Synthetic effect of supports in Cu-Mn–doped oxide catalysts for promoting ozone decomposition under humid environment
The escalating levels of surface ozone concentration pose detrimental effects on public health and the environment. Catalytic decomposition presents an optimal solution for surface ozone removal. Nevertheless, catalyst still encounters challenges such as poisoning and deactivation in the high humidi...
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Published in | Environmental science and pollution research international Vol. 30; no. 46; pp. 102880 - 102893 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.10.2023
Springer Nature B.V |
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Abstract | The escalating levels of surface ozone concentration pose detrimental effects on public health and the environment. Catalytic decomposition presents an optimal solution for surface ozone removal. Nevertheless, catalyst still encounters challenges such as poisoning and deactivation in the high humidity environment. The influence of support on catalytic ozone decomposition was examined at a gas hourly space velocity of 300 L·g
−1
·h
−1
and 85% relative humidity under ambient temperature using Cu-Mn–doped oxide catalysts synthesized via a straightforward coprecipitation method. Notably, the Cu-Mn/SiO
2
catalyst exhibited remarkable performance on ozone decomposition, achieving 98% ozone conversion and stability for 10 h. Further characterization analysis indicated that the catalyst’s enhanced water resistance and activity could be attributed to factors such as an increased number of active sites, a large surface area, abundant active oxygen species, and a lower Mn oxidation state. The catalytic environment created by mixed oxides can offer a clearer understanding of their synergistic effects on catalytic ozone decomposition, providing significant insights into the development of water-resistant catalysts with superior performance.
Graphical Abstract |
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AbstractList | The escalating levels of surface ozone concentration pose detrimental effects on public health and the environment. Catalytic decomposition presents an optimal solution for surface ozone removal. Nevertheless, catalyst still encounters challenges such as poisoning and deactivation in the high humidity environment. The influence of support on catalytic ozone decomposition was examined at a gas hourly space velocity of 300 L·g
·h
and 85% relative humidity under ambient temperature using Cu-Mn-doped oxide catalysts synthesized via a straightforward coprecipitation method. Notably, the Cu-Mn/SiO
catalyst exhibited remarkable performance on ozone decomposition, achieving 98% ozone conversion and stability for 10 h. Further characterization analysis indicated that the catalyst's enhanced water resistance and activity could be attributed to factors such as an increased number of active sites, a large surface area, abundant active oxygen species, and a lower Mn oxidation state. The catalytic environment created by mixed oxides can offer a clearer understanding of their synergistic effects on catalytic ozone decomposition, providing significant insights into the development of water-resistant catalysts with superior performance. The escalating levels of surface ozone concentration pose detrimental effects on public health and the environment. Catalytic decomposition presents an optimal solution for surface ozone removal. Nevertheless, catalyst still encounters challenges such as poisoning and deactivation in the high humidity environment. The influence of support on catalytic ozone decomposition was examined at a gas hourly space velocity of 300 L·g−1·h−1 and 85% relative humidity under ambient temperature using Cu-Mn–doped oxide catalysts synthesized via a straightforward coprecipitation method. Notably, the Cu-Mn/SiO2 catalyst exhibited remarkable performance on ozone decomposition, achieving 98% ozone conversion and stability for 10 h. Further characterization analysis indicated that the catalyst’s enhanced water resistance and activity could be attributed to factors such as an increased number of active sites, a large surface area, abundant active oxygen species, and a lower Mn oxidation state. The catalytic environment created by mixed oxides can offer a clearer understanding of their synergistic effects on catalytic ozone decomposition, providing significant insights into the development of water-resistant catalysts with superior performance. The escalating levels of surface ozone concentration pose detrimental effects on public health and the environment. Catalytic decomposition presents an optimal solution for surface ozone removal. Nevertheless, catalyst still encounters challenges such as poisoning and deactivation in the high humidity environment. The influence of support on catalytic ozone decomposition was examined at a gas hourly space velocity of 300 L·g −1 ·h −1 and 85% relative humidity under ambient temperature using Cu-Mn–doped oxide catalysts synthesized via a straightforward coprecipitation method. Notably, the Cu-Mn/SiO 2 catalyst exhibited remarkable performance on ozone decomposition, achieving 98% ozone conversion and stability for 10 h. Further characterization analysis indicated that the catalyst’s enhanced water resistance and activity could be attributed to factors such as an increased number of active sites, a large surface area, abundant active oxygen species, and a lower Mn oxidation state. The catalytic environment created by mixed oxides can offer a clearer understanding of their synergistic effects on catalytic ozone decomposition, providing significant insights into the development of water-resistant catalysts with superior performance. Graphical Abstract |
Author | Li, Yunhe Sun, Tianjun Zhao, Baogang Ma, Yanming Li, Hao Liang, Peiyuan |
Author_xml | – sequence: 1 givenname: Yunhe surname: Li fullname: Li, Yunhe organization: Marine Engineering College, Dalian Maritime University – sequence: 2 givenname: Hao surname: Li fullname: Li, Hao organization: Environmental Science and Engineering College, Dalian Maritime University – sequence: 3 givenname: Baogang surname: Zhao fullname: Zhao, Baogang email: zhaobg2008@163.com organization: Marine Engineering College, Dalian Maritime University – sequence: 4 givenname: Yanming surname: Ma fullname: Ma, Yanming organization: Marine Engineering College, Dalian Maritime University – sequence: 5 givenname: Peiyuan surname: Liang fullname: Liang, Peiyuan organization: Marine Engineering College, Dalian Maritime University – sequence: 6 givenname: Tianjun surname: Sun fullname: Sun, Tianjun organization: Marine Engineering College, Dalian Maritime University |
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Keywords | spinel CuMn Oxidation states Support modified Water resistance Catalytic decomposition O Oxygen vacancy CuMn2O4 spinel |
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SubjectTerms | Ambient temperature Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Catalysis Catalysts Chemical synthesis Copper Copper - chemistry Decomposition Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Humidity Manganese Manganese - chemistry Mixed oxides Oxidation Oxidation-Reduction Oxides - chemistry Ozone Ozone - chemistry Public health Relative humidity Research Article Silicon dioxide Stability analysis Synergistic effect Valence Waste Water Technology Water Management Water Pollution Control Water resistance |
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Title | Synthetic effect of supports in Cu-Mn–doped oxide catalysts for promoting ozone decomposition under humid environment |
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