Decoupled aqueous batteries using pH-decoupling electrolytes

Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, whic...

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Published inNature reviews. Chemistry Vol. 6; no. 7; pp. 505 - 517
Main Authors Zhu, Yun-hai, Cui, Yang-feng, Xie, Zi-long, Zhuang, Zhen-bang, Huang, Gang, Zhang, Xin-bo
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 01.07.2022
Nature Publishing Group
Subjects
639/301/299/891
639/4077/4079/891
639/638/161/891
Analytical Chemistry
Anolytes
Aqueous electrolytes
Biochemistry
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Decoupling
Electrolytes
Inorganic Chemistry
Lithium
Lithium batteries
Organic Chemistry
Physical Chemistry
Rechargeable batteries
Review Article
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Abstract Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, which theoretically impedes further improvement of their energy density. However, the pH-decoupling electrolyte with an acidic catholyte and an alkaline anolyte has been verified to broaden the operating voltage window of the aqueous electrolyte to over 3 V, which goes beyond the voltage limitations of the aqueous batteries, making high-energy aqueous batteries possible. In this Review, we summarize the latest decoupled aqueous batteries based on pH-decoupling electrolytes from the perspective of ion-selective membranes, competitive redox couples and potential battery prototypes. The inherent defects and problems of these decoupled aqueous batteries are systematically analysed, and the critical scientific issues of this battery technology for future applications are discussed. Developing aqueous batteries with high voltages is possible with the use of pH-decoupling electrolytes with an acidic catholyte and an alkaline anolyte.
AbstractList Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, which theoretically impedes further improvement of their energy density. However, the pH-decoupling electrolyte with an acidic catholyte and an alkaline anolyte has been verified to broaden the operating voltage window of the aqueous electrolyte to over 3 V, which goes beyond the voltage limitations of the aqueous batteries, making high-energy aqueous batteries possible. In this Review, we summarize the latest decoupled aqueous batteries based on pH-decoupling electrolytes from the perspective of ion-selective membranes, competitive redox couples and potential battery prototypes. The inherent defects and problems of these decoupled aqueous batteries are systematically analysed, and the critical scientific issues of this battery technology for future applications are discussed.Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, which theoretically impedes further improvement of their energy density. However, the pH-decoupling electrolyte with an acidic catholyte and an alkaline anolyte has been verified to broaden the operating voltage window of the aqueous electrolyte to over 3 V, which goes beyond the voltage limitations of the aqueous batteries, making high-energy aqueous batteries possible. In this Review, we summarize the latest decoupled aqueous batteries based on pH-decoupling electrolytes from the perspective of ion-selective membranes, competitive redox couples and potential battery prototypes. The inherent defects and problems of these decoupled aqueous batteries are systematically analysed, and the critical scientific issues of this battery technology for future applications are discussed.
Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, which theoretically impedes further improvement of their energy density. However, the pH-decoupling electrolyte with an acidic catholyte and an alkaline anolyte has been verified to broaden the operating voltage window of the aqueous electrolyte to over 3 V, which goes beyond the voltage limitations of the aqueous batteries, making high-energy aqueous batteries possible. In this Review, we summarize the latest decoupled aqueous batteries based on pH-decoupling electrolytes from the perspective of ion-selective membranes, competitive redox couples and potential battery prototypes. The inherent defects and problems of these decoupled aqueous batteries are systematically analysed, and the critical scientific issues of this battery technology for future applications are discussed.
Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, which theoretically impedes further improvement of their energy density. However, the pH-decoupling electrolyte with an acidic catholyte and an alkaline anolyte has been verified to broaden the operating voltage window of the aqueous electrolyte to over 3 V, which goes beyond the voltage limitations of the aqueous batteries, making high-energy aqueous batteries possible. In this Review, we summarize the latest decoupled aqueous batteries based on pH-decoupling electrolytes from the perspective of ion-selective membranes, competitive redox couples and potential battery prototypes. The inherent defects and problems of these decoupled aqueous batteries are systematically analysed, and the critical scientific issues of this battery technology for future applications are discussed.Developing aqueous batteries with high voltages is possible with the use of pH-decoupling electrolytes with an acidic catholyte and an alkaline anolyte.
Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost, abundant resources and high safety. The output voltage of aqueous batteries is limited by the narrow stable voltage window of 1.23 V for water, which theoretically impedes further improvement of their energy density. However, the pH-decoupling electrolyte with an acidic catholyte and an alkaline anolyte has been verified to broaden the operating voltage window of the aqueous electrolyte to over 3 V, which goes beyond the voltage limitations of the aqueous batteries, making high-energy aqueous batteries possible. In this Review, we summarize the latest decoupled aqueous batteries based on pH-decoupling electrolytes from the perspective of ion-selective membranes, competitive redox couples and potential battery prototypes. The inherent defects and problems of these decoupled aqueous batteries are systematically analysed, and the critical scientific issues of this battery technology for future applications are discussed. Developing aqueous batteries with high voltages is possible with the use of pH-decoupling electrolytes with an acidic catholyte and an alkaline anolyte.
Author Zhu, Yun-hai
Xie, Zi-long
Huang, Gang
Zhuang, Zhen-bang
Cui, Yang-feng
Zhang, Xin-bo
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  surname: Zhu
  fullname: Zhu, Yun-hai
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  givenname: Yang-feng
  surname: Cui
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  organization: State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, School of Materials Science and Engineering, Changchun University of Science and Technology
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  orcidid: 0000-0002-9937-6862
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  fullname: Xie, Zi-long
  organization: State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, University of Science and Technology of China
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  givenname: Zhen-bang
  surname: Zhuang
  fullname: Zhuang, Zhen-bang
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  orcidid: 0000-0003-2518-8145
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  givenname: Xin-bo
  orcidid: 0000-0002-5806-159X
  surname: Zhang
  fullname: Zhang, Xin-bo
  email: xbzhang@ciac.ac.cn
  organization: State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, University of Science and Technology of China
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Snippet Aqueous batteries have been considered as the most promising alternatives to the dominant lithium-based battery technologies because of their low cost,...
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SubjectTerms 639/301/299/891
639/4077/4079/891
639/638/161/891
Analytical Chemistry
Anolytes
Aqueous electrolytes
Biochemistry
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Decoupling
Electrolytes
Inorganic Chemistry
Lithium
Lithium batteries
Organic Chemistry
Physical Chemistry
Rechargeable batteries
Review Article
Title Decoupled aqueous batteries using pH-decoupling electrolytes
URI https://link.springer.com/article/10.1038/s41570-022-00397-3
https://www.ncbi.nlm.nih.gov/pubmed/37117314
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