, Zhuohua |
| AuthorAffiliation | Chinese Academy of Sciences Institute of Chemistry Beijing Advanced Innovation Center for Tree Breeding by Molecular Design Beijing National Laboratory for Molecular Sciences CAS Research/Education Center for Excellence in Molecular Sciences CAS Key Laboratory of Colloid and Interface and Thermodynamics Beijing Forestry University Beijing Key Laboratory of Lignocellulosic Chemistry |
| AuthorAffiliation_xml | – name: CAS Key Laboratory of Colloid and Interface and Thermodynamics – name: Beijing National Laboratory for Molecular Sciences – name: Institute of Chemistry – name: Chinese Academy of Sciences – name: Beijing Forestry University – name: Beijing Advanced Innovation Center for Tree Breeding by Molecular Design – name: CAS Research/Education Center for Excellence in Molecular Sciences – name: Beijing Key Laboratory of Lignocellulosic Chemistry |
| Author_xml | – sequence: 1 givenname: Si surname: Hong fullname: Hong, Si – sequence: 2 givenname: Xiao-Jun surname: Shen fullname: Shen, Xiao-Jun – sequence: 3 givenname: Zhimin surname: Xue fullname: Xue, Zhimin – sequence: 4 givenname: Zhuohua surname: Sun fullname: Sun, Zhuohua – sequence: 5 givenname: Tong-Qi surname: Yuan fullname: Yuan, Tong-Qi |
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| Snippet | Lignin is the most abundant natural aromatic feedstock, and the conversion of lignin to value-added chemicals has drawn immense attention in biorefineries.... |
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| SubjectTerms | biomass Biorefineries biorefining delignification feedstocks Fractionation Functional groups Green chemistry Lignin Lignocellulose Pretreatment Recyclability solubility Solvents Structure-function relationships Sustainable development Transformations value added |
| Title | Structure-function relationships of deep eutectic solvents for lignin extraction and chemical transformation |
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