Application of sulfonium-, thiophenium-, and thioxonium-based salts as electric double-layer capacitor electrolytes
The purpose of this paper is to develop novel molten salts based on sulfonium, thiophenium, and thioxonium cations as electrolytes for EDLCs. We evaluated various kinds of the salts, with tetrafluoroborate (BF 4) and bis(trifluorometanesulfonyl)amide (TFSA) anions, including several kinds of ionic l...
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| Published in | Journal of power sources Vol. 195; no. 19; pp. 6970 - 6976 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier B.V
01.10.2010
Elsevier |
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| Abstract | The purpose of this paper is to develop novel molten salts based on sulfonium, thiophenium, and thioxonium cations as electrolytes for EDLCs. We evaluated various kinds of the salts, with tetrafluoroborate (BF
4) and bis(trifluorometanesulfonyl)amide (TFSA) anions, including several kinds of ionic liquids. The cell using the electrolyte containing diethylmethylsulfonium (DEMS)–BF
4 salt had the higher capacitance and the lower DC-IR value than those containing conventional salts such as 1-ethyl-3-methylimidazolium (EMI)–BF
4 and
N,
N,
N-triethyl-
N-methylammonium (TEMA)–BF
4 at 243
K and 2
V. The capacitance and DC-IR at low temperature depended strongly on the structure, particularly on the size of each ion. We also examined the durability of cells by continuous charging at 333
K and 2.5
V. The stabilities of sulfonium-, thiophenium-, and thioxonium-based electrolytes were much inferior to that of EMI–BF
4. |
|---|---|
| AbstractList | The purpose of this paper is to develop novel molten salts based on sulfonium, thiophenium, and thioxonium cations as electrolytes for EDLCs. We evaluated various kinds of the salts, with tetrafluoroborate (BF sub(4)) and bis(trifluorometanesulfonyl)amide (TFSA) anions, including several kinds of ionic liquids. The cell using the electrolyte containing diethylmethylsulfonium (DEMS)-BF sub(4) salt had the higher capacitance and the lower DC-IR value than those containing conventional salts such as 1-ethyl-3-methylimidazolium (EMI)-BF sub(4) and N,N,N-triethyl-N-methylammonium (TEMA)-BF sub(4) at 243 K and 2 V. The capacitance and DC-IR at low temperature depended strongly on the structure, particularly on the size of each ion. We also examined the durability of cells by continuous charging at 333 K and 2.5 V. The stabilities of sulfonium-, thiophenium-, and thioxonium-based electrolytes were much inferior to that of EMI-BF sub(4). The purpose of this paper is to develop novel molten salts based on sulfonium, thiophenium, and thioxonium cations as electrolytes for EDLCs. We evaluated various kinds of the salts, with tetrafluoroborate (BF 4) and bis(trifluorometanesulfonyl)amide (TFSA) anions, including several kinds of ionic liquids. The cell using the electrolyte containing diethylmethylsulfonium (DEMS)–BF 4 salt had the higher capacitance and the lower DC-IR value than those containing conventional salts such as 1-ethyl-3-methylimidazolium (EMI)–BF 4 and N, N, N-triethyl- N-methylammonium (TEMA)–BF 4 at 243 K and 2 V. The capacitance and DC-IR at low temperature depended strongly on the structure, particularly on the size of each ion. We also examined the durability of cells by continuous charging at 333 K and 2.5 V. The stabilities of sulfonium-, thiophenium-, and thioxonium-based electrolytes were much inferior to that of EMI–BF 4. |
| Author | Yoshida, M. Orita, A. Kamijima, K. Yang, L. |
| Author_xml | – sequence: 1 givenname: A. surname: Orita fullname: Orita, A. email: a-orita@hitachi-chem.co.jp organization: Research & Development Center, Hitachi Chemical Co., Ltd., 1380-1 Tarazaki, Hitachinaka-shi, Ibaraki 312-0003, Japan – sequence: 2 givenname: K. surname: Kamijima fullname: Kamijima, K. organization: Research & Development Center, Hitachi Chemical Co., Ltd., 1380-1 Tarazaki, Hitachinaka-shi, Ibaraki 312-0003, Japan – sequence: 3 givenname: M. surname: Yoshida fullname: Yoshida, M. organization: Research & Development Center, Hitachi Chemical Co., Ltd., 1380-1 Tarazaki, Hitachinaka-shi, Ibaraki 312-0003, Japan – sequence: 4 givenname: L. surname: Yang fullname: Yang, L. organization: School of Chemistry and Chemical Technology, Shanghai Jiaotong University, China |
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| Keywords | Electrolyte Capacitor EDLC Sulfonium Molten salt Thiophenium Supercapacitor Electrolytic capacitor Double layers |
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| Snippet | The purpose of this paper is to develop novel molten salts based on sulfonium, thiophenium, and thioxonium cations as electrolytes for EDLCs. We evaluated... |
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| SubjectTerms | Applied sciences Capacitor Capacitors. Resistors. Filters EDLC Electrical engineering. Electrical power engineering Electrolyte Exact sciences and technology Molten salt Sulfonium Thiophenium Various equipment and components |
| Title | Application of sulfonium-, thiophenium-, and thioxonium-based salts as electric double-layer capacitor electrolytes |
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