Construction of S-scheme Bi2WO6/g-C3N4 heterostructure nanosheets with enhanced visible-light photocatalytic degradation for ammonium dinitramide
Photocatalysis technology is considered as a promising environmental remediation strategy. Herein, photocatalytic degradation of ammonium dinitramide (ADN, main component of propellant) was investigated over Bi2WO6/g-C3N4 (BWO/CN) heterostructure nanosheets prepared by a one-step in-situ hydrotherma...
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| Published in | Journal of hazardous materials Vol. 412; p. 125217 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.06.2021
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| Subjects | |
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| Abstract | Photocatalysis technology is considered as a promising environmental remediation strategy. Herein, photocatalytic degradation of ammonium dinitramide (ADN, main component of propellant) was investigated over Bi2WO6/g-C3N4 (BWO/CN) heterostructure nanosheets prepared by a one-step in-situ hydrothermal method. The operating conditions including ADN initial concentration, catalyst dosage, initial pH, temperature and green oxidizer (hydrogen peroxide) were optimized systematically. Under optimal conditions, the photocatalytic degradation rate of ADN over BWO/CN can reach 98.93% after 80 min visible-light irradiation. Besides, the composite has excellent stability for ADN treatment and nitrate ions are the major degradation products. Furthermore, S-scheme heterojunction mechanism was proposed to explain the extremely high REDOX performance of BWO/CN composite.
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•Bi2WO6/g-C3N4 composites were fabricated by a hydrothermal method.•Photocatalytic degradation of ADN was investigated over Bi2WO6/g-C3N4.•The highest degradation rate reaches 98.93% under optimal conditions.•The main degradation products are nitrate ions.•S-scheme charge transfer mechanism was proposed. |
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| AbstractList | Photocatalysis technology is considered as a promising environmental remediation strategy. Herein, photocatalytic degradation of ammonium dinitramide (ADN, main component of propellant) was investigated over Bi2WO6/g-C3N4 (BWO/CN) heterostructure nanosheets prepared by a one-step in-situ hydrothermal method. The operating conditions including ADN initial concentration, catalyst dosage, initial pH, temperature and green oxidizer (hydrogen peroxide) were optimized systematically. Under optimal conditions, the photocatalytic degradation rate of ADN over BWO/CN can reach 98.93% after 80 min visible-light irradiation. Besides, the composite has excellent stability for ADN treatment and nitrate ions are the major degradation products. Furthermore, S-scheme heterojunction mechanism was proposed to explain the extremely high REDOX performance of BWO/CN composite.
[Display omitted]
•Bi2WO6/g-C3N4 composites were fabricated by a hydrothermal method.•Photocatalytic degradation of ADN was investigated over Bi2WO6/g-C3N4.•The highest degradation rate reaches 98.93% under optimal conditions.•The main degradation products are nitrate ions.•S-scheme charge transfer mechanism was proposed. Photocatalysis technology is considered as a promising environmental remediation strategy. Herein, photocatalytic degradation of ammonium dinitramide (ADN, main component of propellant) was investigated over Bi2WO6/g-C3N4 (BWO/CN) heterostructure nanosheets prepared by a one-step in-situ hydrothermal method. The operating conditions including ADN initial concentration, catalyst dosage, initial pH, temperature and green oxidizer (hydrogen peroxide) were optimized systematically. Under optimal conditions, the photocatalytic degradation rate of ADN over BWO/CN can reach 98.93% after 80 min visible-light irradiation. Besides, the composite has excellent stability for ADN treatment and nitrate ions are the major degradation products. Furthermore, S-scheme heterojunction mechanism was proposed to explain the extremely high REDOX performance of BWO/CN composite.Photocatalysis technology is considered as a promising environmental remediation strategy. Herein, photocatalytic degradation of ammonium dinitramide (ADN, main component of propellant) was investigated over Bi2WO6/g-C3N4 (BWO/CN) heterostructure nanosheets prepared by a one-step in-situ hydrothermal method. The operating conditions including ADN initial concentration, catalyst dosage, initial pH, temperature and green oxidizer (hydrogen peroxide) were optimized systematically. Under optimal conditions, the photocatalytic degradation rate of ADN over BWO/CN can reach 98.93% after 80 min visible-light irradiation. Besides, the composite has excellent stability for ADN treatment and nitrate ions are the major degradation products. Furthermore, S-scheme heterojunction mechanism was proposed to explain the extremely high REDOX performance of BWO/CN composite. Photocatalysis technology is considered as a promising environmental remediation strategy. Herein, photocatalytic degradation of ammonium dinitramide (ADN, main component of propellant) was investigated over Bi₂WO₆/g-C₃N₄ (BWO/CN) heterostructure nanosheets prepared by a one-step in-situ hydrothermal method. The operating conditions including ADN initial concentration, catalyst dosage, initial pH, temperature and green oxidizer (hydrogen peroxide) were optimized systematically. Under optimal conditions, the photocatalytic degradation rate of ADN over BWO/CN can reach 98.93% after 80 min visible-light irradiation. Besides, the composite has excellent stability for ADN treatment and nitrate ions are the major degradation products. Furthermore, S-scheme heterojunction mechanism was proposed to explain the extremely high REDOX performance of BWO/CN composite. |
| ArticleNumber | 125217 |
| Author | Dong, Shuai Xue, Wenhua Li, Hui Liu, Enzhou Xu, Kangzhen Lian, Xiaoyan |
| Author_xml | – sequence: 1 givenname: Xiaoyan surname: Lian fullname: Lian, Xiaoyan organization: School of Chemical Engineering/Xi’an Key Laboratory of Special Energy Materials, Northwest University, Xi’an 710069, China – sequence: 2 givenname: Wenhua surname: Xue fullname: Xue, Wenhua organization: School of Chemical Engineering/Xi’an Key Laboratory of Special Energy Materials, Northwest University, Xi’an 710069, China – sequence: 3 givenname: Shuai surname: Dong fullname: Dong, Shuai organization: School of Chemical Engineering/Xi’an Key Laboratory of Special Energy Materials, Northwest University, Xi’an 710069, China – sequence: 4 givenname: Enzhou surname: Liu fullname: Liu, Enzhou organization: School of Chemical Engineering/Xi’an Key Laboratory of Special Energy Materials, Northwest University, Xi’an 710069, China – sequence: 5 givenname: Hui surname: Li fullname: Li, Hui organization: Xi’an Modern Chemistry Research Institute, Xi’an 710065, China – sequence: 6 givenname: Kangzhen surname: Xu fullname: Xu, Kangzhen email: xukz@nwu.edu.cn organization: School of Chemical Engineering/Xi’an Key Laboratory of Special Energy Materials, Northwest University, Xi’an 710069, China |
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| SubjectTerms | ammonium Ammonium dinitramide Bi2WO6 catalysts G-C3N4 hot water treatment hydrogen peroxide irradiation light nanosheets nitrates oxidants Photocatalysis remediation S-scheme temperature |
| Title | Construction of S-scheme Bi2WO6/g-C3N4 heterostructure nanosheets with enhanced visible-light photocatalytic degradation for ammonium dinitramide |
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