Solvation of ions in helium

We review the solvation of atomic, molecular or cluster ions in HNDs. After briefly discussing the properties of snowballs in bulk helium we consider experimental conditions for the efficient synthesis of charged, doped HNDs. We show that the cluster ions observed in conventional mass spectrometers...

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Published inInternational reviews in physical chemistry Vol. 39; no. 4; pp. 465 - 516
Main Authors González-Lezana, Tomás, Echt, Olof, Gatchell, Michael, Bartolomei, Massimiliano, Campos-Martínez, José, Scheier, Paul
Format Journal Article
LanguageEnglish
Published Abingdon Taylor & Francis 01.10.2020
Taylor & Francis Ltd
Subjects
Anomalies
Aromatic hydrocarbons
Clusters
Excitation spectra
Fluids
Helium
Mass spectrometers
Solvation
Submerging
Superfluidity
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Abstract We review the solvation of atomic, molecular or cluster ions in HNDs. After briefly discussing the properties of snowballs in bulk helium we consider experimental conditions for the efficient synthesis of charged, doped HNDs. We show that the cluster ions observed in conventional mass spectrometers originate from fission of highly charged HNDs. The ionization threshold of HNDs doped with alkalis reveals the minimum cluster size required for full immersion. The abundance distributions of He X ions frequently reveal local anomalies or magic numbers. We demonstrate that the abundance is approximately proportional to the evaporation energy. Observed and calculated magic numbers will be compiled, including data for ions solvated in molecular hydrogen. Alternative methods to forming He X that do not employ HNDs will be summarized. Electronic excitation spectra of C and polycyclic aromatic hydrocarbon ions reveal the properties of the helium adsorption layer in quantitative detail. Next we discuss theoretical efforts to describe the interaction between ions and helium. We close with summarizing the size dependence of physical quantities computed for atomic alkali and alkaline earth cations in helium, such as binding energy, superfluid fraction, structural order, radial density profiles, and the existence of first and higher solvation shells.
AbstractList We review the solvation of atomic, molecular or cluster ions in HNDs. After briefly discussing the properties of snowballs in bulk helium we consider experimental conditions for the efficient synthesis of charged, doped HNDs. We show that the cluster ions observed in conventional mass spectrometers originate from fission of highly charged HNDs. The ionization threshold of HNDs doped with alkalis reveals the minimum cluster size required for full immersion. The abundance distributions of HeNX +/- ions frequently reveal local anomalies or magic numbers. We demonstrate that the abundance is approximately proportional to the evaporation energy. Observed and calculated magic numbers will be compiled, including data for ions solvated in molecular hydrogen. Alternative methods to forming HeNX+ that do not employ HNDs will be summarized. Electronic excitation spectra of C-60(+) and polycyclic aromatic hydrocarbon ions reveal the properties of the helium adsorption layer in quantitative detail. Next we discuss theoretical efforts to describe the interaction between ions and helium. We close with summarizing the size dependence of physical quantities computed for atomic alkali and alkaline earth cations in helium, such as binding energy, superfluid fraction, structural order, radial density profiles, and the existence of first and higher solvation shells.
We review the solvation of atomic, molecular or cluster ions in HNDs. After briefly discussing the properties of snowballs in bulk helium we consider experimental conditions for the efficient synthesis of charged, doped HNDs. We show that the cluster ions observed in conventional mass spectrometers originate from fission of highly charged HNDs. The ionization threshold of HNDs doped with alkalis reveals the minimum cluster size required for full immersion. The abundance distributions of HeX ions frequently reveal local anomalies or magic numbers. We demonstrate that the abundance is approximately proportional to the evaporation energy. Observed and calculated magic numbers will be compiled, including data for ions solvated in molecular hydrogen. Alternative methods to forming HeX that do not employ HNDs will be summarized. Electronic excitation spectra of C and polycyclic aromatic hydrocarbon ions reveal the properties of the helium adsorption layer in quantitative detail. Next we discuss theoretical efforts to describe the interaction between ions and helium. We close with summarizing the size dependence of physical quantities computed for atomic alkali and alkaline earth cations in helium, such as binding energy, superfluid fraction, structural order, radial density profiles, and the existence of first and higher solvation shells.
We review the solvation of atomic, molecular or cluster ions in HNDs. After briefly discussing the properties of snowballs in bulk helium we consider experimental conditions for the efficient synthesis of charged, doped HNDs. We show that the cluster ions observed in conventional mass spectrometers originate from fission of highly charged HNDs. The ionization threshold of HNDs doped with alkalis reveals the minimum cluster size required for full immersion. The abundance distributions of He X ions frequently reveal local anomalies or magic numbers. We demonstrate that the abundance is approximately proportional to the evaporation energy. Observed and calculated magic numbers will be compiled, including data for ions solvated in molecular hydrogen. Alternative methods to forming He X that do not employ HNDs will be summarized. Electronic excitation spectra of C and polycyclic aromatic hydrocarbon ions reveal the properties of the helium adsorption layer in quantitative detail. Next we discuss theoretical efforts to describe the interaction between ions and helium. We close with summarizing the size dependence of physical quantities computed for atomic alkali and alkaline earth cations in helium, such as binding energy, superfluid fraction, structural order, radial density profiles, and the existence of first and higher solvation shells.
Author Scheier, Paul
Campos-Martínez, José
González-Lezana, Tomás
Gatchell, Michael
Bartolomei, Massimiliano
Echt, Olof
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  surname: González-Lezana
  fullname: González-Lezana, Tomás
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  organization: Instituto de Física Fundamental, Consejo Superior de Investigaciones Científicas IFF-CSIC
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  givenname: Olof
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  surname: Echt
  fullname: Echt, Olof
  organization: Department of Physics, University of New Hampshire
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  givenname: Michael
  orcidid: 0000-0003-1028-7976
  surname: Gatchell
  fullname: Gatchell, Michael
  organization: Department of Physics, Stockholm University
– sequence: 4
  givenname: Massimiliano
  orcidid: 0000-0001-8643-4106
  surname: Bartolomei
  fullname: Bartolomei, Massimiliano
  organization: Instituto de Física Fundamental, Consejo Superior de Investigaciones Científicas IFF-CSIC
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  givenname: José
  orcidid: 0000-0002-8848-6353
  surname: Campos-Martínez
  fullname: Campos-Martínez, José
  organization: Instituto de Física Fundamental, Consejo Superior de Investigaciones Científicas IFF-CSIC
– sequence: 6
  givenname: Paul
  orcidid: 0000-0002-7480-6205
  surname: Scheier
  fullname: Scheier, Paul
  organization: Institut für Ionenphysik und Angewandte Physik, Universität Innsbruck
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Copyright 2020 Informa UK Limited, trading as Taylor & Francis Group 2020
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Snippet We review the solvation of atomic, molecular or cluster ions in HNDs. After briefly discussing the properties of snowballs in bulk helium we consider...
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SubjectTerms Anomalies
Aromatic hydrocarbons
Clusters
Excitation spectra
Fluids
Helium
Mass spectrometers
Solvation
Submerging
Superfluidity
Title Solvation of ions in helium
URI https://www.tandfonline.com/doi/abs/10.1080/0144235X.2020.1794585
https://www.proquest.com/docview/2456813652
https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-185282
Volume 39
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