Resonance Raman study of ring deuterated 4-dimethylaminobenzonitrile (DMABN-d 4): the ground, ICT and triplet states

Picosecond and nanosecond time-resolved resonance Raman spectra of the intramolecular charge transfer (ICT) and triplet state of DMABN-d 4 have been obtained over the frequency range from 650 to 2250 cm −1. The spectra and the isotopic shifts observed on going from normal DMABN to the ring deuterate...

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Published inJournal of photochemistry and photobiology. A, Chemistry. Vol. 142; no. 2; pp. 177 - 185
Main Authors Ma, C, Kwok, W.M, Matousek, P, Parker, A.W, Phillips, D, Toner, W.T, Towrie, M
Format Journal Article
LanguageEnglish
Published Elsevier B.V 14.09.2001
Subjects
4-Dimethylaminobenzonitrile (DMABN)
Intramolecular charge transfer reaction
TICT
Triplet state
Intramolecular charge transfer reaction
TICT
Triplet state
4-Dimethylaminobenzonitrile (DMABN)
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Abstract Picosecond and nanosecond time-resolved resonance Raman spectra of the intramolecular charge transfer (ICT) and triplet state of DMABN-d 4 have been obtained over the frequency range from 650 to 2250 cm −1. The spectra and the isotopic shifts observed on going from normal DMABN to the ring deuterated analogue are interpreted with the aid of DFT vibrational analysis of ground state spectra and comparisons made with closely related compounds. The data confirm our previous results but the isotopic shifts induced by the ring deuteration provide additional evidence clarifying the planar structure of the triplet state and indicating full localisation of negative charge on the cyano group.
AbstractList Picosecond and nanosecond time-resolved resonance Raman spectra of the intramolecular charge transfer (ICT) and triplet state of DMABN-d 4 have been obtained over the frequency range from 650 to 2250 cm −1. The spectra and the isotopic shifts observed on going from normal DMABN to the ring deuterated analogue are interpreted with the aid of DFT vibrational analysis of ground state spectra and comparisons made with closely related compounds. The data confirm our previous results but the isotopic shifts induced by the ring deuteration provide additional evidence clarifying the planar structure of the triplet state and indicating full localisation of negative charge on the cyano group.
Author Matousek, P
Ma, C
Parker, A.W
Kwok, W.M
Toner, W.T
Towrie, M
Phillips, D
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Keywords Intramolecular charge transfer reaction
TICT
Triplet state
4-Dimethylaminobenzonitrile (DMABN)
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SSID ssj0004441
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Snippet Picosecond and nanosecond time-resolved resonance Raman spectra of the intramolecular charge transfer (ICT) and triplet state of DMABN-d 4 have been obtained...
SourceID crossref
elsevier
SourceType Aggregation Database
Publisher
StartPage 177
SubjectTerms 4-Dimethylaminobenzonitrile (DMABN)
Intramolecular charge transfer reaction
TICT
Triplet state
Title Resonance Raman study of ring deuterated 4-dimethylaminobenzonitrile (DMABN-d 4): the ground, ICT and triplet states
URI https://dx.doi.org/10.1016/S1010-6030(01)00512-3
Volume 142
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