Hyperelastic Kevlar Nanofiber Aerogels as Robust Thermal Switches for Smart Thermal Management
Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have attracted increasing interest. Aerogels exhibit single‐mode thermal insulation properties regardless of the surrounding temperature. In this s...
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Published in | Advanced materials (Weinheim) Vol. 35; no. 3; pp. e2207638 - n/a |
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Abstract | Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have attracted increasing interest. Aerogels exhibit single‐mode thermal insulation properties regardless of the surrounding temperature. In this study, hyperelastic Kevlar nanofiber aerogels (HEKAs) are designed and fabricated by a slow‐proton‐release‐modulating gelation and thermoinduced crosslinking strategy. The method does not use crosslinking agents and endows the ultralow‐density (4.7 mg cm−3) HEKAs with low thermal conductivity (0.029 W m−1 K−1), high porosity (99.75%), high thermal stability (550 °C), and increased compression resilience (80%) and fatigue resistance. Proofs of the concept of the HEKAs acting as on–off thermal switches are demonstrated through experiments and simulations. The thermal switches exhibit a rapid thermal response speed of 0.73 °C s−1, high heat flux of 2044 J m−2 s−1, and switching ratio of 7.5. Heat dissipation can be reversibly switched on/off more than fifty times owing to the hyperelasticity and fatigue resistance of the HEKAs. This study suggests a route to fulfill the hyperelasticity of highly porous aerogels and to tailor heat flux on‐demand.
Hyperelastic Kevlar nanofiber aerogels (HEKAs) are synthesized by a slow‐proton‐release‐modulating gelation and thermo‐induced crosslinking strategy. The HEKAs exhibit low thermal conductivity and ultralow density, high porosity, and compression resilience. The application of HEKAs as thermal switches is demonstrated, which exhibit high responsive speed and heat flux. The heat loss can be reversibly switched on/off over 50 times. |
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AbstractList | Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have attracted increasing interest. Aerogels exhibit single‐mode thermal insulation properties regardless of the surrounding temperature. In this study, hyperelastic Kevlar nanofiber aerogels (HEKAs) are designed and fabricated by a slow‐proton‐release‐modulating gelation and thermoinduced crosslinking strategy. The method does not use crosslinking agents and endows the ultralow‐density (4.7 mg cm−3) HEKAs with low thermal conductivity (0.029 W m−1 K−1), high porosity (99.75%), high thermal stability (550 °C), and increased compression resilience (80%) and fatigue resistance. Proofs of the concept of the HEKAs acting as on–off thermal switches are demonstrated through experiments and simulations. The thermal switches exhibit a rapid thermal response speed of 0.73 °C s−1, high heat flux of 2044 J m−2 s−1, and switching ratio of 7.5. Heat dissipation can be reversibly switched on/off more than fifty times owing to the hyperelasticity and fatigue resistance of the HEKAs. This study suggests a route to fulfill the hyperelasticity of highly porous aerogels and to tailor heat flux on‐demand. Abstract Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have attracted increasing interest. Aerogels exhibit single‐mode thermal insulation properties regardless of the surrounding temperature. In this study, hyperelastic Kevlar nanofiber aerogels (HEKAs) are designed and fabricated by a slow‐proton‐release‐modulating gelation and thermoinduced crosslinking strategy. The method does not use crosslinking agents and endows the ultralow‐density (4.7 mg cm −3 ) HEKAs with low thermal conductivity (0.029 W m −1 K −1 ), high porosity (99.75%), high thermal stability (550 °C), and increased compression resilience (80%) and fatigue resistance. Proofs of the concept of the HEKAs acting as on–off thermal switches are demonstrated through experiments and simulations. The thermal switches exhibit a rapid thermal response speed of 0.73 °C s −1 , high heat flux of 2044 J m −2 s −1 , and switching ratio of 7.5. Heat dissipation can be reversibly switched on/off more than fifty times owing to the hyperelasticity and fatigue resistance of the HEKAs. This study suggests a route to fulfill the hyperelasticity of highly porous aerogels and to tailor heat flux on‐demand. Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have attracted increasing interest. Aerogels exhibit single-mode thermal insulation properties regardless of the surrounding temperature. In this study, hyperelastic Kevlar nanofiber aerogels (HEKAs) are designed and fabricated by a slow-proton-release-modulating gelation and thermoinduced crosslinking strategy. The method does not use crosslinking agents and endows the ultralow-density (4.7 mg cm ) HEKAs with low thermal conductivity (0.029 W m K ), high porosity (99.75%), high thermal stability (550 °C), and increased compression resilience (80%) and fatigue resistance. Proofs of the concept of the HEKAs acting as on-off thermal switches are demonstrated through experiments and simulations. The thermal switches exhibit a rapid thermal response speed of 0.73 °C s , high heat flux of 2044 J m s , and switching ratio of 7.5. Heat dissipation can be reversibly switched on/off more than fifty times owing to the hyperelasticity and fatigue resistance of the HEKAs. This study suggests a route to fulfill the hyperelasticity of highly porous aerogels and to tailor heat flux on-demand. Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have attracted increasing interest. Aerogels exhibit single‐mode thermal insulation properties regardless of the surrounding temperature. In this study, hyperelastic Kevlar nanofiber aerogels (HEKAs) are designed and fabricated by a slow‐proton‐release‐modulating gelation and thermoinduced crosslinking strategy. The method does not use crosslinking agents and endows the ultralow‐density (4.7 mg cm−3) HEKAs with low thermal conductivity (0.029 W m−1 K−1), high porosity (99.75%), high thermal stability (550 °C), and increased compression resilience (80%) and fatigue resistance. Proofs of the concept of the HEKAs acting as on–off thermal switches are demonstrated through experiments and simulations. The thermal switches exhibit a rapid thermal response speed of 0.73 °C s−1, high heat flux of 2044 J m−2 s−1, and switching ratio of 7.5. Heat dissipation can be reversibly switched on/off more than fifty times owing to the hyperelasticity and fatigue resistance of the HEKAs. This study suggests a route to fulfill the hyperelasticity of highly porous aerogels and to tailor heat flux on‐demand. Hyperelastic Kevlar nanofiber aerogels (HEKAs) are synthesized by a slow‐proton‐release‐modulating gelation and thermo‐induced crosslinking strategy. The HEKAs exhibit low thermal conductivity and ultralow density, high porosity, and compression resilience. The application of HEKAs as thermal switches is demonstrated, which exhibit high responsive speed and heat flux. The heat loss can be reversibly switched on/off over 50 times. |
Author | Wu, Fushuo Cheng, Yingying Zhang, Peigen Sun, ZhengMing Wang, Jin Hu, Peiying Wang, Jing |
Author_xml | – sequence: 1 givenname: Peiying surname: Hu fullname: Hu, Peiying organization: Chinese Academy of Sciences – sequence: 2 givenname: Jing surname: Wang fullname: Wang, Jing organization: Chinese Academy of Sciences – sequence: 3 givenname: Peigen surname: Zhang fullname: Zhang, Peigen email: zhpeigen@seu.edu.cn organization: Southeast University – sequence: 4 givenname: Fushuo surname: Wu fullname: Wu, Fushuo organization: Southeast University – sequence: 5 givenname: Yingying surname: Cheng fullname: Cheng, Yingying organization: Chinese Academy of Sciences – sequence: 6 givenname: Jin orcidid: 0000-0003-1573-574X surname: Wang fullname: Wang, Jin email: jwang2014@sinano.ac.cn organization: Chinese Academy of Sciences – sequence: 7 givenname: ZhengMing surname: Sun fullname: Sun, ZhengMing email: zmsun@seu.edu.cn organization: Southeast University |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36271721$$D View this record in MEDLINE/PubMed |
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Keywords | hyperelasticity aerogels Kevlar nanofibers thermal management thermal switches |
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Snippet | Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface area, have... Abstract Aerogels, the lightest artificial solid materials characterized by low density and thermal conductivity, high porosity, and large specific surface... |
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SubjectTerms | Aerogels Aramid fibers Crosslinking Density Fatigue strength Heat conductivity Heat flux Heat transfer hyperelasticity Kevlar (trademark) Kevlar nanofibers Materials science Nanofibers Porosity Switches Thermal conductivity Thermal insulation Thermal management Thermal response Thermal simulation Thermal stability thermal switches |
Title | Hyperelastic Kevlar Nanofiber Aerogels as Robust Thermal Switches for Smart Thermal Management |
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