Buried interface molecular hybrid for inverted perovskite solar cells

Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of t...

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Published in	Nature (London) Vol. 632; no. 8025; pp. 536 - 542
Main Authors	Liu, Sanwan, Li, Jingbai, Xiao, Wenshan, Chen, Rui, Sun, Zhenxing, Zhang, Yong, Lei, Xia, Hu, Shuaifeng, Kober-Czerny, Manuel, Wang, Jianan, Ren, Fumeng, Zhou, Qisen, Raza, Hasan, Gao, You, Ji, Yitong, Li, Sibo, Li, Huan, Qiu, Longbin, Huang, Wenchao, Zhao, Yan, Xu, Baomin, Liu, Zonghao, Snaith, Henry J., Park, Nam-Gyu, Chen, Wei
Format	Journal Article
Language	English
Published	London Nature Publishing Group UK 15.08.2024 Nature Publishing Group
Subjects	119/118 639/301 639/301/299 639/301/299/946 Acids Antibiotics Buried structures Carboxylic acids Efficiency Energy conversion efficiency Heterojunctions Humanities and Social Sciences Interface stability Interfaces Molecular structure Morphology multidisciplinary Perovskites Phosphonic acids Photovoltaic cells Photovoltaics Scanning electron microscopy Science Science (multidisciplinary) Self-assembly Solar cells Wettability
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Abstract	Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of the inverted perovskite solar cells have exceeded 25% owing to the development of improved self-assembled molecules 1 – 5 and passivation strategies 6 – 8 . However, poor wettability and agglomeration of self-assembled molecules 9 – 12 cause interfacial losses, impeding further improvement in the power conversion efficiency and stability. Here we report a molecular hybrid at the buried interface in inverted perovskite solar cells that co-assembled the popular self-assembled molecule [4-(3,6-dimethyl-9 H -carbazol-9-yl)butyl]phosphonic acid (Me-4PACz) with the multiple aromatic carboxylic acid 4,4′,4″-nitrilotribenzoic acid (NA) to improve the heterojunction interface. The molecular hybrid of Me-4PACz with NA could substantially improve the interfacial characteristics. The resulting inverted perovskite solar cells demonstrated a record certified steady-state efficiency of 26.54%. Crucially, this strategy aligns seamlessly with large-scale manufacturing, achieving one of the highest certified power conversion efficiencies for inverted mini-modules at 22.74% (aperture area 11.1 cm 2 ). Our device also maintained 96.1% of its initial power conversion efficiency after more than 2,400 h of 1-sun operation in ambient air. High efficiency in perovskite solar cells is achieved by using a molecular hybrid of a self-assembled monolayer with nitrilotribenzoic acid.
AbstractList	Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of the inverted perovskite solar cells have exceeded 25% owing to the development of improved self-assembled molecules 1 – 5 and passivation strategies 6 – 8 . However, poor wettability and agglomeration of self-assembled molecules 9 – 12 cause interfacial losses, impeding further improvement in the power conversion efficiency and stability. Here we report a molecular hybrid at the buried interface in inverted perovskite solar cells that co-assembled the popular self-assembled molecule [4-(3,6-dimethyl-9 H -carbazol-9-yl)butyl]phosphonic acid (Me-4PACz) with the multiple aromatic carboxylic acid 4,4′,4″-nitrilotribenzoic acid (NA) to improve the heterojunction interface. The molecular hybrid of Me-4PACz with NA could substantially improve the interfacial characteristics. The resulting inverted perovskite solar cells demonstrated a record certified steady-state efficiency of 26.54%. Crucially, this strategy aligns seamlessly with large-scale manufacturing, achieving one of the highest certified power conversion efficiencies for inverted mini-modules at 22.74% (aperture area 11.1 cm 2 ). Our device also maintained 96.1% of its initial power conversion efficiency after more than 2,400 h of 1-sun operation in ambient air. High efficiency in perovskite solar cells is achieved by using a molecular hybrid of a self-assembled monolayer with nitrilotribenzoic acid. Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of the inverted perovskite solar cells have exceeded 25% owing to the development of improved self-assembled molecules1-5 and passivation strategies6-8. However, poor wettability and agglomeration of self-assembled molecules9-12 cause interfacial losses, impeding further improvement in the power conversion efficiency and stability. Here we report a molecular hybrid at the buried interface in inverted perovskite solar cells that co-assembled the popular self-assembled molecule [4-(3,6-dimethyl-9H-carbazol-9-yl)butyl]phosphonic acid (Me-4PACz) with the multiple aromatic carboxylic acid 4,4',4″-nitrilotribenzoic acid (NA) to improve the heterojunction interface. The molecular hybrid of Me-4PACz with NA could substantially improve the interfacial characteristics. The resulting inverted perovskite solar cells demonstrated a record certified steady-state efficiency of 26.54%. Crucially, this strategy aligns seamlessly with large-scale manufacturing, achieving one of the highest certified power conversion efficiencies for inverted mini-modules at 22.74% (aperture area 11.1 cm2). Our device also maintained 96.1% of its initial power conversion efficiency after more than 2,400 h of 1-sun operation in ambient air.Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of the inverted perovskite solar cells have exceeded 25% owing to the development of improved self-assembled molecules1-5 and passivation strategies6-8. However, poor wettability and agglomeration of self-assembled molecules9-12 cause interfacial losses, impeding further improvement in the power conversion efficiency and stability. Here we report a molecular hybrid at the buried interface in inverted perovskite solar cells that co-assembled the popular self-assembled molecule [4-(3,6-dimethyl-9H-carbazol-9-yl)butyl]phosphonic acid (Me-4PACz) with the multiple aromatic carboxylic acid 4,4',4″-nitrilotribenzoic acid (NA) to improve the heterojunction interface. The molecular hybrid of Me-4PACz with NA could substantially improve the interfacial characteristics. The resulting inverted perovskite solar cells demonstrated a record certified steady-state efficiency of 26.54%. Crucially, this strategy aligns seamlessly with large-scale manufacturing, achieving one of the highest certified power conversion efficiencies for inverted mini-modules at 22.74% (aperture area 11.1 cm2). Our device also maintained 96.1% of its initial power conversion efficiency after more than 2,400 h of 1-sun operation in ambient air. Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of the inverted perovskite solar cells have exceeded 25% owing to the development of improved self-assembled molecules and passivation strategies . However, poor wettability and agglomeration of self-assembled molecules cause interfacial losses, impeding further improvement in the power conversion efficiency and stability. Here we report a molecular hybrid at the buried interface in inverted perovskite solar cells that co-assembled the popular self-assembled molecule [4-(3,6-dimethyl-9H-carbazol-9-yl)butyl]phosphonic acid (Me-4PACz) with the multiple aromatic carboxylic acid 4,4',4″-nitrilotribenzoic acid (NA) to improve the heterojunction interface. The molecular hybrid of Me-4PACz with NA could substantially improve the interfacial characteristics. The resulting inverted perovskite solar cells demonstrated a record certified steady-state efficiency of 26.54%. Crucially, this strategy aligns seamlessly with large-scale manufacturing, achieving one of the highest certified power conversion efficiencies for inverted mini-modules at 22.74% (aperture area 11.1 cm ). Our device also maintained 96.1% of its initial power conversion efficiency after more than 2,400 h of 1-sun operation in ambient air. Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better power conversion efficiency and operational stability compared with the normal device structure. Specifically, power conversion efficiencies of the inverted perovskite solar cells have exceeded 25% owing to the development of improved self-assembled molecules1-5 and passivation strategies6-8. However, poor wettability and agglomeration of self-assembled molecules9-12 cause interfacial losses, impeding further improvement in the power conversion efficiency and stability. Here we report a molecular hybrid at the buried interface in inverted perovskite solar cells that со-assembled the popular self-assembled molecule [4-(3,6-dimethyl-9H-carbazol-9-yl)butyl]phosphonic acid (Me-4PACz) with the multiple aromatic carboxylic acid 4,4',4"-nitrilotribenzoic acid (NA) to improve the heterojunction interface. The molecular hybrid of Me-4PACz with NA could substantially improve the interfacial characteristics. The resulting inverted perovskite solar cells demonstrated a record certified steady-state efficiency of 26.54%. Crucially, this strategy aligns seamlessly with large-scale manufacturing, achieving one of the highest certified power conversion efficiencies for inverted mini-modules at 22.74% (aperture area 11.1 cm2). Our device also maintained 96.1% of its initial power conversion efficiency after more than 2,400 h of 1-sun operation in ambient air.
