Self-assembled carbon nitride/cobalt (III) porphyrin photocatalyst for mimicking natural photosynthesis
Natural photosynthesis is the primary route that supplies energy required for the endurance of all living things. The initial step in this process is the absorption of solar light by an organic-inorganic molecular organization called a light harvesting complex. This complicated natural solar energy...
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| Published in | Diamond and related materials Vol. 101; p. 107648 |
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| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
01.01.2020
Elsevier BV |
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| Online Access | Get full text |
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| Abstract | Natural photosynthesis is the primary route that supplies energy required for the endurance of all living things. The initial step in this process is the absorption of solar light by an organic-inorganic molecular organization called a light harvesting complex. This complicated natural solar energy conversion platform has inspired scientists to create artificial counter parts. As a means to achieve this, a self-assembled light harvesting carbon nitride/cobalt tetra-phenyl-porphyrin (CN/Co(III)TPP) material as a highly selective solar light active photocatalyst has been developed. The system exhibited excellent NADH regeneration (87.87%) and L-glutamate (94.30%) production under visible light irradiation. The current research endeavor highlights the development and application of a self-assembled CN/Co(III)TPP photocatalyst for the selective production of L-glutamate from α-ketoglutarate.
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•A self-assembled light harvesting carbon nitride/cobalt tetra-phenyl-porphyrin (CN/Co(III)TPP) photocatalyst was synthesized•As prepared photocatalyst is characterized by several characterization techniques to determine physio-chemical properties.•Visible light active CN/Co(III)TPP photocatalyst is used for 1,4-NADH regeneration and L-glutamate production.•The yield of NADH regeneration and L-glutamate production were found to be 87.9% and 94.3%, respectively in 60 min. |
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| AbstractList | Natural photosynthesis is the primary route that supplies energy required for the endurance of all living things. The initial step in this process is the absorption of solar light by an organic-inorganic molecular organization called a light harvesting complex. This complicated natural solar energy conversion platform has inspired scientists to create artificial counter parts. As a means to achieve this, a self-assembled light harvesting carbon nitride/cobalt tetra-phenyl-porphyrin (CN/Co(III)TPP) material as a highly selective solar light active photocatalyst has been developed. The system exhibited excellent NADH regeneration (87.87%) and L-glutamate (94.30%) production under visible light irradiation. The current research endeavor highlights the development and application of a self-assembled CN/Co(III)TPP photocatalyst for the selective production of L-glutamate from α-ketoglutarate. Natural photosynthesis is the primary route that supplies energy required for the endurance of all living things. The initial step in this process is the absorption of solar light by an organic-inorganic molecular organization called a light harvesting complex. This complicated natural solar energy conversion platform has inspired scientists to create artificial counter parts. As a means to achieve this, a self-assembled light harvesting carbon nitride/cobalt tetra-phenyl-porphyrin (CN/Co(III)TPP) material as a highly selective solar light active photocatalyst has been developed. The system exhibited excellent NADH regeneration (87.87%) and L-glutamate (94.30%) production under visible light irradiation. The current research endeavor highlights the development and application of a self-assembled CN/Co(III)TPP photocatalyst for the selective production of L-glutamate from α-ketoglutarate. [Display omitted] •A self-assembled light harvesting carbon nitride/cobalt tetra-phenyl-porphyrin (CN/Co(III)TPP) photocatalyst was synthesized•As prepared photocatalyst is characterized by several characterization techniques to determine physio-chemical properties.•Visible light active CN/Co(III)TPP photocatalyst is used for 1,4-NADH regeneration and L-glutamate production.•The yield of NADH regeneration and L-glutamate production were found to be 87.9% and 94.3%, respectively in 60 min. |
| ArticleNumber | 107648 |
| Author | Shambhavi Pandey, Gajanan Kumar, Utkarsh Yadav, B.C. Singh, Chandani Sharma, Kavita Chaubey, Surabhi Singh, Pooja Baeg, Jin-Ook Kumar, Abhishek Yadav, Rajesh K. Dwivedi, D.K. |
| Author_xml | – sequence: 1 givenname: Chandani surname: Singh fullname: Singh, Chandani organization: Department of Chemistry and Environmental Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 2 givenname: Surabhi surname: Chaubey fullname: Chaubey, Surabhi organization: Department of Chemistry and Environmental Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 3 givenname: Pooja surname: Singh fullname: Singh, Pooja organization: Department of Chemistry and Environmental Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 4 givenname: Kavita surname: Sharma fullname: Sharma, Kavita organization: Department of Chemistry and Environmental Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 5 surname: Shambhavi fullname: Shambhavi organization: Department of Chemistry and Environmental Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 6 givenname: Abhishek surname: Kumar fullname: Kumar, Abhishek organization: Department of Chemistry, Indian Institute of Technology Delhi, Hauz Khas, New Delhi 110016, India – sequence: 7 givenname: Rajesh K. surname: Yadav fullname: Yadav, Rajesh K. email: rajeshkr_yadav2003@yahoo.co.in organization: Department of Chemistry and Environmental Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 8 givenname: D.K. surname: Dwivedi fullname: Dwivedi, D.K. organization: Department of Physics and Material Science, Madan Mohan Malaviya University of Technology, Gorakhpur 273010, UP, India – sequence: 9 givenname: Jin-Ook surname: Baeg fullname: Baeg, Jin-Ook organization: Artificial Photosynthesis Research Group, Korea Research Institute of Technology, 100-Jang-dong, Yuseong-gu, Daejeon 305-600, Republic of Korea – sequence: 10 givenname: Utkarsh surname: Kumar fullname: Kumar, Utkarsh organization: Department of Chemistry and Physics, Babasaheb Bhimrao Ambedkar University (A Central University), Lucknow 226025, UP, India – sequence: 11 givenname: B.C. surname: Yadav fullname: Yadav, B.C. organization: Department of Chemistry and Physics, Babasaheb Bhimrao Ambedkar University (A Central University), Lucknow 226025, UP, India – sequence: 12 givenname: Gajanan surname: Pandey fullname: Pandey, Gajanan organization: Department of Chemistry and Physics, Babasaheb Bhimrao Ambedkar University (A Central University), Lucknow 226025, UP, India |
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| Keywords | 1,4-NADH regeneration carbon nitride catalytic processes morphology L-glutamate production |
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| SubjectTerms | 1,4-NADH regeneration Carbon Carbon nitride catalytic processes Cobalt Endurance L-glutamate production Light irradiation morphology Nicotinamide adenine dinucleotide Photocatalysts Photosynthesis Regeneration Self-assembly Solar energy conversion |
| Title | Self-assembled carbon nitride/cobalt (III) porphyrin photocatalyst for mimicking natural photosynthesis |
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