Tuning the electronic structure of layered vanadium pentoxide by pre-intercalation of potassium ions for superior room/low-temperature aqueous zinc-ion batteries
Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn 2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K + pre-intercalated layered V 2 O 5 (K 0.5 V 2 O 5 ) composites with metallic features a...
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| Published in | Nanoscale Vol. 13; no. 4; pp. 2399 - 247 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
04.02.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn
2+
diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K
+
pre-intercalated layered V
2
O
5
(K
0.5
V
2
O
5
) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K
0.5
V
2
O
5
electrode delivers a high reversible capacity of 251 mA h g
−1
at 5 A g
−1
after 1000 cycles. Even at a low temperature of −20 °C, high reversible capacities of 241 and 115 mA h g
−1
can be obtained after 1000 cycles at 1 and 5 A g
−1
, respectively. The outstanding electrochemical performance is attributed to the incorporation of K
+
into the layered V
2
O
5
, which acts as pillars to promote the Zn
2+
diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K
+
can benefit electron migration, and therefore enhance the Zn
2+
(de)intercalation kinetics. Meanwhile, the Zn
2+
storage mechanism of K
0.5
V
2
O
5
is revealed by
ex situ
X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs.
Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn
2+
diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. |
|---|---|
| AbstractList | Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K+ pre-intercalated layered V2O5 (K0.5V2O5) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K0.5V2O5 electrode delivers a high reversible capacity of 251 mA h g-1 at 5 A g-1 after 1000 cycles. Even at a low temperature of -20 °C, high reversible capacities of 241 and 115 mA h g-1 can be obtained after 1000 cycles at 1 and 5 A g-1, respectively. The outstanding electrochemical performance is attributed to the incorporation of K+ into the layered V2O5, which acts as pillars to promote the Zn2+ diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K+ can benefit electron migration, and therefore enhance the Zn2+ (de)intercalation kinetics. Meanwhile, the Zn2+ storage mechanism of K0.5V2O5 is revealed by ex situ X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs. Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn 2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K + pre-intercalated layered V 2 O 5 (K 0.5 V 2 O 5 ) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K 0.5 V 2 O 5 electrode delivers a high reversible capacity of 251 mA h g −1 at 5 A g −1 after 1000 cycles. Even at a low temperature of −20 °C, high reversible capacities of 241 and 115 mA h g −1 can be obtained after 1000 cycles at 1 and 5 A g −1 , respectively. The outstanding electrochemical performance is attributed to the incorporation of K + into the layered V 2 O 5 , which acts as pillars to promote the Zn 2+ diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K + can benefit electron migration, and therefore enhance the Zn 2+ (de)intercalation kinetics. Meanwhile, the Zn 2+ storage mechanism of K 0.5 V 2 O 5 is revealed by ex situ X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs. Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn 2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K + pre-intercalated layered V 2 O 5 (K 0.5 V 2 O 5 ) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K 0.5 V 2 O 5 electrode delivers a high reversible capacity of 251 mA h g −1 at 5 A g −1 after 1000 cycles. Even at a low temperature of −20 °C, high reversible capacities of 241 and 115 mA h g −1 can be obtained after 1000 cycles at 1 and 5 A g −1 , respectively. The outstanding electrochemical performance is attributed to the incorporation of K + into the layered V 2 O 5 , which acts as pillars to promote the Zn 2+ diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K + can benefit electron migration, and therefore enhance the Zn 2+ (de)intercalation kinetics. Meanwhile, the Zn 2+ storage mechanism of K 0.5 V 2 O 5 is revealed by ex situ X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs. Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn 2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K+ pre-intercalated layered V2O5 (K0.5V2O5) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K0.5V2O5 electrode delivers a high reversible capacity of 251 mA h g-1 at 5 A g-1 after 1000 cycles. Even at a low temperature of -20 °C, high reversible capacities of 241 and 115 mA h g-1 can be obtained after 1000 cycles at 1 and 5 A g-1, respectively. The outstanding electrochemical performance is attributed to the incorporation of K+ into the layered V2O5, which acts as pillars to promote the Zn2+ diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K+ can benefit electron migration, and therefore enhance the Zn2+ (de)intercalation kinetics. Meanwhile, the Zn2+ storage mechanism of K0.5V2O5 is revealed by ex situ X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs.Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K+ pre-intercalated layered V2O5 (K0.5V2O5) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K0.5V2O5 electrode delivers a high reversible capacity of 251 mA h g-1 at 5 A g-1 after 1000 cycles. Even at a low temperature of -20 °C, high reversible capacities of 241 and 115 mA h g-1 can be obtained after 1000 cycles at 1 and 5 A g-1, respectively. The outstanding electrochemical performance is attributed to the incorporation of K+ into the layered V2O5, which acts as pillars to promote the Zn2+ diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K+ can benefit electron migration, and therefore enhance the Zn2+ (de)intercalation kinetics. Meanwhile, the Zn2+ storage mechanism of K0.5V2O5 is revealed by ex situ X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs. Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate, long-term cycling and low-temperature properties. Herein, K+ pre-intercalated layered V2O5 (K0.5V2O5) composites with metallic features are capable of delivering excellent zinc storage performance. Specifically, the K0.5V2O5 electrode delivers a high reversible capacity of 251 mA h g−1 at 5 A g−1 after 1000 cycles. Even at a low temperature of −20 °C, high reversible capacities of 241 and 115 mA h g−1 can be obtained after 1000 cycles at 1 and 5 A g−1, respectively. The outstanding electrochemical performance is attributed to the incorporation of K+ into the layered V2O5, which acts as pillars to promote the Zn2+ diffusion and increase the structural stability during cycling. Density functional theory calculations demonstrate that the interlayer doping of K+ can benefit electron migration, and therefore enhance the Zn2+ (de)intercalation kinetics. Meanwhile, the Zn2+ storage mechanism of K0.5V2O5 is revealed by ex situ X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy characterization. This work may pave the way for exploiting high-performance cathodes for aqueous ZIBs. |
| Author | Dong, Huilong Su, Guang Chen, Shufeng Geng, Hongbo Cheng, Yafei Wei, Huaixin Liu, Quan Ang, Edison Huixiang Li, Cheng Chao |
| AuthorAffiliation | School of Materials Engineering Guangdong University of Technology Changshu Institute of Technology Nankai University College of Chemistry Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) School of Chemical Biology and Materials Engineering Suzhou University of Science and Technology Natural Sciences and Science Education Nanyang Technological University School of Chemical Engineering and Light Industry National Institute of Education |
| AuthorAffiliation_xml | – name: School of Chemical Biology and Materials Engineering – name: Natural Sciences and Science Education – name: National Institute of Education – name: School of Chemical Engineering and Light Industry – name: Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) – name: Changshu Institute of Technology – name: Guangdong University of Technology – name: Suzhou University of Science and Technology – name: School of Materials Engineering – name: College of Chemistry – name: Nanyang Technological University – name: Nankai University |
| Author_xml | – sequence: 1 givenname: Guang surname: Su fullname: Su, Guang – sequence: 2 givenname: Shufeng surname: Chen fullname: Chen, Shufeng – sequence: 3 givenname: Huilong surname: Dong fullname: Dong, Huilong – sequence: 4 givenname: Yafei surname: Cheng fullname: Cheng, Yafei – sequence: 5 givenname: Quan surname: Liu fullname: Liu, Quan – sequence: 6 givenname: Huaixin surname: Wei fullname: Wei, Huaixin – sequence: 7 givenname: Edison Huixiang surname: Ang fullname: Ang, Edison Huixiang – sequence: 8 givenname: Hongbo surname: Geng fullname: Geng, Hongbo – sequence: 9 givenname: Cheng Chao surname: Li fullname: Li, Cheng Chao |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33491718$$D View this record in MEDLINE/PubMed |
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| Snippet | Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn
2+
diffusion kinetics, continue to face challenges in terms of achieving superior high rate,... Aqueous zinc-ion batteries (ZIBs), due to their sluggish Zn2+ diffusion kinetics, continue to face challenges in terms of achieving superior high rate,... |
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| SubjectTerms | Cycles Density functional theory Diffusion layers Electrochemical analysis Electron microscopy Electronic structure Intercalation Interlayers Kinetics Low temperature Microscopy Photoelectrons Rechargeable batteries Structural stability Vanadium pentoxide |
| Title | Tuning the electronic structure of layered vanadium pentoxide by pre-intercalation of potassium ions for superior room/low-temperature aqueous zinc-ion batteries |
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