Author	Liu, Zonghao Xiao, Wenshan Wang, Jianan Kober-Czerny, Manuel Huang, Wenchao Ji, Yitong Li, Sibo Hu, Shuaifeng Xu, Baomin Zhou, Qisen Lei, Xia Ren, Fumeng Snaith, Henry J. Liu, Sanwan Gao, You Li, Jingbai Qiu, Longbin Park, Nam-Gyu Raza, Hasan Li, Huan Chen, Rui Sun, Zhenxing Chen, Wei Zhao, Yan Zhang, Yong
Author_xml	– sequence: 1 givenname: Sanwan surname: Liu fullname: Liu, Sanwan organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST), Optics Valley Laboratory – sequence: 2 givenname: Jingbai orcidid: 0000-0003-4743-0318 surname: Li fullname: Li, Jingbai organization: Hoffmann Institute of Advanced Materials, Shenzhen Polytechnic University – sequence: 3 givenname: Wenshan surname: Xiao fullname: Xiao, Wenshan organization: Key State Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology – sequence: 4 givenname: Rui surname: Chen fullname: Chen, Rui organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 5 givenname: Zhenxing surname: Sun fullname: Sun, Zhenxing organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 6 givenname: Yong orcidid: 0009-0008-5570-5637 surname: Zhang fullname: Zhang, Yong organization: Department of Materials Science and Engineering, Southern University of Science and Technology – sequence: 7 givenname: Xia orcidid: 0009-0001-6499-2745 surname: Lei fullname: Lei, Xia organization: Hoffmann Institute of Advanced Materials, Shenzhen Polytechnic University, Department of Materials Science and Engineering, Southern University of Science and Technology – sequence: 8 givenname: Shuaifeng orcidid: 0000-0003-1312-075X surname: Hu fullname: Hu, Shuaifeng organization: Clarendon Laboratory, Department of Physics, University of Oxford – sequence: 9 givenname: Manuel orcidid: 0000-0002-7807-3133 surname: Kober-Czerny fullname: Kober-Czerny, Manuel organization: Clarendon Laboratory, Department of Physics, University of Oxford – sequence: 10 givenname: Jianan surname: Wang fullname: Wang, Jianan organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 11 givenname: Fumeng surname: Ren fullname: Ren, Fumeng organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 12 givenname: Qisen surname: Zhou fullname: Zhou, Qisen organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 13 givenname: Hasan orcidid: 0009-0006-5653-9197 surname: Raza fullname: Raza, Hasan organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 14 givenname: You surname: Gao fullname: Gao, You organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST) – sequence: 15 givenname: Yitong surname: Ji fullname: Ji, Yitong organization: Key State Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology – sequence: 16 givenname: Sibo surname: Li fullname: Li, Sibo organization: Shenzhen Key Laboratory of Intelligent Robotics and Flexible Manufacturing Systems, Department of Mechanical and Energy Engineering, SUSTech Energy Institute for Carbon Neutrality, Southern University of Science and Technology – sequence: 17 givenname: Huan surname: Li fullname: Li, Huan organization: Shenzhen Key Laboratory of Intelligent Robotics and Flexible Manufacturing Systems, Department of Mechanical and Energy Engineering, SUSTech Energy Institute for Carbon Neutrality, Southern University of Science and Technology – sequence: 18 givenname: Longbin orcidid: 0000-0002-7696-4901 surname: Qiu fullname: Qiu, Longbin organization: Shenzhen Key Laboratory of Intelligent Robotics and Flexible Manufacturing Systems, Department of Mechanical and Energy Engineering, SUSTech Energy Institute for Carbon Neutrality, Southern University of Science and Technology – sequence: 19 givenname: Wenchao orcidid: 0000-0003-4992-1727 surname: Huang fullname: Huang, Wenchao organization: Key State Laboratory of Advanced Technology for Materials Synthesis and Processing, School of Materials Science and Engineering, Wuhan University of Technology, Hubei Longzhong Laboratory, Wuhan University of Technology Xiangyang Demonstration Zone – sequence: 20 givenname: Yan orcidid: 0000-0002-1234-4455 surname: Zhao fullname: Zhao, Yan organization: College of Materials Science and Engineering, Sichuan University, The Institute of Technological Sciences, Wuhan University – sequence: 21 givenname: Baomin orcidid: 0000-0002-2868-0613 surname: Xu fullname: Xu, Baomin organization: Department of Materials Science and Engineering, Southern University of Science and Technology – sequence: 22 givenname: Zonghao orcidid: 0000-0003-4743-6971 surname: Liu fullname: Liu, Zonghao email: liuzonghao@hust.edu.cn organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST), Optics Valley Laboratory – sequence: 23 givenname: Henry J. orcidid: 0000-0001-8511-790X surname: Snaith fullname: Snaith, Henry J. organization: Clarendon Laboratory, Department of Physics, University of Oxford – sequence: 24 givenname: Nam-Gyu orcidid: 0000-0003-2368-6300 surname: Park fullname: Park, Nam-Gyu email: npark@skku.edu organization: School of Chemical Engineering and Center for Antibonding Regulated Crystals, Sungkyunkwan University (SKKU), SKKU Institute of Energy Science and Technology (SIEST), Sungkyunkwan University – sequence: 25 givenname: Wei orcidid: 0000-0002-2418-9210 surname: Chen fullname: Chen, Wei email: wnlochenwei@hust.edu.cn organization: Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology (HUST), Optics Valley Laboratory
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/38925147$$D View this record in MEDLINE/PubMed
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Snippet	Perovskite solar cells with an inverted architecture provide a key pathway for commercializing this emerging photovoltaic technology because of the better...
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SubjectTerms	119/118 639/301 639/301/299 639/301/299/946 Acids Antibiotics Buried structures Carboxylic acids Efficiency Energy conversion efficiency Heterojunctions Humanities and Social Sciences Interface stability Interfaces Molecular structure Morphology multidisciplinary Perovskites Phosphonic acids Photovoltaic cells Photovoltaics Scanning electron microscopy Science Science (multidisciplinary) Self-assembly Solar cells Wettability
Title	Buried interface molecular hybrid for inverted perovskite solar cells
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