Enhanced thermoelectric properties of Cu1.8S by Ti-doping induced secondary phase
Cu1.8S is a promising thermoelectric material with characteristics of superionic conductors. This study has been focused on the effect of Ti4+ doping on both electron and phonon transport properties of TixCu1.8-xS (x = 0, 0.04, 0.07, 0.10). The thermoelectric figure of merit (ZT) was greatly enhance...
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| Published in | Journal of alloys and compounds Vol. 731; pp. 577 - 583 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.01.2018
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| Abstract | Cu1.8S is a promising thermoelectric material with characteristics of superionic conductors. This study has been focused on the effect of Ti4+ doping on both electron and phonon transport properties of TixCu1.8-xS (x = 0, 0.04, 0.07, 0.10). The thermoelectric figure of merit (ZT) was greatly enhanced when 0.07 ≤ x ≤ 0.10, mainly due to a decreased thermal conductivity (0.62–0.77 Wm−1K−1) caused by the formation of the lower-conductive Cu4(TiS4) and Cu1.96S second phases, and the introduced point defects. Along with an improved Seebeck coefficient, a peak ZT value of 0.54 at 673 K was obtained in the Ti0.07Cu1.73S composition, which is twice as large as that of the undoped one. A maximum efficiency of about 3.7% at Th = 673 K with a proper output power density (Pd∼0.56 Wcm−2) was obtained. Our results indicate that the introduction of Ti4+ in copper sulfide thermoelectric materials is an effective and convenient strategy to improve ZT by decreasing thermal conductivity.
•An improved α and low κ (0.62–0.77 Wm−1K−1) produced by the second phases by adding Ti4+ in Cu1.8S.•The highest ZT up to 0.54 at 673 K is twice as large as that of the undoped one.•A maximum efficiency of 3.7% at Th = 673 K with a proper Pd∼0.56 Wcm−2 was obtained. |
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| AbstractList | Cu1.8S is a promising thermoelectric material with characteristics of superionic conductors. This study has been focused on the effect of Ti4+ doping on both electron and phonon transport properties of TixCu1.8-xS (x = 0, 0.04, 0.07, 0.10). The thermoelectric figure of merit (ZT) was greatly enhanced when 0.07 ≤ x ≤ 0.10, mainly due to a decreased thermal conductivity (0.62–0.77 Wm−1K−1) caused by the formation of the lower-conductive Cu4(TiS4) and Cu1.96S second phases, and the introduced point defects. Along with an improved Seebeck coefficient, a peak ZT value of 0.54 at 673 K was obtained in the Ti0.07Cu1.73S composition, which is twice as large as that of the undoped one. A maximum efficiency of about 3.7% at Th = 673 K with a proper output power density (Pd∼0.56 Wcm−2) was obtained. Our results indicate that the introduction of Ti4+ in copper sulfide thermoelectric materials is an effective and convenient strategy to improve ZT by decreasing thermal conductivity.
•An improved α and low κ (0.62–0.77 Wm−1K−1) produced by the second phases by adding Ti4+ in Cu1.8S.•The highest ZT up to 0.54 at 673 K is twice as large as that of the undoped one.•A maximum efficiency of 3.7% at Th = 673 K with a proper Pd∼0.56 Wcm−2 was obtained. |
| Author | Zhang, Bo-Ping Liang, Dou-Dou Zou, Liang |
| Author_xml | – sequence: 1 givenname: Dou-Dou surname: Liang fullname: Liang, Dou-Dou – sequence: 2 givenname: Bo-Ping surname: Zhang fullname: Zhang, Bo-Ping email: bpzhang@ustb.edu.cn – sequence: 3 givenname: Liang surname: Zou fullname: Zou, Liang |
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| Snippet | Cu1.8S is a promising thermoelectric material with characteristics of superionic conductors. This study has been focused on the effect of Ti4+ doping on both... |
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| SubjectTerms | Cu1.8S Superionic Thermoelectric Ti4+ doping |
| Title | Enhanced thermoelectric properties of Cu1.8S by Ti-doping induced secondary phase |
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